IP Library › Granted Patent US 11,566,114
Granted Patent B2
US 11,566,114 · App. 16/759,252 · Granted Jan 31, 2023

Fiber-reinforced thermoplastic resin filament and shaped product of same

Inventors: Masayuki Koshi (Nagoya, JP); Yoshihiro Naruse (Nagoya, JP); Shoma Ishida (Nagoya, JP)
Assignee: Toray Industries, Inc.
C08J5/042D06M15/63D06M15/647C08J2371/00C08J2381/04D06M2101/30
View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 11,566,114
App. No.
16/759,252
Granted
Jan 31, 2023
Kind
B2
Abstract

A fiber-reinforced thermoplastic resin filament is obtained by impregnating a continuous reinforcing fiber with a thermoplastic resin, and satisfies all of conditions (a) to (c). (a) The volume ratio of a reinforcing fiber in a fiber-reinforced thermoplastic resin filament is 30 to 80%; and the volume ratio of a thermoplastic resin in a fiber-reinforced thermoplastic resin filament is 70 to 20%. (b) The thickness of a fiber-reinforced thermoplastic resin filament is 0.01 to 3 mm. (c) The length of a filament contained in a fiber-reinforced thermoplastic resin filament is 1 m or more.

Claims (21)

1. A fiber-reinforced thermoplastic resin 3D printing filament of continuous reinforcing fiber impregnated with a thermoplastic resin, having

(a) a volume content of the reinforcing fiber of 30 to 80 vol % and a volume content of the thermoplastic resin filament of 70 to 20 vol %,

(b) a thickness of 0.01 to 3 mm,

(c) a filament length of 1 m or more, and

(d) a circular filament cross section.

2. The fiber-reinforced thermoplastic resin 3D printing filament according to claim 1 , having a void rate of 5% or less.

3. The fiber-reinforced thermoplastic resin 3D printing filament according to claim 1 , having a flexural rigidity of 1 N·m 2 or less.

4. The fiber-reinforced thermoplastic resin 3D printing filament according to claim 1 , wherein the reinforcing fiber is made of at least one selected from a group consisting of a carbon fiber, a glass fiber and an aramid fiber.

5. The fiber-reinforced thermoplastic resin 3D printing filament according to claim 1 , wherein the thermoplastic resin is made of at least one selected from a group consisting of polyphenylene sulfide resin (PPS), polyarylene ether ketone resin (PAEK), polyetherimide resin (PEI), polyether sulfone resin (PES) and a liquid crystalline polymer resin (LCP).

6. The fiber-reinforced thermoplastic resin 3D printing filament according to claim 1 , wherein the reinforcing fiber has 90% or more of an average value D of a dispersion parameter d calculated by steps (i) to (iv):

(i) taking an image of a cross section of the fiber-reinforced thermoplastic resin filament perpendicular to an orientation direction;

(ii) dividing the image of the cross section into square units having a side length t within a range of Formula (1);

(iii) calculating the dispersion parameter d by Formula (2);

(iv) calculating the average value D of the dispersion parameter d by repeating a plurality of sets of steps (i) to (iii),

1.5 a≤t≤ 2.5 a   (1), where:

a: fiber diameter; and

t: side length of unit,

Dispersion parameter d =100×(the number of units including reinforcing fibers within range)/(the number of all units)  (2).

7. The fiber-reinforced thermoplastic resin 3D printing filament according to claim 1 , wherein the average value D of the dispersion parameter d has 4% or more of a coefficient of variance.

8. The fiber-reinforced thermoplastic resin 3D printing filament according to claim 1 , further comprising an outer most layer coated with the thermoplastic resin.

9. A shaped product, comprising the fiber-reinforced thermoplastic resin 3D printing filament according to claim 1 .

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Apr 24, 2020
From: KOSHI, MASAYUKI; NARUSE, YOSHIHIRO; ISHIDA, SHOMA
To: TORAY INDUSTRIES, INC.
Reel/Frame 052493/0375 →
Priority Claims (1)
JP JP2017-214604 · Nov 7, 2017 · national
Continuity (1)
Related Publication 20200369838A1 · Nov 26, 2020