IP Library Granted Patent US 9,537,095
Granted Patent B2
US 9,537,095 · App. 14/332,924 · Granted Jan 3, 2017

Tellurium compounds useful for deposition of tellurium containing materials

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Quick Facts
Patent No.
US 9,537,095
App. No.
14/332,924
Granted
Jan 3, 2017
Kind
B2
Abstract

Precursors for use in depositing tellurium-containing films on substrates such as wafers or other microelectronic device substrates, as well as associated processes of making and using such precursors, and source packages of such precursors. The precursors are useful for deposition of Ge 2 Sb 2 Te 5 chalcogenide thin films in the manufacture of nonvolatile Phase Change Memory (PCM), by deposition techniques such as chemical vapor deposition (CVD) and atomic layer deposition (ALD).

Claims (20)

1. A method of forming a phase change material comprising a tellurium-containing film, comprising volatilizing a tellurium precursor composition to form a tellurium precursor vapor, and contacting the tellurium precursor vapor with a substrate to deposit tellurium thereon, wherein the tellurium precursor composition comprises a tellurium precursor comprising a diorgano ditelluride compound wherein each organo group is the same and is selected from the group consisting of C 1 -C 8 alkyl; C 1 -C 12 hydrocarbyl selected from aryl, fluoroalkyl, allyl, alkenyl or dienyl; silyl; and substituted silyl.

2. The method of claim 1 , wherein the tellurium precursor is a dialkyl ditelluride wherein the alkyl is C 1 -C 8 alkyl.

3. The method of claim 1 , wherein the tellurium precursor is a C 1 -C 12 hydrocarbyl selected from aryl, fluoroalkyl, allyl, alkenyl or dienyl.

4. The method of claim 1 , wherein the tellurium precursor is diisopropyl ditelluride.

5. The method of claim 1 , wherein the tellurium precursor is dimethyl ditelluride.

6. The method of claim 1 , wherein the tellurium precursor is diethylditelluride.

7. The method of claim 1 , wherein the phase change material is a GST film.

8. The method of claim 1 , wherein the contacting comprises atomic layer deposition.

9. The method of claim 1 , wherein the contacting comprises chemical vapor deposition.

10. The method of claim 1 , wherein the tellurium-containing film is an amorphous Sb 2 Te 3 film.

11. The method of claim 1 , wherein the tellurium is deposited at a temperature below 300° C.

12. The method of claim 1 , wherein the tellurium precursor composition further comprises a solvent medium with the tellurium precursor dissolved therein.

13. A method of forming a GST film comprising volatilizing a tellurium precursor composition to form a tellurium precursor vapor, and contacting the tellurium precursor vapor with a substrate to deposit tellurium thereon, wherein the tellurium precursor composition comprises a tellurium precursor comprising a diorgano ditelluride compound wherein each organo group is the same and is selected from the group consisting of C 1 -C 8 alkyl; C 1 -C 12 hydrocarbyl selected from aryl, fluoroalkyl, allyl, alkenyl or dienyl; silyl; and substituted silyl.

14. The method of claim 13 , wherein the tellurium precursor is a dialkyl ditelluride wherein the alkyl is C 1 -C 8 alkyl.

15. The method of claim 14 , wherein the tellurium precursor is dimethyl ditelluride, diethyl ditelluride or diisopropyl ditelluride.

16. The method of claim 15 , wherein the tellurium precursor is diisopropyl ditelluride.

17. The method of claim 13 , wherein the contacting comprises atomic layer deposition.

18. The method of claim 13 , wherein the contacting comprises chemical vapor deposition.

19. The method of claim 13 , wherein the tellurium-containing film is an amorphous Sb 2 Te 3 film.

20. The method of claim 13 , wherein the tellurium is deposited at a temperature below 300° C.

Assignments (6)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jul 9, 2021
From: ENTEGRIS, INC.
To: SAMSUNG ELECTRONICS CO., LTD.
Reel/Frame 056803/0565 →
RELEASE OF SECURITY INTEREST Recorded Jun 15, 2021
From: MORGAN STANLEY SENIOR FUNDING, INC.
To: ENTEGRIS, INC.
Reel/Frame 056550/0726 →
ASSIGNMENT OF PATENT SECURITY INTEREST RECORDED AT REEL/FRAME 048811/0679 Recorded Nov 5, 2019
From: GOLDMAN SACHS BANK USA
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 050965/0035 →
SECURITY INTEREST Recorded Nov 13, 2018
From: ENTEGRIS, INC.; SAES PURE GAS, INC.
To: GOLDMAN SACHS BANK USA
Reel/Frame 048811/0679 →
CORRECTIVE ASSIGNMENT TO CORRECT THE EXECUTION DATE FOR INVENTOR MATTHIAS STENDER PREVIOUSLY RECORDED ON REEL 033589 FRAME 0579. ASSIGNOR(S) HEREBY CONFIRMS THE ASSIGNMENT. Recorded Sep 2, 2014
From: STENDER, MATTHIAS; XU, CHONGYING; CHEN, TIANNIU; HUNKS, WILLIAM; CHEN, PHILIP S.H.; ROEDER, JEFFREY F.; BAUM, THOMAS H.
To: ENTEGRIS, INC.
Reel/Frame 033667/0243 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 22, 2014
From: STENDER, MATTHIAS; XU, CHONGYING; CHEN, TIANNIU; HUNKS, WILLIAM; CHEN, PHILIP S.H.; ROEDER, JEFFREY F.; BAUM, THOMAS H.
To: ENTEGRIS, INC.
Reel/Frame 033589/0579 →