IP Library Granted Patent US 11,535,757
Granted Patent B2
US 11,535,757 · App. 16/903,385 · Granted Dec 27, 2022

Organic substance-attached porous inorganic oxide particle

Inventors: Yoshifumi Eri (Kanagawa, JP); Takahiro Mizuguchi (Kanagawa, JP); Sakae Takeuchi (Kanagawa, JP); Yuka Zenitani (Kanagawa, JP); Koji Sasaki (Kanagawa, JP)
Assignee: FUJIFILM Business Innovation Corp.
C09C1/3081C01P2004/64C01P2006/22
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Quick Facts
Patent No.
US 11,535,757
App. No.
16/903,385
Granted
Dec 27, 2022
Kind
B2
Abstract

An organic substance-attached porous inorganic oxide particle including porous inorganic oxide particle and an organic substance attached to the surface of the porous inorganic oxide particle. The organic substance-attached porous inorganic oxide particle satisfies a formula below ( Cf−Ce )/2>1 where Cf represents the amount of carbon (atom %) measured by subjecting the surface of the particle to X-ray photoelectron spectroscopy (XPS) after the particle is washed, and Ce represents the amount of carbon (atom %) measured by subjecting the surface of the particle to X-ray photoelectron spectroscopy (XPS) after two-minute surface etching of the particle.

Claims (17)

1. An organic substance-attached porous inorganic oxide particle comprising:

a porous inorganic oxide particle; and

an organic substance attached to a surface of the porous inorganic oxide particle,

wherein the organic substance-attached porous inorganic oxide particle satisfies a formula below

( Cf−Ce )/2>1

where Cf represents the amount of carbon (atom %) measured by subjecting the surface of the particle to X-ray photoelectron spectroscopy (XPS) after the organic substance-attached porous inorganic oxide particle is washed, and Ce represents the amount of carbon (atom %) measured by subjecting the surface of the washed organic substance-attached porous inorganic oxide particle to X-ray photoelectron spectroscopy (XPS) after two-minute surface etching of the particle,

wherein the organic substance-attached porous inorganic oxide particle is washed by mixing the organic substance-attached porous inorganic oxide particle with tetrahydrofuran (THF) to form a mixture, subjecting the mixture to a dispersion treatment, and centrifuging the mixture, followed by removing a supernatant to obtain the washed organic substance-attached porous inorganic oxide particle, and

the washed organic substance-attached porous inorganic oxide particle is surface etched for two minutes by an argon monomer etching method using argon as an etching gas.

2. The organic substance-attached porous inorganic oxide particle according to claim 1 , wherein the organic substance-attached porous inorganic oxide particle satisfies a formula below:

( Cf−Ce )/2≥1.5.

3. The organic substance-attached porous inorganic oxide particle according to claim 1 , wherein the porous inorganic oxide particles have a number average particle diameter within a range of 7 nm to 150 nm.

4. The organic substance-attached porous inorganic oxide particle according to claim 1 , wherein the porous inorganic oxide particles have a number average particle diameter within a range of 7 nm to 60 nm.

5. The organic substance-attached porous inorganic oxide particle according to claim 1 , wherein the porous inorganic oxide particle is a gas-phase method silica particle.

6. The organic substance-attached porous inorganic oxide particle according to claim 1 , wherein the organic substance is oil.

7. The organic substance-attached porous inorganic oxide particle according to claim 6 , wherein the oil is unreactive silicone oil.

8. The organic substance-attached porous inorganic oxide particle according to claim 1 , wherein an amount of the organic substance attached relative to the porous inorganic oxide particle after washing is 4 mass % or higher and 8 mass % or lower.

9. The organic substance-attached porous inorganic oxide particle according to claim 1 , wherein an amount of the organic substance attached relative to the porous inorganic oxide particle after washing is 3 mass % or higher and 6 mass % or lower.

Assignments (2)
CHANGE OF NAME Recorded May 19, 2021
From: FUJI XEROX CO., LTD.
To: FUJIFILM BUSINESS INNOVATION CORP.
Reel/Frame 056294/0219 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 23, 2020
From: ERI, YOSHIFUMI; MIZUGUCHI, TAKAHIRO; TAKEUCHI, SAKAE; ZENITANI, YUKA; SASAKI, KOJI
To: FUJI XEROX CO., LTD.
Reel/Frame 053006/0872 →
Priority Claims (1)
JP JP2019-216812 · Nov 29, 2019 · national
Continuity (1)
Related Publication 20210163754A1 · Jun 3, 2021