IP Library Granted Patent US 10,975,011
Granted Patent B2
US 10,975,011 · App. 16/291,602 · Granted Apr 13, 2021

Ether blends via reactive distillation

Inventors: Ian Lawrence Gaffney (Los Gatos, CA); Evan Michael Visser (Hull, IA); Krishna K. Rao (The Woodlands, TX); Walter Breidenstein (Boyne Falls, MI)
Assignee: GAS TECHNOLOGIES LLC
C07C41/42B01D3/009B01J8/02B01J12/00C07C29/50C07C31/04C07C31/08C07C41/09C07C43/04C07C43/043C07C43/06B01J2208/00805Y02P20/10
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Quick Facts
Patent No.
US 10,975,011
App. No.
16/291,602
Granted
Apr 13, 2021
Kind
B2
Abstract

A method for forming a blend of ethers from a blend of alcohols includes a step of reacting a hydrocarbon-containing gas with an oxygen-containing gas to form first product blend. The first product blend includes a blend of partially oxygenated compounds. The blend of partially oxygenated compounds is provided to a reactive distillation station where it is converted a second product blend. The second product blend typically includes a mixture of ethers. An apparatus implementing the method is also provided.

Claims (19)

1. A method for forming a blend of ethers from a blend of partially oxygenated compounds, the method comprising:

a) reacting a hydrocarbon-containing gas with an oxygen-containing gas to form first product blend in a reactor, the first product blend including a blend of partially oxygenated compounds;

b) providing the blend of partially oxygenated compounds to a reactive distillation station through one or more conduits after formaldehyde has been removed; and

c) converting the blend of partially oxygenated compounds to a second product blend at the reactive distillation station, the second product blend including a mixture of ethers.

2. The method of claim 1 wherein the hydrocarbon-containing gas includes C 1-10 alkanes.

3. The method of claim 1 wherein the hydrocarbon-containing gas includes an alkane selected from the group consisting of methane, ethane, propanes, butanes, pentanes and combinations thereof.

4. The method of claim 1 wherein the hydrocarbon-containing gas includes an alkane selected from the group consisting of methane, ethane, and combinations thereof.

5. The method of claim 1 wherein the first product blend includes C 1-10 alcohols.

6. The method of claim 5 wherein the first product blend includes an alcohol selected from the group consisting of methanol, ethanol, propanols, butanols, pentanols and combinations thereof.

7. The method of claim 1 wherein the first product blend includes an alcohol selected from the group consisting of methanol, ethanol, and combinations thereof.

8. The method of claim 1 wherein the second product blend includes a mixture of C 2-20 alkyl ethers.

9. The method of claim 8 wherein the second product blend includes an ether selected from the group consisting of dimethyl ether, diethyl ether, methylethyl ether, dipropyl ether, methyl propyl ether, ethyl propyl ether, dipropyl ether, methyl butyl ether, propylbutyl ether, dibutylyether, and combinations thereof.

10. The method of claim 8 wherein the second product blend includes an ether selected from the group consisting of dimethyl ether, diethyl ether, methylethyl ether, and combinations thereof.

11. The method of claim 9 wherein the second product blend includes a component selected from the group consisting of C 2-10 esters, methylene glycol ethers, and combinations thereof.

12. The method of claim 9 wherein the second product blend includes formaldehyde.

13. The method of claim 12 further comprising a step of separating the formaldehyde from the second product blend.

14. The method of claim 1 wherein the oxygen-containing gas comprises oxygen.

15. The method of claim 1 wherein the reactive distillation station includes a catalyst packed column having a catalyst that converts alcohols to ethers.

16. The method of claim 15 wherein the catalyst is selected from the group consisting of aluminosilicate catalysts, copper modified alumina catalyst, and combinations thereof.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 10, 2025
From: GAS TECHNOLOGIES LLC
To: GASTECHNO CORP.
Reel/Frame 071374/0823 →
Continuity (4)
Continuation 15660149 · Jul 26, 2017
Division 14777022
Continuation In Part 13843471 · Mar 15, 2013
Related Publication 20190194103A1 · Jun 27, 2019
Cited By (1)
US 12,292,009