IP Library Granted Patent US 10,041,168
Granted Patent B2
US 10,041,168 · App. 14/152,751 · Granted Aug 7, 2018

Graphene structure

Inventors: David A. Boyd (La Cañada Flintridge, CA); Nai-Chang Yeh (Pasadena, CA)
Assignee: California Institute of Technology
C23C16/26C01B32/184C01B32/186C23C16/4405C23C16/511Y10T428/24355
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Quick Facts
Patent No.
US 10,041,168
App. No.
14/152,751
Granted
Aug 7, 2018
Kind
B2
Abstract

A method of forming graphene includes placing a substrate in a processing chamber and introducing a cleaning gas including hydrogen and nitrogen into the processing chamber. The method also includes introducing a carbon source into the processing chamber and initiating a microwave plasma in the processing chamber. The method further includes subjecting the substrate to a flow of the cleaning gas and the carbon source for a predetermined period of time to form the graphene.

Claims (22)

1. A graphene structure comprising:

a copper substrate; and

a single monolayer of CMOS compatible graphene grown at a maximum temperature of 425° C. and disposed on the copper substrate and having an area measured in a unit of length squared, wherein the area is associated with a grain ranging in size between 100 μm and 300 μm and wherein the single monolayer of CMOS compatible graphene is characterized by a height variation measured in the unit of length such that a ratio of the height variation to the area is less than 2.5×10 −2 (per unit of length).

2. The graphene structure of claim 1 wherein the ratio of the height variation to the area is less than 1.25×10 −2 (per unit of length).

3. The graphene structure of claim 1 wherein the single monolayer of CMOS compatible graphene is characterized by a strain variation of less than 0.05%.

4. The graphene structure of claim 1 wherein the copper substrate comprises a single crystal copper substrate.

5. The graphene structure of claim 2 wherein the ratio of the height variation to the area is less than 1.0×10 −2 (per unit of length).

6. The graphene structure of claim 4 wherein the single crystal copper substrate comprises a single crystal (100) substrate.

7. The graphene structure of claim 4 wherein the single crystal copper substrate comprises a single crystal (111) substrate.

8. The graphene structure of claim 1 wherein the ratio of the height variation to the area is greater than 0.25×10 −2 (per unit of length).

9. The graphene structure of claim 1 wherein the unit of length is nanometers.

10. The graphene structure of claim 1 wherein the area is free of grain boundaries.

11. The graphene structure of claim 1 wherein the single monolayer of CMOS compatible graphene is characterized by a first Raman peak associated with a 2D-band mode and a second Raman peak associated with a G-band mode, wherein a ratio of the first Raman Peak to the second Raman peak is about three.

12. A graphene structure comprising:

a copper substrate; and

a single monolayer of CMOS compatible graphene disposed on the copper substrate, grown at a maximum temperature of 425° C., and having a measurement area less than or equal to 100 nm 2 , wherein the measurement area is associated with a grain ranging in size between 100 μm and 300 μm and wherein the single monolayer of CMOS compatible graphene is characterized by a height variation measured in nanometers such that a ratio of the height variation to the measurement area is less than 2.5×10 −2 per nanometer.

13. The graphene structure of claim 12 wherein the ratio of the height variation to the measurement area is less than 1.25×10 −2 per nanometer.

14. The graphene structure of claim 13 wherein the ratio of the height variation to the measurement area is less than 1.0×10 −2 per nanometer.

15. The graphene structure of claim 12 wherein the single monolayer of CMOS compatible graphene is characterized by a strain variation of less than 0.05%.

16. The graphene structure of claim 12 wherein the copper substrate comprises a single crystal copper substrate.

17. The graphene structure of claim 16 wherein the single crystal copper substrate comprises a single crystal (111) substrate.

18. The graphene structure of claim 16 wherein the single crystal copper substrate comprises a single crystal (100) substrate.

Assignments (2)
CONFIRMATORY LICENSE Recorded Jul 16, 2014
From: CALIFORNIA INSTITUTE OF TECHNOLOGY
To: NATIONAL SCIENCE FOUNDATION
Reel/Frame 033341/0046 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 12, 2014
From: BOYD, DAVID A.; YEH, NAI-CHANG
To: CALIFORNIA INSTITUTE OF TECHNOLOGY
Reel/Frame 032412/0876 →
Continuity (5)
Provisional Application 61752209 · Jan 14, 2013
Provisional Application 61752549 · Jan 15, 2013
Provisional Application 61897082 · Oct 29, 2013
Provisional Application 61907628 · Nov 22, 2013
Related Publication 20150079342A1 · Mar 19, 2015
Cited By (1)
US 12,312,679