IP Library Granted Patent US 12,534,664
Granted Patent B1
US 12,534,664 · App. 19/215,103 · Granted Jan 27, 2026

Aqueous injection fluid and method for sulfate scale inhibition in subterranean formations

Inventors: Muhammad Israr (Dhahran, SA); Mobeen Murtaza (Ashariqya, SA); Syed Muhammad Shakil Hussain (Dhahran, SA); Muhammad Shahzad Kamal (Dhahran, SA)
Assignee: King Fahd University of Petroleum and Minerals
C09K8/532
View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 12,534,664
App. No.
19/215,103
Granted
Jan 27, 2026
Kind
B1
Abstract

An aqueous injection fluid for treatment of a subterranean hydrocarbon-bearing formation includes water and at least one water soluble cationic surfactant having a general formula (DCS): where ‘R’ is C 2 -C 4 alkylene which may have one or more —O—, —S— or —S(O) 2 O— groups, ‘X − ’ is halide, ‘x’ is an integer of from 2 to 10 and, ‘y’ is an integer of from 2 to 10.

Claims (33)

1 . A method for inhibiting sulphate scale formation in a well-bore disposed in a hydrocarbon-bearing subterranean formation, comprising:

injecting into the well-bore an aqueous injection fluid comprising:

water, and

at least one water soluble cationic surfactant having a general formula (DCS):

wherein R is C 2 -C 4 alkylene which may have one or more —O—, —S— or —S(O) 2 O— groups;

X − is halide;

x is an integer of from 2 to 10; and

y is an integer of from 2 to 10.

2 . The method according to claim 1 , wherein the water is at least one selected from the group consisting of fresh water, seawater, brackish water, and formation water.

3 . The method according to claim 1 , wherein the aqueous injection fluid has a total dissolved solids content of at least about 50,000 parts per million by weight.

4 . The method according to claim 1 , wherein the aqueous injection fluid has a total dissolved solids content of from about 50,000 to about 300,000 parts per million by weight.

5 . The method according to claim 1 , wherein the water soluble cationic surfactant (DCS) has a critical micelle concentration of from about 0.015 to about 0.025 mmolL −1 .

6 . The method according to claim 1 , wherein the water soluble cationic surfactant (DCS) has a thermal degradation temperature of at least about 250° C., as determined by Thermogravimetric Analysis.

7 . The method according to claim 1 , wherein the water soluble cationic surfactant (DCS) has a thermal degradation temperature of from about 250° C. to about 300° C., as determined by Thermogravimetric Analysis.

8 . The method according to claim 1 , wherein the water soluble cationic surfactant (DCS) has a thermal degradation temperature of from about 270° C. to about 300° C., as determined by Thermogravimetric Analysis.

9 . The method according to claim 1 , wherein the aqueous injection a concentration of the at least one water soluble cationic surfactant (DCS) is from about 50 to about 2,500 parts per million by weight.

10 . The method according to claim 1 , wherein the aqueous injection fluid a concentration of the at least one water soluble cationic surfactant (DCS) is from about 50 to about, 1500 parts per million by weight.

11 . The method according to claim 1 , wherein

R is C 2 -C 4 alkylene;

X − is Cl − or Br − ;

x is an integer of from 3 to 10; and

y is an integer of from 3 to 10.

12 . The method according to claim 11 , wherein X − is Br − .

13 . The method according to claim 1 , wherein:

R is C 2 -C 4 alkylene which is interrupted by —O—;

X − is Cl − or Br − ;

x is an integer of from 3 to 10; and,

y is in an integer of from 3 to 10.

14 . The method according to claim 13 , wherein X − is Br − .

15 . The method according to claim 1 , wherein the well-bore has a static bottom hole temperature of at least about 100° C.

16 . The method according to claim 1 , wherein the well-bore has a static bottom hole temperature of at least about 150° C.

17 . The method according to claim 1 , wherein the well-bore has a bottom hole pressure of at least about 69 MPa.

18 . The method according to claim 1 , wherein the well-bore has a bottom hole pressure of from about 69 to about 138 MPa.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 22, 2025
From: ISRAR, MUHAMMAD; MURTAZA, MOBEEN; HUSSAIN, SYED MUHAMMAD SHAKIL; KAMAL, MUHAMMAD SHAHZAD
To: KING FAHD UNIVERSITY OF PETROLEUM AND MINERALS
Reel/Frame 071203/0068 →
References Cited (7)
US 20080188636A1 · Argyropoulos et al. · 2008 [cited by applicant]
US 20180135187A1 · Crawford et al. · 2018 [cited by applicant]
CN 104650838A · 2015 [cited by applicant]
CN 114806529A · 2022 [cited by applicant]
Israr (M. Israr, et al., Structural insights into pyridinium-based dicationic surfactants at harsh conditions: Influence of spacer groups on thermal stability and surface properties, Heliyon 11 (2025) e42625). [cited by examiner]
Devi (Y.G. Devi et al., Impacts of pyridinium gemini surfactants on corrosion inhibition of carbon steel, Surfaces and Interfaces 45 (2024) 103796). [cited by examiner]
M.M. Shaban, at al., “Novel trimeric cationic pyrdinium surfactants as bi-functional corrosion inhibitors and antiscalants for API 5L X70 carbon steel against oilfield formation water”, Journal of Molecular Liquids, vol… [cited by applicant]