IP Library Granted Patent US 10,702,826
Granted Patent B2
US 10,702,826 · App. 16/216,205 · Granted Jul 7, 2020

Method and apparatus for increasing mass transfer in aqueous gas adsorption processes

Inventors: Kunlei Liu (Lexington, KY); Leland R. Widger (Lexington, KY); Zhen Fan (Lexington, KY); Joshuah Stolaroff (Lexington, KY)
Assignee: UNIVERSITY OF KENTUCKY RESEARCH FOUNDTION
B01D53/1475B01D53/1493B01D53/18B01J19/32B01D15/305B01D15/327B01D2257/504B01D2325/36B01D2325/38
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Quick Facts
Patent No.
US 10,702,826
App. No.
16/216,205
Granted
Jul 7, 2020
Kind
B2
Abstract

A method of removing and capturing an acid gas from a fluid stream includes exposing the fluid stream to an aqueous scrubbing solution in the presence of a packing element including alternating hydrophobic and hydrophilic features or zones. A related apparatus is also disclosed.

Claims (8)

1. A method of removing and capturing an acid gas from a fluid stream, comprising:

counterflowing the fluid stream against an aqueous scrubbing solution in an absorber with a packing element within, wherein the packing element comprises a first corrugated plate, a second corrugated plate and a third corrugated plate with flow channels in a stacked arrangement, the first and third corrugated plates each having perforations, wherein the second corrugated plate does not include perforations and comprises on a surface of a flow channel alternating hydrophobic and hydrophilic zones such that liquid flowing through the flow channel of the second corrugated plate creates internal turbulence in order to form a dynamically refreshing and reactive liquid-gas interface and capture acid gas from the fluid stream.

2. The method of claim 1 including recovering the acid gas captured by the aqueous scrubbing solution and regenerating the aqueous scrubbing solution.

3. The method of claim 2 wherein the fluid stream is flue gas and the acid gas is carbon dioxide.

4. The method of claim 1 , including providing said hydrophobic zones on a surface of the packing element with a width or length of between 1 mm and 100 mm.

5. The method of claim 4 , including providing said hydrophilic zones on a surface of the packing element with a width or length of between 1 mm and 100 mm.

6. The method of claim 5 , including providing a hydrophobic zone at an edge of the packing element.

7. The method of claim 6 , wherein the fluid stream is a flue gas, the acid gas is carbon dioxide and the aqueous scrubbing solution includes an aqueous amine for carbon capture.

Assignments (3)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 29, 2021
From: STOLAROFF, JOSHUAH
To: LAWRENCE LIVERMORE NATIONAL SECURITY, LLC
Reel/Frame 055754/0102 →
CONFIRMATORY LICENSE Recorded Sep 1, 2020
From: LAWRENCE LIVERMORE NATIONAL SECURITY, LLC
To: U.S. DEPARTMENT OF ENERGY
Reel/Frame 053667/0191 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 11, 2018
From: LIU, KUNLEI; WIDGER, LELAND R.; FAN, ZHEN; STOLAROFF, JOSHUAH
To: UNIVERSITY OF KENTUCKY RESEARCH FOUNDATION
Reel/Frame 047744/0562 →
Continuity (2)
Provisional Application 62597479 · Dec 12, 2017
Related Publication 20190176080A1 · Jun 13, 2019