IP Library Granted Patent US 11,213,369
Granted Patent B2
US 11,213,369 · App. 16/835,101 · Granted Jan 4, 2022

Multilayer polymer sheets

Inventors: Chunhua Li (Cupertino, CA); Yan Chen (Cupertino, CA); Heinz Pudleiner (Krefeld, DE); Klaus Meyer (Dormagen, DE); Joerg Nickel (Dormagen, DE); Craig Pehlert (Lenox, MA)
Assignee: Align Technology, Inc.
A61C7/08B29C51/14B32B7/02B32B25/08B32B25/20B32B27/08B32B27/281B32B27/285B32B27/286B32B27/308B32B27/32B32B27/34B32B27/36B32B27/365B32B27/40A61C7/00A61C13/00A61C19/06A61F5/56A63B71/085B29K2067/00B29K2075/00B29K2995/007B29K2995/0026B29K2995/0077B29K2995/0082B29L2031/753B32B25/14B32B27/283B32B27/30B32B27/302B32B2250/03B32B2250/24B32B2250/40B32B2274/00B32B2307/40B32B2307/412B32B2307/50B32B2307/51B32B2307/536B32B2307/54B32B2307/546B32B2319/00B32B2323/00B32B2323/04B32B2323/10B32B2323/16B32B2333/04B32B2367/00B32B2371/00B32B2375/00B32B2377/00B32B2383/00B32B2535/00B32B2555/00Y10T428/31551Y10T428/31565Y10T428/31786
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Quick Facts
Patent No.
US 11,213,369
App. No.
16/835,101
Granted
Jan 4, 2022
Kind
B2
Abstract

Multilayer polymer sheets are provided, as well as related methods, systems, and appliances.

Claims (19)

1. A multilayer sheet comprising:

a first outer polymer layer comprising co-polyester and a second outer polymer layer comprising co-polyester, each of the first and second outer polymer layers having a hardness of about 60 A to about 85 D, wherein each of the first outer polymer layer and the second polymer layer comprises a compression set greater than 40% after 24 hours at 70° C.; and

an inner polymer layer comprising thermoplastic polyurethane, wherein the multilayer sheet is incorporated into an orthodontic appliance.

2. The multilayer sheet of claim 1 , wherein at least one of the first outer polymer layer and the second outer polymer layer comprises one or more of: a flexural modulus of greater than about 35,000 psi, or a light transmission between 400 nm and 800 nm of greater than about 75%.

3. The multilayer sheet of claim 1 , wherein at least one of the first outer polymer layer and the second outer polymer layer comprises a blend of polymeric materials, including the co-polyester and one or more materials selected from the group consisting of: a thermoplastic polyurethane elastomer, a silicone rubber, an elastomeric alloy, a thermoplastic elastomer, a thermoplastic vulcanizate elastomer, a block copolymer elastomer, a polyolefin blend elastomer, a thermoplastic co-polyester elastomer, and a thermoplastic polyamide elastomer.

4. The multilayer sheet of claim 1 , wherein the inner polymer layer comprises a blend of polymeric materials, including the thermoplastic polyurethane and one or more materials selected from the group consisting of: a polyester, a co-polyester, a polypropylene, a polyethylene, a polypropylene and polyethylene copolymer, an acrylic, a polyetheretherketone, a polyamide, a polyethylene terephthalate, a polybutylene terephthalate, a polyetherimide, a cyclic block copolymer, a polyethersulfone, and a polytrimethylene terephthalate.

5. The multilayer sheet of claim 1 , wherein the inner polymer layer comprises at least two layers, and wherein one layer is the thermoplastic polyurethane and at least one layer of the inner polymer layer independently comprises a polymeric material selected from the group consisting of: a polyester, a co-polyester, a polypropylene, a polyethylene, a polypropylene and polyethylene copolymer, an acrylic, a polyetheretherketone, a polyamide, a polyethylene terephthalate, a polybutylene terephthalate, a polyetherimide, a cyclic block copolymer, a polyethersulfone, and a polytrimethylene terephthalate, and a combination thereof.

6. The multilayer sheet of claim 1 comprising a thickness of between 500 μm and 1200 μm.

7. The multilayer sheet of claim 1 , wherein the inner polymer layer comprises at least one of: an elongation at yield of greater than about 4%, an elongation at break of greater than about 70%, a stress relaxation of greater than about 10% at 24 hours testing at a relative humidity of between 90% and 100%, a light transmission between 400 nm and 800 nm of greater than about 75%, or a tensile strength at yield between 4000 psi and 6500 psi.

8. A multilayer sheet comprising:

a first outer polymer layer comprising co-polyester and a second outer polymer layer comprising co-polyester, each of the first and second outer polymer layers having a flexural modulus of greater than about 35,000 psi and a compression set of greater than 40% after 24 hours at 70° C.; and

an inner polymer layer comprising thermoplastic polyurethane, the inner polymer layer having an elongation at break of greater than about 70%, wherein the multilayer sheet is incorporated into an orthodontic appliance.

9. The multilayer sheet of claim 8 , wherein each of the first and second outer polymer layers each have a hardness of about 60 A to about 85 D.

10. The multilayer sheet of claim 8 , wherein at least one of the first outer polymer layer and the second outer polymer layer comprises a light transmission between 400 nm and 800 nm of greater than about 75%.

11. The multilayer sheet of claim 8 , wherein at least one of the first outer polymer layer and the second outer polymer layer comprises a blend of polymeric materials, including the co-polyester and one or more materials selected from the group consisting of: a thermoplastic polyurethane elastomer, a silicone rubber, an elastomeric alloy, a thermoplastic elastomer, a thermoplastic vulcanizate elastomer, a block copolymer elastomer, a polyolefin blend elastomer, a thermoplastic co-polyester elastomer, and a thermoplastic polyamide elastomer.

12. The multilayer sheet of claim 8 , wherein the inner polymer layer comprises a blend of polymeric materials, including the thermoplastic polyurethane and one or more materials selected from the group consisting of: a polyester, a co-polyester, a polypropylene, a polyethylene, a polypropylene and polyethylene copolymer, an acrylic, a polyetheretherketone, a polyamide, a polyethylene terephthalate, a polybutylene terephthalate, a polyetherimide, a cyclic block copolymer, a polyethersulfone, and a polytrimethylene terephthalate.

13. The multilayer sheet of claim 8 , wherein the inner polymer layer comprises at least two layers, and wherein one layer is the thermoplastic polyurethane and at least one layer of the inner polymer layer independently comprises a polymeric material selected from the group consisting of: a polyester, a co-polyester, a polypropylene, a polyethylene, a polypropylene and polyethylene copolymer, an acrylic, a polyetheretherketone, a polyamide, a polyethylene terephthalate, a polybutylene terephthalate, a polyetherimide, a cyclic block copolymer, a polyethersulfone, and a polytrimethylene terephthalate, and any combination thereof.

14. The multilayer sheet of claim 8 comprising a thickness of between 500 μm and 1200 μm.

15. The multilayer sheet of claim 8 , wherein the inner polymer layer comprises at least one of: an elongation at yield of greater than about 4%, a stress relaxation of greater than about 10% at 24 hours testing at a relative humidity of between 90% and 100%, a light transmission between 400 nm and 800 nm of greater than about 75%, or a tensile strength at yield between 4000 psi and 6500 psi.

Assignments (5)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 9, 2021
From: COVESTRO DEUTSCHLAND AKTIENGESELLSCHAFT; COVESTRO LLC
To: ALIGN TECHNOLOGY, INC.
Reel/Frame 057432/0424 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 26, 2021
From: LI, CHUNHUA; CHEN, YAN
To: ALIGN TECHNOLOGY, INC.
Reel/Frame 055739/0591 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 26, 2021
From: PUDLEINER, HEINZ, DR.; MEYER, KLAUS; NICKEL, JOERG
To: COVESTRO DEUTSCHEAND AKTIENGESELESCHAFT
Reel/Frame 055739/0812 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 26, 2021
From: PEHLERT, CRAIG
To: COVESTRO LLC
Reel/Frame 055739/0938 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 26, 2021
From: COVESTRO DEUTSCHLAND AKTIENGESELLSCHAFT; COVESTRO LLC
To: ALIGN TECHNOLOGY, INC.
Reel/Frame 057181/0393 →
Continuity (3)
Continuation 15476655 · Mar 31, 2017
Division 13470681 · May 14, 2012
Related Publication 20200346449A1 · Nov 5, 2020