IP Library Granted Patent US 11,123,465
Granted Patent B2
US 11,123,465 · App. 16/303,687 · Granted Sep 21, 2021

Methods of using thermally expanded graphite to remove proteins from blood and to treat sepsis

Inventors: Yury Gogotsi (Warminster, PA); Vadym Mochalin (Rolla, MO); Nicholas Pescatore (Ambler, PA)
Assignee: Drexel University
A61M1/3486B01J20/205B01J20/28083B01J20/28085B01J20/321A61M2202/0445A61M2202/07
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Quick Facts
Patent No.
US 11,123,465
App. No.
16/303,687
Granted
Sep 21, 2021
Kind
B2
Abstract

The present disclosure is directed to methods of removing proteins, including cytokines, from blood and blood products, the methods comprising contacting the blood or blood product with a form of carbon having high graphitic contents and slit-shaped mesopores and macropores, the pore size dimensions chosen to be comparable to the size of the proteins, wherein the contacting results in the removal of high levels of the protein from the blood or blood product in minutes or hours.

Claims (12)

1. A method of removing proteins or peptides from blood or a blood product, the method comprising contacting the blood or blood product with a carbon form having slit-shaped mesopores and macropores, the pore size dimensions chosen to be comparable to the size of the proteins or peptides, wherein the carbon form comprises thermally expanded graphite (TEG), and wherein the contacting results in the removal of at least 80% of the protein or the peptide from the blood or blood product in less than 120 minutes.

2. The method of claim 1 , wherein the protein or the peptide has a molecular weight in a range of from 5 to 60 kDa.

3. The method of claim 1 , wherein the protein/peptide is a cytokine.

4. The method of claim 3 , wherein the cytokine is a chemokine, interferon, interleukin, lymphokine, or tumour necrosis factor.

5. The method of claim 1 , wherein the protein is IL-6, IL-8, or TNF-α, lymphotoxin-α (aka TNF-β).

6. The method of claim 1 , wherein at least 80% of the protein or the peptide is removed from the blood or blood product in less than 60 minutes.

7. The method of claim 1 , wherein the carbon form is dispersed within a polymer composite.

8. The method of claim 1 , wherein the protein is or comprises IL-6.

9. The method of claim 1 , wherein the protein is or comprises IL-8.

10. The method of claim 1 , wherein the protein is or comprises TNF-α.

11. A method of treating sepsis in a patient in need thereof, comprising performing the method of claim 1 to the blood of the patient.

12. The method of claim 11 , wherein the blood or blood products are processed through a hemoperfusion cartridge.

Assignments (3)
CONFIRMATORY LICENSE Recorded Apr 25, 2019
From: DREXEL UNIVERSITY
To: NATIONAL SCIENCE FOUNDATION
Reel/Frame 050391/0811 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 21, 2018
From: MOCHALIN, VADYM N.; GOGOTSI, YURY; PESCATORE, NICHOLAS
To: DREXEL UNIVERSITY
Reel/Frame 047559/0612 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 21, 2018
From: MOCHALIN, VADYM N.; GOGOTSI, YURY; PESCATORE, NICHOLAS
To: DREXEL UNIVERSITY
Reel/Frame 047559/0667 →
Continuity (3)
Provisional Application 62353078 · Jun 22, 2016
Provisional Application 62341661 · May 26, 2016
Related Publication 20200316281A1 · Oct 8, 2020