IP Library › Granted Patent US 11,309,190
Granted Patent B2
US 11,309,190 · App. 16/746,239 · Granted Apr 19, 2022

Semiconductor device and method of manufacture

Inventors: Jian-Jou Lian (Tainan, TW); Chun-Neng Lin (Hsinchu County, TW); Chieh-Wei Chen (Taoyuan, TW); Tzu-Ang Chiang (I-lan, TW); Ming-Hsi Yeh (Hsinchu, TW)
Assignee: Taiwan Semiconductor Manufacturing Company, Ltd.
H01L21/32134C09K13/00H01L21/28079H01L21/28088H01L21/28097H01L21/823437H01L29/517H01L29/66795H01L21/0276H01L21/32139H01L21/76224H01L21/823431H01L21/823481H01L29/6656H01L29/66545
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Quick Facts
Patent No.
US 11,309,190
App. No.
16/746,239
Granted
Apr 19, 2022
Kind
B2
Abstract

In a wet etching process to pattern a metal layer such as a p-metal work function layer over a dielectric layer such as a high-k gate dielectric layer, a selectivity of the wet etching solution between the metal layer and the dielectric layer is increased utilizing an inhibitor. The inhibitor includes such inhibitors as a phosphoric acid, a carboxylic acid, an amino acid, or a hydroxyl group.

Claims (35)

1. A method of manufacturing a semiconductor device, the method comprising:

forming a p-metal work function layer over a dielectric layer; and

applying a wet etching solution to the p-metal work function layer to remove a portion of the p-metal work function layer, wherein applying the wet etching solution forms a protective layer on an exposed surface of the dielectric layer after the portion of the p-metal work function layer has been removed, the wet etching solution comprising:

a metal etchant;

an inhibitor for the dielectric layer; and

a solvent.

2. The method of claim 1 , wherein the dielectric layer is hafnium oxide.

3. The method of claim 1 , wherein the inhibitor is a phosphoric acid.

4. The method of claim 1 , wherein the inhibitor is a carboxylic acid.

5. The method of claim 1 , wherein the inhibitor is an amino acid.

6. The method of claim 1 , wherein the inhibitor comprises a hydroxyl group.

7. The method of claim 1 , further comprising removing the protective layer.

8. A method of manufacturing a semiconductor device, the method comprising:

depositing a first p-work function layer onto a high-k dielectric layer; and

etching the first p-work function layer with a wet etching solution to expose a first portion of the high-k dielectric layer, wherein the wet etching solution comprises an inhibitor for the high-k dielectric layer, wherein the high-k dielectric layer reacts with the wet etching solution to form a protective layer on the high-k dielectric layer.

9. The method of claim 8 , wherein the protective layer comprises phosphorous, nitrogen, or carbon.

10. The method of claim 8 , wherein the wet etching solution further comprises:

a solvent;

a first metal etchant; and

an oxidizer.

11. The method of claim 8 , wherein the inhibitor comprises one or more of a phosphoric acid, a carboxylic acid, or an amino acid.

12. The method of claim 8 , wherein the protective layer forms a hydrophobic surface.

13. The method of claim 8 , wherein the high-k dielectric layer comprises hafnium oxide and the first p-work function layer comprises titanium nitride.

14. The method of claim 13 , wherein a selectivity of the wet etching solution between the titanium nitride and the high-k dielectric layer is at least 100:1.

15. A method of manufacturing a semiconductor device, the method comprising:

dispensing an etching solution over a p-metal work function material, the p-metal work function material being on a dielectric layer, wherein dispensing the etching solution etches the p-metal work function material to expose a portion of the dielectric layer, the etching solution forming a protective layer on the portion of the dielectric layer, the etching solution comprising:

a solvent;

a first metal etchant;

an oxidizer; and

an inhibitor comprising one or more of a phosphoric acid, a carboxylic acid, or an amino acid, the inhibitor being for the dielectric layer.

16. The method of claim 15 , wherein the inhibitor comprises di-(2-ethylhexyl)phosphoric acid.

17. The method of claim 15 , wherein the inhibitor comprises the carboxylic acid.

18. The method of claim 15 , wherein the inhibitor comprises glycine.

19. The method of claim 15 , wherein the inhibitor has a concentration of less than about 5%-volume.

20. The method of claim 15 , wherein the etching solution has a selectivity between titanium nitride and hafnium oxide of at least 100.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 18, 2020
From: LIAN, JIAN-JOU; LIN, CHUN-NENG; CHEN, CHIEH-WEI; CHIANG, TZU-ANG; YEH, MING-HSI
To: TAIWAN SEMICONDUCTOR MANUFACTURING COMPANY, LTD.
Reel/Frame 051846/0820 →
Continuity (1)
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