IP Library Granted Patent US 11,186,756
Granted Patent B2
US 11,186,756 · App. 16/485,885 · Granted Nov 30, 2021

Epoxy-acrylic hybrid adhesive

Inventors: Gary L. Jialanella (Auburn Hills, MI); Eric E. Cole (Auburn Hills, MI)
Assignee: DDP SPECIALTY ELECTRONIC MATERIALS US, LLC
C09J175/16C09J4/06C09J5/00C09J2451/00C09J2463/00C09J2475/00
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Quick Facts
Patent No.
US 11,186,756
App. No.
16/485,885
Granted
Nov 30, 2021
Kind
B2
Abstract

The invention relates to a two-component adhesive based on hybrid urethane-acrylate epoxies comprising a core/shell rubber demonstrating good T-peel strength. The adhesives are suitable for use in industry, e.g., as adhesives for transportation industry applications.

Claims (17)

1. A two-component adhesive composition comprising an A-side and a B-side:

A) the A-side comprising:

i) a) an acrylate-capped polyurethane having a Tg equal to or greater than 20° C.,

i) b) an acrylate-capped polyurethane having a Tg equal to or less than −20° C.,

ii) a core/shell graft copolymer,

iii) a phosphorous compound with mono-esters of phosphonic or mono- and diesters of phosphonic and phosphoric acids having one unit of vinyl or allylic unsaturation present,

iv) an olefinically-unsaturated carboxylic acid,

v) an olefinically-unsaturated carboxylic acid ester, and

vi) a reducing agent and

B) the B-side comprising:

i) an epoxy resin

ii) a oxidizing agent,

iii) a stabilizer, and

iv) a filler.

2. The adhesive composition of claim 1 further comprising vii) a rheology modifier in the A-side, in the B-side, or in both the A-side and B-side.

3. The adhesive composition of claim 1 wherein the acrylate-capped polyurethane A) i) is obtained by reacting a polyol with a multifunctional isocyanate to complete reaction of the isocyanate to obtain a pre-polymer, and capping the pre-polymer with acrylate groups.

4. The adhesive composition of claim 1 wherein the epoxy resin B) i) comprises a liquid epoxy resin.

Assignments (5)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 14, 2021
From: JIALANELLA, GARY L.; COLE, ERIC E.
To: DOW GLOBAL TECHNOLOGIES LLC
Reel/Frame 056297/0664 →
CHANGE OF NAME Recorded Mar 30, 2021
From: DDP SPECIALTY ELECTRONIC MATERIALS US, INC.
To: DDP SPECIALTY ELECTRONIC MATERIALS US, LLC
Reel/Frame 055763/0302 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 24, 2021
From: JIALANELLA, GARY L.; COLE, ERIC E.
To: DOW GLOBAL TECHNOLOGIES LLC
Reel/Frame 056328/0618 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 24, 2021
From: DOW GLOBAL TECHNOLOGIES LLC
To: THE DOW CHEMICAL COMPANY
Reel/Frame 055398/0151 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 24, 2021
From: THE DOW CHEMICAL COMPANY
To: DDP SPECIALTY ELECTRONIC MATERIALS US, INC.
Reel/Frame 055399/0001 →
Continuity (2)
Provisional Application 62472905 · Mar 17, 2017
Related Publication 20200002587A1 · Jan 2, 2020