IP Library Granted Patent US 9,080,244
Granted Patent B2
US 9,080,244 · App. 13/660,720 · Granted Jul 14, 2015

Process for iron and steel production

Inventors: Stuart Licht (Leesburg, VA); Baohui Wang (Daqing, CN)
Assignee: The George Washington University
C25C1/06C21C5/56C25C3/34
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Quick Facts
Patent No.
US 9,080,244
App. No.
13/660,720
Granted
Jul 14, 2015
Kind
B2
Abstract

A method of producing iron by: solubilizing iron oxide as a lithiated iron oxide in a molten carbonate having lithium carbonate; and subjecting the lithiated iron oxide to electrolysis to obtain iron and oxygen. The molten alkali metal carbonate salt may further include lithium oxide. Additionally the lithium carbonate may be simultaneously subjected to electrolysis to produce steel instead of iron.

Claims (37)

1. A method of producing iron comprising:

(i) solubilizing iron oxide in a molten carbonate comprising lithium carbonate to form a lithiated iron oxide; and

(ii) subjecting the lithiated iron oxide to electrolysis to obtain iron and oxygen.

2. The method of claim 1 , wherein the iron oxide comprises Fe 2 O 3 .

3. The method of claim 1 , wherein the molten carbonate is a mixed eutectic molten carbonate.

4. The method of claim 1 , wherein the molten carbonate further comprises Li 2 O.

5. The method of claim 1 , wherein the iron oxide comprises Fe 3 O 4 .

6. The method of claim 1 , wherein the iron oxide comprises impurities.

7. The method of claim 1 , wherein step (ii) occurs with carbon dioxide in contact with the molten carbonate.

8. The method of claim 1 , wherein the solubilizing in step (i) comprises dissolving iron oxide in the molten carbonate.

9. The method of claim 1 , wherein the solubilizing in step (i) comprises dissolving iron oxide in the molten carbonate in the presence of a lithium salt.

10. The method of claim 1 , wherein carbothermal carbon dioxide emission is eliminated.

11. The method of claim 1 , wherein the ratio of iron oxide to molten lithium carbonate ranges from about 20 weight percent to about 60 weight percent.

12. The method of claim 1 , wherein about 7 to about 14 moles of iron oxide is solubilized per kilogram of molten carbonate.

13. The method of claim 1 , wherein about 0.7 to about 4 moles of iron oxide is solubilized per kilogram of molten carbonate.

14. A method of producing steel comprising:

(i) solubilizing iron oxide in a molten carbonate comprising lithium carbonate to form a lithiated iron oxide; and

(ii) subjecting the lithiated iron oxide and the molten carbonate to electrolysis to obtain steel and oxygen.

15. The method of claim 14 , wherein the iron oxide comprises Fe 2 O 3 .

16. The method of claim 14 , wherein the molten carbonate is a mixed eutectic molten carbonate.

17. The method of claim 14 , wherein the molten carbonate further comprises Li 2 O.

18. The method of claim 14 , wherein the iron oxide comprises Fe 3 O 4 .

19. The method of claim 14 , wherein the iron oxide comprises impurities.

20. The method of claim 14 , wherein step (ii) occurs with carbon dioxide in contact with the molten carbonate.

21. The method of claim 14 , wherein the solubilizing in step (i) comprises dissolving iron oxide in the molten carbonate.

22. The method of claim 10 , wherein the solubilizing in step (i) comprises dissolving iron oxide in the presence of a lithium salt.

23. A method of producing iron comprising:

(i) dissolving iron oxide in a molten carbonate salt comprising lithium carbonate at a temperature sufficient to solubilize the iron oxide as lithiated iron oxide; and

(ii) subjecting the lithiated iron oxide to electrolysis to obtain iron and oxygen.

24. A method of producing steel comprising:

(i) dissolving iron oxide in a molten carbonate salt comprising lithium carbonate at a temperature sufficient to solubilize the iron oxide as lithiated iron oxide; and

(ii) subjecting the lithiated iron oxide and the molten carbonate to electrolysis to obtain steel and oxygen.

25. A method of producing iron comprising:

(i) solubilizing an oxide consisting essentially of iron oxide in a molten carbonate comprising lithium carbonate to form a lithiated iron oxide;

(ii) optionally adding a lithium salt; and

(iii) subjecting the lithiated iron oxide to electrolysis to obtain iron and oxygen.

26. The method of claim 25 , wherein the lithium salt is Li 2 O.

Assignments (3)
REDOMICILE IN FLORIDA Recorded Nov 5, 2022
From: C2CNT LLC
To: C2CNT LLC
Reel/Frame 061884/0781 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 27, 2020
From: THE GEORGE WASHINGTON UNIVERSITY
To: C2CNT LLC
Reel/Frame 052247/0387 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 11, 2013
From: LICHT, STUART; WANG, BAOHUI
To: GEORGE WASHINGTON UNIVERSITY,THE
Reel/Frame 029810/0587 →
Continuity (5)
Continuation PCTUS2011035176 · May 4, 2011
Provisional Application 61331109 · May 4, 2010
Provisional Application 61426030 · Dec 22, 2010
Provisional Application 61438610 · Feb 1, 2011
Related Publication 20130134050A1 · May 30, 2013