IP Library Granted Patent US 10,892,094
Granted Patent B2
US 10,892,094 · App. 16/270,493 · Granted Jan 12, 2021

Boron nitride and method of producing boron nitride

Inventors: Narayan S. Hosmane (DeKalb, IL); Amartya Chakrabarti (Hoffman Estates, IL); Shena M. Peter (Rock Island, IL)
Assignee: Board of Trustees of Northern Illinois University
H01G4/08B82Y30/00C01B21/0646C30B7/10C30B7/105C30B29/403C30B29/60C30B29/64B82Y40/00C01P2002/72C01P2002/82C01P2004/03C01P2004/04C01P2004/24C01P2006/40C01P2006/80Y10S977/734Y10S977/842
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Quick Facts
Patent No.
US 10,892,094
App. No.
16/270,493
Granted
Jan 12, 2021
Kind
B2
Abstract

BN nanosheets are prepared by a method comprising heating to a temperature of at least 500° C., a mixture comprising: (1) an alkali borohydride, and (2) an ammonium salt. NaN 3 may be included to increase the yield. No catalyst is required, and the product produced contains less than 0.1 atomic percent metal impurities.

Claims (40)

1. h-BN nanosheets,

wherein the h-BN nanosheets contain less than 0.1 atomic percent metal impurities and have a full width at half maximum (FWHM) of the X-ray powder diffraction pattern for a d 002 peak of at most 0.50 degrees,

the h-BN nanosheets have an aspect ratio of at least 10:1, and

the h-BN nanosheets are not nanofibers.

2. The h-BN nanosheets of claim 1 , wherein the h-BN nanosheets are few layer h-BN nanosheets.

3. The h-BN nanosheets of claim 2 , wherein the h-BN nanosheets have 6 to 20 layers of BN.

4. The h-BN nanosheets of claim 1 , wherein the h-BN nanosheets do not contain r-BN, as determined by X-ray powder diffraction.

5. The h-BN nanosheets of claim 1 , wherein the h-BN nanosheets have a full width at half maximum (FWHM) of the X-ray powder diffraction pattern for a d 002 peak of at most 0.30 degrees.

6. The h-BN nanosheets of claim 1 , wherein the h-BN nanosheets have a full width at half maximum (FWHM) of the X-ray powder diffraction pattern for a d 100 peak of at most 0.50 degrees.

7. The h-BN nanosheets of claim 1 , wherein the h-BN nanosheets have a full width at half maximum (FWHM) of the X-ray powder diffraction pattern for a d 100 peak of at most 0.25 degrees.

8. The h-BN nanosheets of claim 1 , wherein the h-BN nanosheets have a particle size of 250 to 900 nm.

9. A capacitor, comprising:

(a) a substrate,

(b) a first conductive layer, on the substrate

(c) an insulating layer, on the conductive layer, and

(d) a second conductive layer, on the insulating layer,

wherein the insulating layer comprises the h-BN nanosheets of claim 1 .

10. The capacitor of claim 9 , wherein the h-BN nanosheets are few layer h-BN nanosheets.

11. The capacitor of claim 9 , wherein the h-BN nanosheets have 6 to 20 layers of BN.

12. The capacitor of claim 9 , wherein the h-BN nanosheets do not contain r-BN, as determined by X-ray powder diffraction.

13. The capacitor of claim 9 , wherein the h-BN nanosheets have a full width at half maximum (FWHM) of the X-ray powder diffraction pattern for a d 002 peak of at most 0.30 degrees.

14. The capacitor of claim 9 , wherein the h-BN nanosheets have a full width at half maximum (FWHM) of the X-ray powder diffraction pattern for a d 100 peak of at most 0.50 degrees.

15. The capacitor of claim 9 , wherein the h-BN nanosheets have a full width at half maximum (FWHM) of the X-ray powder diffraction pattern for a d 100 peak of at most 0.25 degrees.

16. The h-BN nanosheets of claim 1 ,

wherein the h-BN nanosheets have 6 to 20 layers of BN,

the h-BN nanosheets do not contain r-BN, as determined by X-ray powder diffraction, and

the h-BN nanosheets have a particle size of 250 to 900 nm.

17. The h-BN nanosheets of claim 1 ,

wherein the h-BN nanosheets have 6 to 20 layers of BN, and

the h-BN nanosheets have a full width at half maximum (FWHM) of the X-ray powder diffraction pattern for a d 100 peak of at most 0.25 degrees.

18. The h-BN nanosheets of claim 1 ,

wherein the h-BN nanosheets have a full width at half maximum (FWHM) of the X-ray powder diffraction pattern for a d 002 peak of at most 0.30 degrees, and

the h-BN nanosheets have a full width at half maximum (FWHM) of the X-ray powder diffraction pattern for a d 100 peak of at most 0.25 degrees.

19. The capacitor of claim 9 ,

wherein the h-BN nanosheets have 6 to 20 layers of BN,

the h-BN nanosheets do not contain r-BN, as determined by X-ray powder diffraction, and

the h-BN nanosheets have a particle size of 250 to 900 nm.

20. The capacitor of claim 9 ,

wherein the h-BN nanosheets have 6 to 20 layers of BN, and

the h-BN nanosheets have a full width at half maximum (FWHM) of the X-ray powder diffraction pattern for a d 100 peak of at most 0.25 degrees.

Assignments (1)
CONFIRMATORY LICENSE Recorded Mar 1, 2019
From: NORTHERN ILLINOIS UNIVERSITY
To: NATIONAL SCIENCE FOUNDATION
Reel/Frame 048479/0702 →
Continuity (3)
Continuation 15100217
Provisional Application 61909912 · Nov 27, 2013
Related Publication 20190244756A1 · Aug 8, 2019