IP Library Granted Patent US 11,484,507
Granted Patent B2
US 11,484,507 · App. 16/466,566 · Granted Nov 1, 2022

Polymeric nanoparticles providing nucleic acids encoding TNF-α

Inventors: Surender Kharbanda (Natick, MA); Vasundhara Shukla (Ghaziabad Up, IN); Donald Kufe (Wellesley, MA); Harpal Singh (New Delhi, IN)
Assignee: Hillstream BioPharma, Inc.
A61K9/5153A61K38/191A61K45/06A61K47/6455A61K47/6937A61P35/00C07K14/525C07K14/7151
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Quick Facts
Patent No.
US 11,484,507
App. No.
16/466,566
Granted
Nov 1, 2022
Kind
B2
Abstract

The present invention relates to polymeric nanoparticles comprising a cytokine or a nucleic acid encoding for a cytokine, pharmaceutical compositions comprising the same, and methods for treating certain diseases comprising administering these polymeric nanoparticles to a subject in need thereof.

Claims (38)

1. A composition comprising

a) polymeric nanoparticles comprising poly(lactic acid)-poly(ethylene glycol)-poly(propylene glycol)-poly(ethylene glycol) (PLA-PEG-PPG-PEG) tetra-block copolymer; and

b) an isolated nucleic acid encoding a protein comprising an amino acid sequence at least 95% identical to the amino acid sequence of SEQ ID NO: 9.

2. The composition of claim 1 , wherein the PLA-PEG-PPG-PEG tetra-block copolymer is formed from chemical conjugation of PEG-PPG-PEG tri-block copolymer with PLA.

3. The composition of claim 1 , wherein the molecular weight of PLA is between about 10,000 and about 100,000 daltons.

4. The composition of claim 1 , further comprising a peptide comprising an amino acid sequence selected from the group consisting of SEQ ID NOs: 1, 2, 3, 4, 5, 6, 7, 8, and polyarginine, wherein the peptide and the isolated nucleic acid form a complex.

5. The composition of claim 1 , further comprising a cationic cell-penetrating peptide.

6. The composition of claim 1 , further comprising an agent selected from the group consisting of doxorubicin, daunorubicin, decitabine, irinotecan, SN-38, cytarabine, docetaxel, triptolide, geldanamycin, 17-AAG, 5-FU, oxaliplatin, carboplatin, methotrexate, paclitaxel, indenoisoquinolines, and bortezomib.

7. The composition of claim 1 , wherein the polymeric nanoparticles further comprise a targeting moiety attached to the outside of the polymeric nanoparticles, and wherein the targeting moiety is an antibody, peptide, or aptamer.

8. The composition of claim 1 , wherein the polymeric nanoparticle comprises a tetra-block copolymer selected from the group consisting of PLA 12kDa -PEG-PPG-PEG-DNA, PLA 12kDa -PEG-PPG-PEG-Pt-DNA, PLA 72kDa -PEG-PPG-PEG-DNA and PLA 72kDa -PEG-PPG-PEG-Pt-DNA.

9. The composition of claim 1 , wherein the isolated nucleic acid comprises a nucleotide sequence at least 95% identical to nucleotides 404-874 of SEQ ID NO:11.

10. The composition of claim 1 , wherein the isolated nucleic acid comprises nucleotides 404-874 of SEQ ID NO:11.

11. The composition of claim 1 , wherein the isolated nucleic acid comprises a nucleotide sequence at least 95% identical to nucleotides 176-874 of SEQ ID NO:11.

12. The composition of claim 1 , wherein the isolated nucleic acid comprises nucleotides 176-874 of SEQ ID NO:11.

13. The composition of claim 1 , wherein the isolated nucleic acid comprises a nucleotide sequence at least 95% identical to the nucleotide sequence of SEQ ID NO:11.

14. The composition of claim 1 , wherein the isolated nucleic acid comprises the nucleotide sequence of SEQ ID NO:11.

15. The composition of claim 1 , wherein the isolated nucleic acid encodes the amino acid sequence of SEQ ID NO:9.

16. The composition of claim 1 , wherein the isolated nucleic acid encodes an amino acid sequence at least 95% identical to the amino acid sequence of SEQ ID NO:10.

17. The composition of claim 1 , wherein the isolated nucleic acid encodes the amino acid sequence of SEQ ID NO:10.

18. A pharmaceutical composition comprising

a) polymeric nanoparticles comprising PLA-PEG-PPG-PEG tetra-block copolymer; and

b) an isolated nucleic acid encoding a protein comprising an amino acid sequence at least 95% identical to the amino acid sequence of SEQ ID NO: 9.

19. The pharmaceutical composition of claim 18 , wherein the PLA-PEG-PPG-PEG tetra-block copolymer is formed from chemical conjugation of PEG-PPG-PEG tri-block copolymer with PLA.

20. The pharmaceutical composition of claim 18 , wherein the molecular weight of PLA is between about 10,000 and about 100,000 daltons.

21. The pharmaceutical composition of claim 18 , further comprising a peptide comprising an amino acid sequence selected from the group consisting of SEQ ID NOs: 1, 2, 3, 4, 5, 6, 7, 8, and polyarginine, wherein the peptide and the isolated nucleic acid form a complex.

22. The pharmaceutical composition of claim 18 , further comprising a cationic cell-penetrating peptide.

23. The pharmaceutical composition of claim 18 , further comprising an agent selected from the group consisting of doxorubicin, daunorubicin, decitabine, irinotecan, SN-38, cytarabine, docetaxel, triptolide, geldanamycin, 17-AAG, 5-FU, oxaliplatin, carboplatin, methotrexate, paclitaxel, indenoisoquinolines, and bortezomib.

24. The pharmaceutical composition of claim 18 , wherein the polymeric nanoparticles further comprise a targeting moiety attached to the outside of the polymeric nanoparticles, and wherein the targeting moiety is an antibody, peptide, or aptamer.

25. The pharmaceutical composition of claim 18 , wherein the isolated nucleic acid comprises a nucleotide sequence at least 95% identical to nucleotides 404-874 of SEQ ID NO:11.

26. The pharmaceutical composition of claim 18 , wherein the isolated nucleic acid comprises nucleotides 404-874 of SEQ ID NO:11.

27. The pharmaceutical composition of claim 18 , wherein the isolated nucleic acid comprises a nucleotide sequence at least 95% identical to nucleotides 176-874 of SEQ ID NO:11.

28. The pharmaceutical composition of claim 18 , wherein the isolated nucleic acid comprises nucleotides 176-874 of SEQ ID NO:11.

29. The pharmaceutical composition of claim 18 , wherein the isolated nucleic acid comprises a nucleotide sequence at least 95% identical to the nucleotide sequence of SEQ ID NO:11.

30. The pharmaceutical composition of claim 18 , wherein the isolated nucleic acid comprises the nucleotide sequence of SEQ ID NO:11.

31. The pharmaceutical composition of claim 18 , wherein the isolated nucleic acid encodes the amino acid sequence of SEQ ID NO:9.

32. The pharmaceutical composition of claim 18 , wherein the isolated nucleic acid encodes an amino acid sequence at least 95% identical to the amino acid sequence of SEQ ID NO:10.

33. The pharmaceutical composition of claim 18 , wherein the isolated nucleic acid encodes the amino acid sequence of SEQ ID NO:10.

34. The pharmaceutical composition of claim 18 , wherein the polymeric nanoparticle comprises a tetra-block copolymer selected from the group consisting of PLA 12kDa -PEG-PPG-PEG-DNA, PLA 12kDa -PEG-PPG-PEG-Pt-DNA, PLA 72kDa -PEG-PPG-PEG-DNA and PLA 72kDa -PEG-PPG-PEG-Pt-DNA.

Assignments (4)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 2, 2026
From: THARIMMUNE, INC.
To: GRAVITAS LIFE SCIENCES, INC.
Reel/Frame 073355/0059 →
CHANGE OF NAME Recorded Feb 3, 2025
From: HILLSTREAM BIOPHARMA, INC.
To: THARIMMUNE, INC.
Reel/Frame 070096/0468 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 11, 2022
From: NANOPROTEAGEN
To: HILLSTREAM BIOPHARMA, INC.
Reel/Frame 061734/0362 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 6, 2019
From: KHARBANDA, SURENDER; SHUKLA, VASUNDHARA; KUFE, DONALD; SINGH, HARPAL
To: NANOPROTEAGEN
Reel/Frame 051205/0522 →
Continuity (2)
Provisional Application 62416574 · Nov 2, 2016
Related Publication 20190321305A1 · Oct 24, 2019