IP Library Granted Patent US 9,663,382
Granted Patent B2
US 9,663,382 · App. 13/627,259 · Granted May 30, 2017

Method of synthesizing anatase TiO

Inventors: Jiehua Liu (Singapore, SG); Xue-Wei Liu (Singapore, SG); Xiangfeng Wei (Singapore, SG)
Assignee: NANYANG TECHNOLOGICAL UNIVERSITY
C01G23/053C07F7/006C07F15/0046H01G9/2031C01P2002/72C01P2004/03C01P2004/04C01P2004/24C01P2006/12C01P2006/14C01P2006/17Y02E10/542
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Quick Facts
Patent No.
US 9,663,382
App. No.
13/627,259
Granted
May 30, 2017
Kind
B2
Abstract

A method of synthesizing anatase TiO 2 nanosheets, the method comprising the steps of: (a) mixing a titanium complex with an ethanolamine derivative; (b) adding water to form a mixture; and (c) heating the mixture at a temperature ranging from about 150° C. to about 200° C. to obtain anatase TiO 2 nanosheets having O-terminated {100} facets.

Claims (16)

1. A method of synthesizing anatase TiO 2 nanosheets, the method comprising the steps of:

(a) mixing a titanium complex with an ethanolamine derivative;

(b) adding sufficient water to completely hydrolyze the titanium complex to form a mixture, the mixture comprising Ti(OH) 4 ; and

(c) heating the mixture at only one temperature ranging from about 150° C. to about 200° C. to obtain anatase TiO 2 nanosheets having O-terminated {100} facets.

2. The method of claim 1 , further comprising

(d) heating the anatase TiO 2 nanosheets having O-terminated {100} facets at a temperature ranging from about 400° C. to about 600° C. to obtain anatase TiO 2 nanosheets having activated {100} facets.

3. The method of claim 1 , further comprising, after step (c), washing with ethanol, centrifuging and drying the anatase TiO 2 nanosheets having O-terminated {100} facets at a temperature ranging from room temperature to about 200° C.

4. The method of claim 1 , wherein the titanium complex is a titanium (IV) complex.

5. A method of fabricating a dye-sensitized solar cell, the method comprising:

(a) mixing a titanium complex with an ethanolamine derivative;

(b) adding sufficient water to completely hydrolyze the titanium complex to form a mixture, the mixture comprising Ti(OH) 4 ;

(c) heating the mixture at only one temperature ranging from about 150° C. to about 200° C. to obtain anatase TiO 2 nanosheets having O-terminated {100} facets;

(d) heating the anatase TiO 2 nanosheets having O-terminated {100} facets at a temperature ranging from about 400° C. to about 600° C. to obtain anatase TiO 2 nanosheets having activated {100} facets; and

(e) soaking the anatase TiO 2 nanosheets having activated {100} facets in a N719 industry standard dye solution to obtain anatase TiO 2 nanosheets having O-(dye)-terminated {100} facets.

6. The method of claim 5 , further comprising, immediately after step (c) and before step (d), washing with ethanol, centrifuging and drying the anatase TiO 2 nanosheets having O-terminated {100} facets at a temperature ranging from room temperature to about 200° C.

7. The method of claim 5 , wherein the titanium complex is a titanium (IV) complex.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 13, 2015
From: LIU, JIEHUA; LIU, XUE-WEI; WEI, XIANGFENG
To: NANYANG TECHNOLOGICAL UNIVERSITY
Reel/Frame 035632/0171 →
Continuity (2)
Provisional Application 61539222 · Sep 26, 2011
Related Publication 20130079520A1 · Mar 28, 2013