IP Library Granted Patent US 12,160,005
Granted Patent B2
US 12,160,005 · App. 17/396,031 · Granted Dec 3, 2024

Black metallic nanorod arrays and method of manufacturing thereof

Inventors: Da Deng (Troy, MI); Minjun Bae (Detroit, MI)
Assignee: Wayne State University
H01M4/628H01M4/661H01M4/667H01M4/70H01M10/052H01M2004/021H01M2004/025
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Quick Facts
Patent No.
US 12,160,005
App. No.
17/396,031
Granted
Dec 3, 2024
Kind
B2
Abstract

A device may include a metallic substrate and a plurality of nanorod arrays arranged on the substrate. The nanorod arrays may be made of porous metallic nanostructures and may appear black in color.

Claims (45)

1. A device comprising:

a metallic substrate;

a plurality of nanorod arrays arranged on the substrate;

wherein the plurality of nanorod arrays are made from a process including:

forming metal oxide nanorod arrays on a metallic substrate;

spreading Mg on the metal oxide nanorod arrays;

heating the metal oxide nanorod arrays with Mg, resulting in metallic nanorod arrays;

removing excess Mg and MgO from the metallic nanorod arrays; and

drying the metallic nanorod arrays.

2. The device of claim 1 , wherein at least one of the metallic substrate is foil and the metal is titanium.

3. The device of claim 1 , wherein the metal is selected from a group comprising copper, iron, lead, nickel, tin, vanadium, zinc, aluminum, silicon, and alloys thereof.

4. The device of claim 1 , wherein the device is a lithium-ion or lithium-metal battery, and the metallic substrate is a current collector.

5. A method for forming black metallic nanorod arrays, comprising:

forming metal oxide nanorod arrays on a metallic substrate;

spreading Mg on the metal oxide nanorod arrays;

heating the metal oxide nanorod arrays with Mg, resulting in metallic nanorod arrays;

removing excess Mg and MgO from the metallic nanorod arrays; and

drying the metallic nanorod arrays.

6. The method of claim 5 , wherein the metal oxide is TiO 2 .

7. The method of claim 5 , wherein the metallic substrate is a metal foil.

8. The method of claim 5 , wherein forming the metal oxide nanorod arrays includes:

hydrothermally treating a piece of the metal substrate;

treating the metal substrate with an acid; and

heating the metal substrate.

9. The method of claim 8 , wherein the acid is HCl.

10. The method of claim 8 , further comprising placing two pieces of the metal substrate with nanorod arrays in a crucible before spreading the Mg thereon.

11. The method of claim 10 , wherein heating the metal oxide nanorod arrays with Mg is done in a crucible under argon.

12. The method of claim 5 , wherein removing excess Mg and MgO is done by treating the metallic nanorod arrays with HCl.

13. The method of claim 5 , wherein drying the metallic nanorod arrays is done in a vacuum oven.

14. A method for forming black metallic nanorod arrays, comprising:

forming metal oxide nanorod arrays on a metallic substrate;

spreading Mg on the metal oxide nanorod arrays;

heating the metal oxide nanorod arrays with Mg after said spreading Mg on the metal oxide nanorod arrays, resulting in metallic nanorod arrays;

removing excess Mg and MgO from the metallic nanorod arrays; and

drying the metallic nanorod arrays;

wherein the nanorod arrays are porous and appear black in color.

15. The method of claim 14 , wherein the metal oxide is TiO 2 and the metallic substrate is a Ti foil.

16. The method of claim 14 , wherein forming the metal oxide nanorod arrays includes:

hydrothermally treating a piece of the metal substrate;

treating the metal substrate with an acid; and

heating the metal substrate.

17. The method of claim 14 , further comprising placing two pieces of the metal substrate with nanorod arrays in a crucible before spreading the Mg thereon.

18. The method of claim 17 , wherein heating the metal oxide nanorod arrays with Mg is done in a crucible under argon.

19. The method of claim 14 , wherein removing excess Mg and MgO is done by treating the metallic nanorod arrays with HCl.

20. The method of claim 5 , wherein the metallic nanorod arrays have a black color once dried.

Assignments (2)
CONFIRMATORY LICENSE Recorded Feb 10, 2025
From: WAYNE STATE UNIVERSITY
To: UNITED STATES DEPARTMENT OF ENERGY
Reel/Frame 070159/0771 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 6, 2021
From: DENG, DA; BAE, MINJUN
To: WAYNE STATE UNIVERSITY
Reel/Frame 057105/0758 →
Continuity (2)
Provisional Application 63062613 · Aug 7, 2020
Related Publication 20220045331A1 · Feb 10, 2022