IP Library Granted Patent US 7,972,417
Granted Patent B2
US 7,972,417 · App. 12/053,528 · Granted Jul 5, 2011

Hydrogen gas separator system having a micro-channel construction for efficiently separating hydrogen gas from a mixed gas source

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Quick Facts
Patent No.
US 7,972,417
App. No.
12/053,528
Granted
Jul 5, 2011
Kind
B2
Abstract

A hydrogen purification method that is used to separate hydrogen gas from a source gas. A hydrogen separator into which flows the source. Within the hydrogen separator is at least one hydrogen permeable tube that is made of a hydrogen permeable material. A support tube is provided for each hydrogen permeable tube. A support tube is coaxially aligned with the hydrogen permeable tube, wherein a micro-channel exists between the hydrogen permeable tube and the support tube in an area of overlap. The source gas is introduced into the micro-channel. The source gas spreads thinly over the hydrogen permeable tube in the micro-channel. The restrictions of the micro-channel cause the source gas to embody turbulent flow characteristics as it flows through the micro-channel. The turbulent flow causes the hydrogen separator to separate hydrogen from the source gas in a highly efficient manner.

Claims (31)

1. A method of separating hydrogen gas from a source gas, comprising the steps of:

providing a tube of hydrogen permeable material having a first end, an inside surface and an inside diameter;

providing a support tube having an outside surface and an outside diameter, wherein said outside diameter of said support tube is just smaller than said inside diameter of said tube of hydrogen permeable material;

coaxially positioning said tube of hydrogen permeable material around said support tube creating a micro-channel of less than three hundred microns between said outside surface of said support tube and said inside surface of said tube of hydrogen permeable material;

providing a catalyst within said micro-channel; and

passing the source gas through said catalyst and through said micro-channel at a flow rate that causes said source gas to have turbulent flow characteristics while flowing through said micro-channel, wherein hydrogen from said source gas comes into contact with said hydrogen permeable material and is presented the opportunity to be absorbed by said hydrogen permeable material and separated from said source gas.

2. The method according to claim 1 , wherein said step of passing the source gas through said micro-channel includes introducing said source gas to said micro-channel through said support tube.

3. The method according to claim 2 , wherein said step of coaxially positioning said tube of hydrogen permeable material around said support tube includes inserting said support tube through said first end of said tube of hydrogen permeable material.

4. The method according to claim 3 , further including the step of collecting hydrogen gas separated from said source gas.

5. The method according to claim 4 , wherein said step of collecting hydrogen gas includes collecting said hydrogen gas from said first end of said tube of hydrogen permeable material.

6. The method according to claim 4 , wherein said step of providing a tube of hydrogen permeable material, includes providing a plurality of tubes of hydrogen permeable material, wherein said plurality of tubes communicate with a first common chamber.

7. The method according to claim 6 , wherein said step of collecting hydrogen gas includes drawing said hydrogen gas from said first common chamber.

8. A method of separating hydrogen gas from a source gas, comprising the steps of:

providing a tube of hydrogen permeable material having a first end, an outside surface and an outside diameter;

providing a support tube having a first end, a second end, an inside surface and an inside diameter, wherein said inside diameter of said support tube is larger than said outside diameter of said tube of hydrogen permeable material;

coaxially positioning said tube of hydrogen permeable material inside said support tube creating a micro-channel between said inside surface of said support tube and said outside surface of said tube of hydrogen permeable material; and

passing the source gas through said micro-channel at a flow rate that causes said source gas to have turbulent flow characteristics while flowing through said micro-channel, wherein hydrogen from said source gas comes into contact with said hydrogen permeable material and is absorbed by said hydrogen permeable material, therein being separated from said source gas.

9. The method according to claim 8 , wherein said micro-channel extends no more than three-hundred microns between said inside surface of said support tube and said outside surface of said tube of hydrogen permeable material.

10. The method according to claim 8 , wherein said step of passing the source gas through said micro-channel includes introducing said source gas to said micro-channel through said support tube.

11. The method according to claim 8 , wherein said step of coaxially positioning said tube of hydrogen permeable material inside said support tube includes inserting said first end of said tube of hydrogen permeable material though said second end of said support tube.

12. The method according to claim 11 , further including the step of collecting hydrogen gas separated from said source gas.

13. The method according to claim 12 , wherein said step of collecting hydrogen gas includes collecting said hydrogen gas from said first end of said tube of hydrogen permeable material.

14. The method according to claim 12 , wherein said step of providing a tube of hydrogen permeable material, includes providing a plurality of tubes of hydrogen permeable material, wherein said plurality of tubes communicate with a first common chamber.

15. The method according to claim 14 , wherein said step of collecting hydrogen gas includes drawing said hydrogen gas from said first common chamber.

16. In a hydrogen separator that separates hydrogen gas from a source gas, a method of inducing turbulent flow in said source gas as it flows past a hydrogen permeable membrane in order to produce a more efficient absorption of hydrogen from said source gas by said hydrogen permeable membrane, said method comprising:

providing a hydrogen permeable membrane in the form of hydrogen permeable tube having an open end;

providing a support tube;

coaxially aligning said hydrogen permeable tube and said support tube, wherein a micro-channel of no more than three-hundred microns exists between said hydrogen permeable tube and said support tube;

introducing said source gas into said micro-channel at a flow rate that causes said source gas to have turbulent flow characteristics as it flows through said micro-channel, wherein said hydrogen gas within said source gas permeates through said hydrogen permeable tube and is separated from said source gas; and

collecting hydrogen gas from said open end of said hydrogen permeable tube.

17. The method according to claim 16 , further including the step of introducing said source gas into said micro-channel through said supply tube.

Assignments (6)
CHANGE OF NAME Recorded Mar 4, 2026
From: SAES PURE GAS, INC.
To: ENTEGRIS GP, INC.
Reel/Frame 073971/0763 →
SECURITY INTEREST Recorded Jul 8, 2022
From: ENTEGRIS, INC.; ENTEGRIS GP, INC.; POCO GRAPHITE, INC.; CMC MATERIALS, INC.; INTERNATIONAL TEST SOLUTIONS, LLC; QED TECHNOLOGIES INTERNATIONAL, INC.
To: TRUIST BANK, AS NOTES COLLATERAL AGENT
Reel/Frame 060613/0072 →
ASSIGNMENT OF PATENT SECURITY INTEREST RECORDED AT REEL/FRAME 048811/0679 Recorded Nov 5, 2019
From: GOLDMAN SACHS BANK USA
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 050965/0035 →
SECURITY INTEREST Recorded Nov 13, 2018
From: ENTEGRIS, INC.; SAES PURE GAS, INC.
To: GOLDMAN SACHS BANK USA
Reel/Frame 048811/0679 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 13, 2013
From: POWER & ENERGY, INC.
To: SAES PURE GAS, INC.
Reel/Frame 031782/0052 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Apr 10, 2008
From: BOSSARD, PETER R.; METTES, JACOB
To: POWER & ENERGY, INC.
Reel/Frame 020792/0166 →