IP Library Granted Patent US 10,933,070
Granted Patent B2
US 10,933,070 · App. 16/299,254 · Granted Mar 2, 2021

Heterocyclic amides as kinase inhibitors

Inventors: Jae U. Jeong (Collegeville, PA); Deepak Bandyopadhyay (King of Prussia, PA); Patrick M. Eidam (Collegeville, PA); Philip Anthony Harris (Collegeville, PA); Jianxing Kang (Collegeville, PA); Bryan Wayne King (Collegeville, PA); Ami Lakdawala Shah (Collegeville, PA); Lara Kathryn Leister (Collegeville, PA); Attiq Rahman (Collegeville, PA); Joshi M. Ramanjulu (Collegeville, PA); Clark A. Sehon (Collegeville, PA); Robert Singhaus, Jr. (Collegeville, PA); Daohua Zhang (Collegeville, PA)
Assignee: GlaxoSmithKline Intellectual Property Development Limited
A61K31/553A61K31/55A61K31/551C07D223/08C07D267/14C07D281/10C07D403/12C07D403/14C07D409/12C07D413/12C07D413/14C07D417/12C07D487/04C07D498/04
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Quick Facts
Patent No.
US 10,933,070
App. No.
16/299,254
Granted
Mar 2, 2021
Kind
B2
Abstract

Disclosed are compounds having the formula: wherein X, Y, Z 1 , Z 2 , Z 3 , Z 4 , R 5 , R A , m, A. L, and B are as defined herein, and methods of making and using the same.

Claims (25)

1. A compound according to Formula (I):

or pharmaceutically acceptable salt thereof, wherein:

X is NH;

Y is CH 2 or CH 2 CH 2 ;

Z 1 , Z 2 , Z 3 , and Z 4 are each CH; or

Z 1 is CR 1 and Z 2 , Z 3 and Z 4 are each CH; or

Z 1 , Z 2 , and Z 4 are each CH and Z 3 is CR 3 ; or

Z 1 , Z 3 , and Z 4 are each CH and Z 2 is CR 2 ; or

Z 1 , Z 2 , and Z 3 are each CH and Z 4 is CR 4 ; or

Z 1 and Z 3 are CH, Z 2 is CR 2 , and Z 4 is CR 4 ;

or Z 1 and Z 3 are both N, Z 2 is CH and Z 4 is CH or CR 4 ; or

Z 1 is N, Z 2 is CR 2 and Z 3 and Z 4 are CH; or

Z 3 is N, and Z 2 , Z 3 and Z 4 are CH;

R 1 is methyl,

R 2 is chloro, bromo, —CN, —CH 3 , OH, B(OH) 2 , CF 3 C(OH) 2 , CH 3 OCH 2 CH 2 O—, 5H-tetrazol-5-yl, pyrazol-3-yl, or 5-methyl-1,3,4-oxadiazol-2-yl;

R 3 is fluoro, chloro, bromo, —OCH 3 , B(OH) 2 , —COOH, CH 3 SO 2 —, CH 3 SO 2 NHC(O)—, CH 3 C(O)NH—, (CH 3 ) 2 NC(O)—, CH 3 OC(O)—, (CH 3 )C(O)N(CH 3 )—, HOCH 2 CH 2 C(O)NH—, CH 3 OCH 2 CH 2 NHC(O)NH—, CH 3 SO 2 CH 2 CH 2 NHC(O)—, CH 3 CH 2 NHC(O)NH—, CH 3 OC(O)NH—, morpholin-4-yl-CO—, pyrrolidin-1-yl-CH 2 CH 2 NHC(O)—, tetrahydrofuran-2-yl-CH 2 O—, pyrrolidin-1-yl-CH 2 CH 2 O—, tetrazol-5-yl, 1-(2-cyanoethyl)-tetrazol-5-yl, pyrazol-1-yl, pyrazol-3-yl, 1-methyl-pyrazol-3-yl, 1-methyl-pyrrol-4-yl-C(O)NH—, or 5-oxo-4,5-dihydro-1,3,4-oxadiazol-2-yl;

R 4 is fluoro or methyl;

A is furyl, thienyl, oxazolyl, isoxazolyl, thiazolyl, 1,2,4-oxadiazolyl, 1,3,4-oxadiazolyl, pyrrolyl, pyrazolyl, imidazolyl, 1,2,3-triazolyl, 1,2,4-triazolyl, tetrazolyl, piperidinyl, pyrrolidinyl, phenyl or pyridyl;

m is 0 or m is 1 and R A is methyl;

L is O, S, N(CH 3 ), CH 2 , CH 2 CH 2 , CH(CH 3 ), CF 2 , CH 2 O, CH 2 N(CH 3 ), or CH(OH); and

B is thien-2-yl, pyrazol-1-yl, 3,5-dimethylpyrazol-1-yl, 4-methylpyrazol-1-yl, 3,5-dimethylisoxazol-4-yl, tetrahydrofuran-2-yl, morpholin-4-yl, pyridin-2-yl, 2-oxo-pyridin-1-yl, 6-methylpyridin-3-yl, 2-methylpyrimidin-5-yl, cyclopentyl, cyclohexyl, phenyl, 2-methylphenyl, 4-methylphenyl, 2-trifluoromethylphenyl, 2-fluorophenyl, 3-fluorophenyl, 4-fluorophenyl, 2-iodophenyl, 3-bromophenyl, 4-bromophenyl, 4-chlorophenyl, 2,5-difluorophenyl, 2,4-difluorophenyl, 3,4-difluorophenyl, 3,5-difluorophenyl, or 4-methoxyphenyl;

or -L-B is OCH 2 CH═CH 2 , —CH 2 CH 2 CH 2 CH 2 CH 3 , —OCH 2 CH 2 CH 2 CH 3 , —CH 2 CH 2 CH 3 , or —CH 2 CH(CH 3 ) 2 .

2. The compound according to claim 1 , or pharmaceutically acceptable salt thereof, wherein Y is CH 2 .

3. A pharmaceutical composition comprising the compound according to claim 1 , or pharmaceutically acceptable salt thereof, and one or more pharmaceutically acceptable excipients.

4. A method of treating a RIP1 kinase mediated disease or disorder comprising administering a therapeutically effective amount of the compound or pharmaceutically acceptable salt thereof, according to claim 1 to a human in need thereof, wherein the disease or disorder is selected from ulcerative colitis, Crohn's disease, rheumatoid arthritis, psoriasis, spondyloarthritis, systemic onset juvenile idiopathic arthritis, psoriatic arthritis, osteoarthritis, multiple sclerosis, sepsis, ischemia reperfusion injury of solid organs, and systemic inflammatory response syndrome.

Assignments (2)
CHANGE OF ADDRESS Recorded Oct 8, 2025
From: GLAXOSMITHKLINE INTELLECTUAL PROPERTY DEVELOPMENT LIMITED
To: GLAXOSMITHKLINE INTELLECTUAL PROPERTY DEVELOPMENT LIMITED
Reel/Frame 073032/0390 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 12, 2019
From: BANDYOPADHYAY, DEEPAK; EIDAM, PATRICK M.; GOUGH, PETER J.; HARRIS, PHILIP ANTHONY; JEONG, JAE U.; KANG, JIANXING; KING, BRYAN WAYNE; LAKDAWALA SHAH, AMI; LEISTER, LARA KATHRYN; MARQUIS, ROBERT W., JR.; RAHMAN, ATTIQ; RAMANJULU, JOSHI M.; SEHON, CLARK A.; SINGHAUS, ROBERT, JR.; ZHANG, DAOHUA
To: GLAXOSMITHKLINE INTELLECTUAL PROPERTY DEVELOPMENT LIMITED
Reel/Frame 048569/0288 →
Continuity (7)
Continuation 15835747 · Dec 8, 2017
Continuation 15459141 · Mar 15, 2017
Continuation 15271581 · Sep 21, 2016
Continuation 14763183
Provisional Application 61790044 · Mar 15, 2013
Provisional Application 61765664 · Feb 15, 2013
Related Publication 20190201413A1 · Jul 4, 2019