IP Library Granted Patent US 10,894,233
Granted Patent B2
US 10,894,233 · App. 16/027,896 · Granted Jan 19, 2021

Silicon carbide filter membrane and methods of use

Inventors: Troy Scoggins (Decatur, TX); Abuagela Rashed (Denton, TX)
Assignee: ENTEGRIS, INC.
B01D69/12B01D71/02B01D2325/02B01D2325/04
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Quick Facts
Patent No.
US 10,894,233
App. No.
16/027,896
Granted
Jan 19, 2021
Kind
B2
Abstract

Described are silicon carbide filters for use with liquid metals such as liquid tin, as well as methods of using such a filter to remove particles from the liquid metal, and systems and processes that use the filtered liquid metal.

Claims (35)

1. A multi-layer porous silicon carbide filter membrane for filtering molten tin comprising:

a fine membrane layer of fine porous silicon carbide having a fine pore size and a porosity in a range of from 15 to 27 percent, and

a coarse membrane layer of coarse porous silicon carbide having a coarse pore size and a porosity in a range of from 15 to 22 percent, the coarse pore size being greater than the fine pore size and the fine membrane layer being upstream of the course membrane layer.

2. The membrane of claim 1 , wherein the fine porous silicon carbide has an average pore size of less than 2.0 microns.

3. The membrane of claim 1 , wherein the fine porous silicon carbide has an average pore size of less than 1 micron.

4. The membrane of claim 1 , wherein the coarse membrane has a pore size of greater than 2.0 microns.

5. The membrane of claim 1 , wherein the fine porous silicon carbide has a bubble point of not greater than 15 pounds per square inch.

6. The membrane of claim 1 , wherein the coarse porous silicon carbide has a bubble point of not greater than 20 pounds per square inch.

7. The membrane of claim 1 , wherein the fine porous silicon carbide has a porosity in a range from 20 to 25.

8. The membrane of claim 1 , wherein the fine membrane layer has a thickness in a range from 1 to 7 millimeters.

9. The membrane of claim 1 , wherein the coarse membrane layer has a thickness in a range from 1 to 7 millimeters.

10. The membrane of claim 1 , wherein a total thickness of the fine membrane layer and the coarse membrane layer is in a range from 1 to 15 millimeters.

11. The membrane according to claim 1 , wherein:

the fine membrane layer has silicon carbide particulates that can be detected on a surface of the fine membrane layer, and

the coarse membrane layer has silicon carbide particulates that can be detected on a surface of the coarse membrane layer in an amount that is reduced relative to the amount of silicon carbide particulates that can be detected on a surface of the fine membrane layer.

12. A method of processing molten tin, the method comprising:

(a) providing a multi-layer porous silicon carbide filter membrane comprising:

(i) a fine membrane layer of fine porous silicon carbide having a fine pore size and a porosity in a range of from 15 to 27 percent, and

(ii) a coarse membrane layer of coarse porous silicon carbide having a coarse pore size and a porosity in a range of from 15 to 22 percent such that the pore size of the coarse porous silicon carbide is greater than the pore size of the fine porous silicon carbide and the fine membrane layer is upstream of the coarse membrane layer;

(b) passing the liquid metal through the multi-layer porous silicon carbide filter membrane by first passing the liquid metal through the fine membrane layer; and

(c) after passing the liquid metal through the fine membrane, passing the liquid metal through the coarse membrane layer.

13. The method of claim 12 , wherein the liquid metal is at a temperature of at least 200 degrees Celsius.

14. The method of claim 12 , wherein the fine porous silicon carbide has an average pore size of less than 2.0 microns.

15. The method of claim 12 , wherein the coarse membrane has a pore size of greater than 2.0 microns.

16. The method of claim 12 , wherein the fine porous silicon carbide has a porosity in a range from 20 to 25 percent.

17. The method of claim 12 , wherein the fine membrane layer has a thickness in a range from 1 to 7 millimeters.

18. The method of claim 12 , wherein the coarse membrane layer has a thickness in a range from 1 to 7 millimeters.

19. A method of generating EUV comprising

(a) providing a multi-layer porous silicon carbide filter membrane comprising:

(i) a fine membrane layer of fine porous silicon carbide having a fine pore size and a porosity in a range of from 15 to 27 percent, and

(ii) a coarse membrane layer of coarse porous silicon carbide having a coarse pore size and a porosity in a range of from 15 to 22 percent such that the pore size of the coarse porous silicon carbide is greater than the pore size of the fine porous silicon carbide and the fine membrane layer is upstream of the coarse membrane layer;

(b) passing liquid tin through the multi-layer porous silicon carbide filter membrane by first passing the liquid tin through the fine membrane layer;

(c) after passing the liquid tin through the fine membrane, passing the liquid tin through the coarse membrane layer;

(d) forming the liquid tin into a droplet; and

(e) irradiating the liquid tin to generate extreme ultraviolet radiation.

Assignments (4)
SECURITY INTEREST Recorded Jul 8, 2022
From: ENTEGRIS, INC.; ENTEGRIS GP, INC.; POCO GRAPHITE, INC.; CMC MATERIALS, INC.; INTERNATIONAL TEST SOLUTIONS, LLC; QED TECHNOLOGIES INTERNATIONAL, INC.
To: TRUIST BANK, AS NOTES COLLATERAL AGENT
Reel/Frame 060613/0072 →
ASSIGNMENT OF PATENT SECURITY INTEREST RECORDED AT REEL/FRAME 048811/0679 Recorded Nov 5, 2019
From: GOLDMAN SACHS BANK USA
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 050965/0035 →
SECURITY INTEREST Recorded Nov 13, 2018
From: ENTEGRIS, INC.; SAES PURE GAS, INC.
To: GOLDMAN SACHS BANK USA
Reel/Frame 048811/0679 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jul 5, 2018
From: SCOGGINS, TROY; RASHED, ABUAGELA
To: ENTEGRIS, INC.
Reel/Frame 046272/0174 →