IP Library Granted Patent US 8,324,104
Granted Patent B2
US 8,324,104 · App. 12/934,277 · Granted Dec 4, 2012

Surface treatment in semiconductor manufacturing

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Quick Facts
Patent No.
US 8,324,104
App. No.
12/934,277
Granted
Dec 4, 2012
Kind
B2
Abstract

The present invention provides a process for forming a capping layer on a conducting interconnect for a semiconductor device, the process comprising: providing a substrate comprising one or more conductors in a dielectric layer, the conductors having an oxide layer at their surface; exposing the surface of the substrate to a vapor of β-diketone or a β-ketoimine; and depositing a capping layer on the surface of at least some of the one or more conductors. The present invention further provides an apparatus for carrying out this method.

Claims (37)

1. A process for forming a capping layer on a conducting interconnect for a semiconductor device, the process comprising:

(a) providing a substrate comprising one or more conductors in a dielectric layer, the conductors having an oxide layer at their surface;

(b) exposing the surface of the substrate to a vapour of β-diketone or β-ketoimine without cleaning the surface with an aqueous acidic solution having a pH of 4 or less following formation of the substrate comprising the one or more conductors having the oxide layer at their surface and prior to exposing; and

(c) depositing a capping layer on the surface of at least some of the one or more conductors.

2. The process of claim 1 , wherein the conductor comprises copper.

3. The process of claim 2 , wherein the oxide layer comprises an oxide of palladium.

4. The process of claim 2 , wherein the β-diketone is 1,1,1,5,5,5-hexafluoroacetylacetone.

5. The process of claim 2 , wherein step (b) is carried out in an atmosphere in which the metal is not oxidized.

6. The process of claim 1 , wherein the oxide layer comprises an oxide of palladium.

7. The process of claim 6 , wherein the β-diketone is 1,1,1,5,5,5-hexafluoroacetylacetone.

8. The process of claim 6 , wherein step (b) is carried out in an atmosphere in which the metal is not oxidized.

9. The process of claim 1 , wherein the β-diketone is 1,1,1,5,5,5-hexafluoroacetylacetone.

10. The process of claim 1 , wherein step (b) is carried out in an atmosphere in which the metal is not oxidized.

11. The method of claim 1 , wherein providing a substrate includes providing the substrate following chemical mechanic polishing (CMP) of the substrate.

12. The method of claim 1 , wherein exposing the surface of the substrate to a vapour includes exposing the surface to a vapour comprising β-ketoimine.

13. An apparatus for depositing a capping layer on a conducting interconnect, the apparatus comprising:

a chemical mechanical polishing device;

a first chamber having a support to support a substrate and a heater to heat a substrate placed on the support,

a source of β-diketone or β-ketoimine vapour,

a vacuum pump associated with said first chamber,

a second chamber for carrying out deposition of a capping layer;

the apparatus being adapted so that a substrate may be transferred from said first chamber to said second chamber in a non-oxidizing atmosphere; and

the apparatus being adapted so that the substrate may be transferred from said chemical mechanical polishing device to said first chamber without cleaning with an aqueous acidic solution having a pH of 4 or less.

14. The apparatus according to claim 13 , wherein the source of β-diketone or β-ketoimine vapour comprises a bubbler containing a liquid β-diketone or β-ketoimine connected to said first chamber, and a source of carrier gas connected to said bubbler.

15. The apparatus according to claim 14 , the apparatus further comprising a controller and instructions associated with the controller, wherein the instructions, when executed by the controller, exposes the surface of a substrate placed in the first chamber of the apparatus to a vapour of β-diketone or a β-ketoimine.

16. The apparatus according to claim 13 , the apparatus further comprising a controller and instructions associated with the controller, wherein the instructions, when executed by the controller, exposes the surface of a substrate placed in the first chamber of the apparatus to a vapour of β-diketone or a β-ketoimine.

17. A semiconductor device having conducting interconnects provided with a capping layer obtainable with a process comprising:

(a) providing a substrate comprising one or more conductors in a dielectric layer, the conductors having an oxide layer at their surface;

(b) exposing the surface of the substrate to a vapour of β-diketone or β-ketoimine without cleaning the surface with an aqueous acidic solution having a pH of 4 or less following formation of the substrate comprising the one or more conductors having the oxide layer at their surface and prior to exposing; and

(c) depositing a capping layer on the surface of at least some of the one or more conductors.

18. The device of claim 17 , wherein the conductor comprises copper.

19. The device of claim 17 , wherein the oxide layer comprises an oxide of palladium.

20. The device of claim 19 , wherein step (b) is carried out in an atmosphere in which the metal is not oxidized.

21. The device of claim 17 , wherein the β-diketone is 1,1,1,5,5,5-hexafluoroacetylacetone.

22. The device of claim 17 , wherein step (b) is carried out in an atmosphere in which the metal is not oxidized.

23. The semiconductor device of claim 17 , wherein providing a substrate includes providing the substrate following chemical mechanic polishing (CMP) of the substrate.

24. The semiconductor device of claim 17 , wherein exposing the surface of the substrate to a vapour includes exposing the surface to a vapour comprising β-ketoimine.

Assignments (31)
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVE APPLICATION 11759915 AND REPLACE IT WITH APPLICATION 11759935 PREVIOUSLY RECORDED ON REEL 040925 FRAME 0001. ASSIGNOR(S) HEREBY CONFIRMS THE RELEASE OF SECURITY INTEREST. Recorded Feb 17, 2020
From: MORGAN STANLEY SENIOR FUNDING, INC.
To: NXP, B.V. F/K/A FREESCALE SEMICONDUCTOR, INC.
Reel/Frame 052917/0001 →
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVE APPLICATION 11759915 AND REPLACE IT WITH APPLICATION 11759935 PREVIOUSLY RECORDED ON REEL 040928 FRAME 0001. ASSIGNOR(S) HEREBY CONFIRMS THE RELEASE OF SECURITY INTEREST. Recorded Jan 17, 2020
From: MORGAN STANLEY SENIOR FUNDING, INC.
To: NXP B.V.
Reel/Frame 052915/0001 →
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVE APPLICATION 11759915 AND REPLACE IT WITH APPLICATION 11759935 PREVIOUSLY RECORDED ON REEL 037486 FRAME 0517. ASSIGNOR(S) HEREBY CONFIRMS THE ASSIGNMENT AND ASSUMPTION OF SECURITY INTEREST IN PATENTS. Recorded Dec 10, 2019
From: CITIBANK, N.A.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 053547/0421 →
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVE APPLICATION 12298143 PREVIOUSLY RECORDED ON REEL 039361 FRAME 0212. ASSIGNOR(S) HEREBY CONFIRMS THE SECURITY AGREEMENT SUPPLEMENT. Recorded Oct 22, 2019
From: NXP B.V.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 051029/0387 →
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVE APPLICATION 12298143 PREVIOUSLY RECORDED ON REEL 042985 FRAME 0001. ASSIGNOR(S) HEREBY CONFIRMS THE SECURITY AGREEMENT SUPPLEMENT. Recorded Oct 22, 2019
From: NXP B.V.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 051029/0001 →
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVE APPLICATION 12298143 PREVIOUSLY RECORDED ON REEL 038017 FRAME 0058. ASSIGNOR(S) HEREBY CONFIRMS THE SECURITY AGREEMENT SUPPLEMENT. Recorded Oct 22, 2019
From: NXP B.V.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 051030/0001 →
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVE APPLICATION 12298143 PREVIOUSLY RECORDED ON REEL 042762 FRAME 0145. ASSIGNOR(S) HEREBY CONFIRMS THE SECURITY AGREEMENT SUPPLEMENT. Recorded Oct 22, 2019
From: NXP B.V.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 051145/0184 →
RELEASE OF SECURITY INTEREST Recorded Sep 10, 2019
From: MORGAN STANLEY SENIOR FUNDING, INC.
To: NXP B.V.
Reel/Frame 050745/0001 →
RELEASE OF SECURITY INTEREST Recorded Sep 10, 2019
From: MORGAN STANLEY SENIOR FUNDING, INC.
To: NXP B.V.
Reel/Frame 050744/0097 →
CORRECTIVE ASSIGNMENT TO CORRECT THE TO CORRECT THE APPLICATION NO. FROM 13,883,290 TO 13,833,290 PREVIOUSLY RECORDED ON REEL 041703 FRAME 0536. ASSIGNOR(S) HEREBY CONFIRMS THE THE ASSIGNMENT AND ASSUMPTION OF SECURITY INTEREST IN PATENTS.. Recorded Feb 20, 2019
From: MORGAN STANLEY SENIOR FUNDING, INC.
To: SHENZHEN XINGUODU TECHNOLOGY CO., LTD.
Reel/Frame 048734/0001 →
CORRECTIVE ASSIGNMENT TO CORRECT THE NATURE OF CONVEYANCE PREVIOUSLY RECORDED AT REEL: 040632 FRAME: 0001. ASSIGNOR(S) HEREBY CONFIRMS THE MERGER AND CHANGE OF NAME. Recorded Sep 21, 2017
From: FREESCALE SEMICONDUCTOR INC.
To: NXP USA, INC.
Reel/Frame 044209/0047 →
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVE APPLICATION 12681366 PREVIOUSLY RECORDED ON REEL 039361 FRAME 0212. ASSIGNOR(S) HEREBY CONFIRMS THE SECURITY AGREEMENT SUPPLEMENT. Recorded May 9, 2017
From: NXP B.V.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 042762/0145 →
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVE APPLICATION 12681366 PREVIOUSLY RECORDED ON REEL 038017 FRAME 0058. ASSIGNOR(S) HEREBY CONFIRMS THE SECURITY AGREEMENT SUPPLEMENT. Recorded May 9, 2017
From: NXP B.V.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 042985/0001 →
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVE PATENTS 8108266 AND 8062324 AND REPLACE THEM WITH 6108266 AND 8060324 PREVIOUSLY RECORDED ON REEL 037518 FRAME 0292. ASSIGNOR(S) HEREBY CONFIRMS THE ASSIGNMENT AND ASSUMPTION OF SECURITY INTEREST IN PATENTS. Recorded Feb 1, 2017
From: CITIBANK, N.A.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 041703/0536 →
CHANGE OF NAME Recorded Nov 8, 2016
From: FREESCALE SEMICONDUCTOR, INC.
To: NXP USA, INC.
Reel/Frame 040632/0001 →
RELEASE OF SECURITY INTEREST Recorded Nov 7, 2016
From: MORGAN STANLEY SENIOR FUNDING, INC.
To: NXP B.V.
Reel/Frame 040928/0001 →
RELEASE OF SECURITY INTEREST Recorded Sep 21, 2016
From: MORGAN STANLEY SENIOR FUNDING, INC.
To: NXP, B.V., F/K/A FREESCALE SEMICONDUCTOR, INC.
Reel/Frame 040925/0001 →
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVE APPLICATION 12092129 PREVIOUSLY RECORDED ON REEL 038017 FRAME 0058. ASSIGNOR(S) HEREBY CONFIRMS THE SECURITY AGREEMENT SUPPLEMENT. Recorded Jul 14, 2016
From: NXP B.V.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 039361/0212 →
SUPPLEMENT TO THE SECURITY AGREEMENT Recorded Jun 16, 2016
From: FREESCALE SEMICONDUCTOR, INC.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 039138/0001 →
SECURITY AGREEMENT SUPPLEMENT Recorded Mar 7, 2016
From: NXP B.V.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 038017/0058 →
ASSIGNMENT AND ASSUMPTION OF SECURITY INTEREST IN PATENTS Recorded Jan 13, 2016
From: CITIBANK, N.A.
To: MORGAN STANLEY SENIOR FUNDING, INC.
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ASSIGNMENT AND ASSUMPTION OF SECURITY INTEREST IN PATENTS Recorded Jan 12, 2016
From: CITIBANK, N.A.
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 037486/0517 →
PATENT RELEASE Recorded Dec 21, 2015
From: CITIBANK, N.A., AS COLLATERAL AGENT
To: FREESCALE SEMICONDUCTOR, INC.
Reel/Frame 037357/0285 →
PATENT RELEASE Recorded Dec 21, 2015
From: CITIBANK, N.A., AS COLLATERAL AGENT
To: FREESCALE SEMICONDUCTOR, INC.
Reel/Frame 037357/0334 →
PATENT RELEASE Recorded Dec 21, 2015
From: CITIBANK, N.A., AS COLLATERAL AGENT
To: FREESCALE SEMICONDUCTOR, INC.
Reel/Frame 037357/0387 →
SECURITY AGREEMENT Recorded Nov 6, 2013
From: FREESCALE SEMICONDUCTOR, INC.
To: CITIBANK, N.A., AS NOTES COLLATERAL AGENT
Reel/Frame 031591/0266 →
SECURITY AGREEMENT Recorded Jun 18, 2013
From: FREESCALE SEMICONDUCTOR, INC.
To: CITIBANK, N.A., AS NOTES COLLATERAL AGENT
Reel/Frame 030633/0424 →
SECURITY AGREEMENT Recorded Jan 31, 2012
From: FREESCALE SEMICONDUCTOR, INC.
To: CITIBANK, N.A., AS COLLATERAL AGENT
Reel/Frame 027621/0928 →
SECURITY AGREEMENT Recorded Jan 31, 2012
From: FREESCALE SEMICONDUCTOR, INC.
To: CITIBANK, N.A., AS COLLATERAL AGENT
Reel/Frame 027622/0075 →
SECURITY AGREEMENT Recorded Jan 31, 2012
From: FREESCALE SEMICONDUCTOR, INC.
To: CITIBANK, N.A., AS COLLATERAL AGENT
Reel/Frame 027622/0477 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 24, 2010
From: CALVO-MUNOZ, MARIA LUISA; FARKAS, JANOS
To: FREESCALE SEMICONDUCTOR INC.
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