IP Library › Granted Patent US 12,487,198
Granted Patent B2
US 12,487,198 · App. 17/923,057 · Granted Dec 2, 2025

Concentration detection device and concentration detection method

Inventors: Yasuo Wakabayashi (Wako, JP); Yoshie Otake (Wako, JP); Yujiro Ikeda (Wako, JP)
Assignee: RIKEN
G01N23/222G01N2223/0745G01N2223/106
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Quick Facts
Patent No.
US 12,487,198
App. No.
17/923,057
Granted
Dec 2, 2025
Kind
B2
Abstract

A concentration detector includes: a neutron source emitting neutrons to a target; a gamma ray detector detecting and determining an amount of specific gamma rays that are among gamma rays generated in the target by interactions with the neutrons; and a concentration calculator calculating a concentration of the target at selected depths in the inspection target, based on the detected amount. A relational expression expressing a relation between a plurality of concentrations of the target in a plurality of virtual layers and a detected amount of the specific gamma rays is predetermined for each type of the specific gamma rays or each detection condition. The concentration calculator applies the detected amount for each gamma ray type or each detection condition, to the relational expression for the type or the detection condition, and calculates a concentration of the target component in the layer at each depth or the specific depth.

Claims (40)

1 . A concentration detection device comprising:

a neutron source that emits neutrons to a surface of an inspection target so that specific gamma rays having different energies and derived from a target component in the inspection target are generated in the inspection target as a result of interactions between the target component and the neutrons;

a gamma ray detection device that includes a gamma ray detector detecting a specific gamma ray included in the specific gamma rays, and determines, for each of the different energies, a number of times the gamma ray detector detects the specific gamma ray; and

a concentration calculation device that includes a storage unit storing a plurality of relational expressions;

wherein a plurality of arrangement relations are each defined as one or both of a position relation and an orientation relation among the neutron source, the gamma ray detector, and the inspection target;

each of the plurality of relational expressions is set for corresponding one of the different energies or for corresponding one of a plurality of combinations, and each of the plurality of combinations is a combination of one of the different energies and one of the plurality of arrangement relations;

the inspection target is assumed to be virtually divided into a plurality of layers, and a plurality of concentrations are each defined as a concentration of the target component in corresponding one of the plurality of layers;

each of the plurality of relational expressions expresses, by unknown values of the plurality of concentrations and a plurality of predetermined coefficients, a variable of a number of times the gamma ray detector detects the specific gamma ray for the corresponding one of the different energies or the corresponding one of the plurality of combination; and

the concentration calculation device:

assigns, for each of the different energies or each of the plurality of combinations, the determined number of times to the variable in corresponding one of the plurality of relational expressions, and

calculates, as the concentration of the target component in one or each of the plurality of layers, one or each of the unknown values, from the plurality of relational expressions in each of which the determined number of times has been assigned to the variable.

2 . The concentration detection device according to claim 1 , wherein each of the plurality of relational expressions is expressed as

Σ X i ×α i,k =D k ,

where i denotes a number for each of the plurality of layers, k denotes a number for each of the different energies, each of i and k takes a value from 1 to n, and n is an integer equal to or larger than 2,

X i denotes the concentration of the target component in an i-th layer included in the plurality of layers,

α i,k is a predetermined coefficient included in the plurality of predetermined coefficients, and is set for the i-th layer and a k-th energy included in the different energies,

Σ denotes a total sum concerning all of the plurality of layers i, and

D k is the determined number of times for the k-th energy.

3 . The concentration detection device according to claim 1 , wherein each of the plurality of relational expressions is expressed as

Σ X i ×α i,k,j =D k,j ,

where i denotes a number for each of the plurality of layers, and k denotes a number for each of the different energies,

j denotes a number for each of the plurality of arrangement relations,

i takes a value from 1 to n, k takes a value from 1 to s, i takes a value from 1 to q, each of n, s, and q is an integer equal to or larger than 2, and n is equal to q×s,

Xi denotes the concentration of the target component in an i-th layer included in the plurality of layers,

α i,k,j is a predetermined coefficient included in the plurality of predetermined coefficients, and is set for the i-th layer, a k-th energy included in the different energies, and a j-th arrangement relation included in the plurality of arrangement relations,

Σ denotes a total sum concerning all of the plurality of layers i, and

D k,j denotes the determined number of times for the k-th energy and the j-th arrangement relation that constitute one of the plurality of combinations.

4 . The concentration detection device according to claim 1 , wherein the inspection target is a concrete structure including a reinforcing bar inside, and the target component is chlorine.

5 . A concentration detection method using the concentration detection device according to claim 1 , comprising:

a step (A) of emitting neutrons to a surface of an inspection target by the neutron source so that specific gamma rays having different energies and derived from a target component in the inspection target are generated in the inspection target as a result of interactions between the target component and the neutrons; and

a step (B) of, by the gamma ray detector, detecting a specific gamma ray included in the specific gamma rays, and by gamma ray detection device, determining, for each of the different energies, a number of times the gamma ray detector detects the specific gamma ray,

wherein the detecting at the step (B) is performed for each of the different energies or for each of the plurality of combinations so as to determine the number of times for each of the different energies or for each of the plurality of combinations,

the method comprises:

a step (C) of, by the concentration calculation device, assigning, for each of the different energies or each of the plurality of combinations, the determined number of times to the variable in corresponding one of the plurality of relational expressions, and calculating, as the concentration of the target component in one or each of the plurality of layers, one or each of the unknown values, from the plurality of relational expressions in each of which the determined number of times has been assigned to the variable.

6 . The concentration detection method according to claim 5 , wherein the inspection target is a concrete structure including a reinforcing bar inside, and the target component is chlorine.

7 . The concentration detection method according to claim 5 , wherein the inspection target is a concrete structure including a reinforcing bar inside,

the method comprises:

on assumption that the target component is a component of the reinforcing bar, performing the steps (A) to (C), thereby calculating a concentration of the component of the reinforcing bar in each of the plurality of layers;

a step (D) of determining, as a layer where the reinforcing bar exists, a layer that is included in the plurality of layers and for which the concentration of the component of the reinforcing bar is equal to or larger than a threshold value; and

on assumption that the target component is chlorine, performing the steps (A) to (C), thereby determining a concentration of chlorine in the layer determined at the step (D).

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 3, 2022
From: WAKABAYASHI, YASUO; OTAKE, YOSHIE; IKEDA, YUJIRO
To: RIKEN
Reel/Frame 061645/0639 →
Priority Claims (1)
JP 2020-084238 · May 13, 2020 · national
Continuity (1)
Related Publication 20230152250A1 · May 18, 2023
References Cited (20)
US 5081351A · Roscoe · 1992 [cited by examiner]
US 11841335B2 · Wakabayashi · 2023 [cited by examiner]
US 20030011387A1 · Trejo · 2003 [cited by examiner]
US 20120199754A1 · Nose · 2012 [cited by examiner]
US 20210033542A1 · Wakabayashi · 2021 [cited by examiner]
JP 61210932A · 1986 [cited by applicant]
JP 62282288A · 1987 [cited by applicant]
JP H08220029A · 1996 [cited by examiner]
JP 2001194324A · 2001 [cited by applicant]
JP 3323042B2 · 2002 [cited by examiner]
JP 5926362B1 · 2016 [cited by examiner]
WO 2011046078A1 · 2011 [cited by applicant]
WO 2019198260A1 · 2019 [cited by applicant]
Spyrou, N.M., “Elemental analysis of biological matrices using tomographic techniques,” Article, Journal of Radioanalytical and Nuclear Chemistry (1993). [cited by applicant]
Spyrou, N.M., “Prompt and delayed radiation measurements in the elemental analysis of biological materials: The case for neutron induced gamma-ray emission tomography,” Article, Journal of Radioanalytical and Nuclear Ch… [cited by applicant]
Extended European Search Report issued on Oct. 6, 2023 for European Patent Application No. 21803016.1. [cited by applicant]
Japanese Office Action issued on Oct. 6, 2023 for Japanese Patent Application No. 2020-084238. [cited by applicant]
International Preliminary Report on Patentability issued on Nov. 15, 2022 for PCT International Application No. PCT/JP2021/017704. [cited by applicant]
Japanese Office Action issued on Dec. 15, 2023 for Japanese Patent Application No. 2020-084238. [cited by applicant]
Communication pursuant to Article 94(3) EPC issued on Sep. 23, 2025 for European Patent Application No. 21803016.1. [cited by applicant]