IP Library Granted Patent US 11,034,860
Granted Patent B2
US 11,034,860 · App. 16/493,409 · Granted Jun 15, 2021

Polishing agent, stock solution for polishing agent, and polishing method

Inventors: Masayuki Hanano (Tokyo, JP); Kouji Mishima (Tokyo, JP); Naomi Watanabe (Tokyo, JP)
Assignee: SHOWA DENKO MATERIALS CO., LTD.
C09G1/02C09K3/1409H01L21/31053
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Quick Facts
Patent No.
US 11,034,860
App. No.
16/493,409
Granted
Jun 15, 2021
Kind
B2
Abstract

A polishing agent containing abrasive grains and water, in which the abrasive grains contain silica particles, an average particle diameter R ave of the abrasive grains is 50 nm or more, a ratio R ave /R min of the average particle diameter R ave to an average minor diameter R min of the abrasive grains is 1.0 to 2.0, and a zeta potential of the abrasive grains in the polishing agent is positive.

Claims (35)

1. A polishing agent comprising:

abrasive grains, and

water,

wherein the abrasive grains contain silica particles,

an average secondary particle diameter R ave of the abrasive grains is 50 nm or more,

a ratio R ave /R min of the average secondary particle diameter R ave to an average minor diameter R min of the abrasive grains is 1.0 to 1.3, and

a zeta potential of the abrasive grains in the polishing agent is positive.

2. The polishing agent according to claim 1 , wherein the silica particles contain colloidal silica.

3. The polishing agent according to claim 1 , wherein the average secondary particle diameter R ave is 50 to 100 nm.

4. The polishing agent according to claim 1 , wherein the average secondary particle diameter R ave exceeds 60 nm.

5. The polishing agent according to claim 1 , wherein the ratio R ave /R min is 1.1 to 1.3.

6. The polishing agent according to claim 1 , further comprising a pH adjusting agent.

7. The polishing agent according to claim 1 , wherein a pH is 2.0 to 4.0.

8. A stock solution for a polishing agent for obtaining the polishing agent according to claim 1 ,

wherein the stock solution is diluted with water to obtain the polishing agent.

9. The polishing agent according to claim 1 , wherein the average secondary particle diameter R ave is more than 70 nm.

10. The polishing agent according to claim 1 , wherein the average secondary particle diameter R ave is 80 nm or more.

11. The polishing agent according to claim 1 , wherein the zeta potential of the abrasive grains is 20 mV or less.

12. The polishing agent according to claim 1 , wherein the average secondary particle diameter R ave and the ratio R ave /R min are values of all silica particles contained in the polishing agent.

13. A polishing method comprising a step of polishing and removing at least a part of a silicon oxide film by using the polishing agent according to claim 1 .

14. The polishing method according to claim 13 , wherein the silicon oxide film comprises at least one selected from the group consisting of a TEOS film and a SiH 4 film.

15. The polishing method according to claim 13 , wherein the silicon oxide film comprises a TEOS film.

16. The polishing method according to claim 13 , wherein the silicon oxide film comprises a SiH 4 film.

17. A polishing method comprising a step of polishing and removing at least a part of a silicon oxide film by using the polishing agent obtained by diluting the stock solution for a polishing agent according to claim 8 with water.

18. The polishing method according to claim 17 , wherein the silicon oxide film comprises at least one selected from the group consisting of a TEOS film and a SiH 4 film.

19. The polishing method according to claim 17 , wherein the silicon oxide film comprises a TEOS film.

20. The polishing method according to claim 17 , wherein the silicon oxide film comprises a SiH 4 film.

21. A polishing agent comprising:

abrasive grains, and

water,

wherein the abrasive grains contain silica particles,

an average secondary particle diameter R ave of the abrasive grains is 50 nm or more,

a ratio R ave /R min of the average secondary particle diameter R ave to an average minor diameter R min of the abrasive grains is 1.71 to 2.0, and

a zeta potential of the abrasive grains in the polishing agent is positive.

22. The polishing agent according to claim 21 , wherein the average secondary particle diameter R ave and the ratio R ave /R min are values of all silica particles contained in the polishing agent.

Assignments (5)
CHANGE OF ADDRESS Recorded Feb 14, 2024
From: RESONAC CORPORATION
To: RESONAC CORPORATION
Reel/Frame 066599/0037 →
CHANGE OF NAME Recorded Mar 8, 2023
From: SHOWA DENKO MATERIALS CO., LTD.
To: RESONAC CORPORATION
Reel/Frame 062992/0805 →
CHANGE OF NAME Recorded Feb 26, 2021
From: HITACHI CHEMICAL COMPANY, LTD.
To: SHOWA DENKO MATERIALS CO., LTD.
Reel/Frame 055429/0564 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 24, 2020
From: HANANO, MASAYUKI; MISHIMA, KOUJI; WATANABE, NAOMI
To: HITACHI CHEMICAL COMPANY, LTD.
Reel/Frame 051905/0754 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 18, 2019
From: HANANO, MASAYUKI; MISHIMA, KOUJI; WATANABE, NAOMI
To: HITACHI CHEMICAL COMPANY, LTD.
Reel/Frame 051316/0869 →