IP Library Granted Patent US 11,114,674
Granted Patent B2
US 11,114,674 · App. 16/049,034 · Granted Sep 7, 2021

Proton conductive two-dimensional amorphous carbon film for gas membrane and fuel cell applications

Inventors: Barbaros Ozyilmaz (Singapore, SG); Henrik Andersen (Singapore, SG); Chee Tat Toh (Singapore, SG)
Assignee: National University of Singapore
H01M4/98C23C14/0005C23C16/01C23C16/27H01M4/8657H01M4/8803H01M8/1023H01M8/1039H01M8/1053H01M2008/1095
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Quick Facts
Patent No.
US 11,114,674
App. No.
16/049,034
Granted
Sep 7, 2021
Kind
B2
Abstract

Described is a fuel cell comprising an electrode catalyst assembly, and a two-dimensional (2D) amorphous carbon, wherein the 2D amorphous carbon has a crystallinity (C)≤0.8.

Claims (38)

1. A fuel cell comprising:

an electrode catalyst assembly;

a two-dimensional (2D) amorphous carbon, wherein the 2D amorphous carbon has a crystallinity (C)≤0.8, and

a proton exchange membrane,

wherein the 2D amorphous carbon is disposed between the electrode catalyst assembly and the proton exchange membrane.

2. The fuel cell of claim 1 , wherein the 2D amorphous carbon is a membrane.

3. The fuel cell of claim 1 , wherein the 2D amorphous carbon is a film.

4. The fuel cell of claim 1 , wherein the 2D amorphous carbon has a resistivity of 0.01 to 1000 Ω-cm, inclusive.

5. The fuel cell of claim 1 ,

wherein the electrode catalyst assembly comprises multiple electrode catalyst assemblies,

wherein the proton exchange membrane is disposed between the multiple electrode catalyst assemblies and the 2D amorphous carbon is disposed between each electrode catalyst assembly and the proton exchange membrane.

6. The fuel cell of claim 1 ,

wherein the electrode catalyst assembly comprises multiple electrode catalyst assemblies,

wherein the proton exchange membrane comprises multiple proton exchange membranes,

wherein the 2D amorphous carbon is disposed between the multiple proton exchange membranes, and the multiple proton exchange membranes are disposed between the multiple electrode catalyst assemblies.

7. The fuel cell of claim 1 , wherein the proton exchange membrane is a fluoropolymer.

8. The fuel cell of claim 7 , wherein the fluoropolymer is Nafion®.

9. The fuel cell of claim 1 , wherein the 2D amorphous carbon has a sp 3 /sp 2 bond ratio is 0.2 or less.

10. A fuel cell comprising:

an electrode catalyst assembly; and

a two-dimensional (2D) amorphous carbon having an atomic structure consisting of non-hexagonal carbon rings and hexagonal carbon rings,

wherein a ratio of the hexagonal carbon rings to the non-hexagonal carbon rings is less than 1.0,

wherein the 2D amorphous carbon has a crystallinity (C)<1 and a sp 3 /sp 2 bond ratio is 0.2 or less.

11. The fuel cell of claim 10 , wherein the 2D amorphous carbon is a membrane.

12. The fuel cell of claim 10 , wherein the 2D amorphous carbon is a film.

13. The fuel cell of claim 10 , wherein the 2D amorphous carbon has a resistivity of 0.01 to 1000 Ω-cm, inclusive.

14. The fuel cell of claim 10 , further comprising:

a proton exchange membrane.

15. The fuel cell of claim 14 , wherein the 2D amorphous carbon is disposed between the electrode catalyst assembly and the proton exchange membrane.

16. The fuel cell of claim 14 ,

wherein the electrode catalyst assembly comprises multiple electrode catalyst assemblies,

wherein the proton exchange membrane is disposed between the multiple electrode catalyst assemblies and the 2D amorphous carbon is disposed between each electrode catalyst assembly and the proton exchange membrane.

17. The fuel cell of claim 14 ,

wherein the electrode catalyst assembly comprises multiple electrode catalyst assemblies,

wherein the proton exchange membrane comprises multiple proton exchange membranes,

wherein the 2D amorphous carbon is disposed between the multiple proton exchange membranes, and the multiple proton exchange membranes are disposed between the multiple electrode catalyst assemblies.

18. The fuel cell of claim 14 , wherein the proton exchange membrane is a fluoropolymer.

19. The fuel cell of claim 18 , wherein the fluoropolymer is Nafion®.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 12, 2020
From: OZYILMAZ, BARBAROS; ANDERSEN, HENRIK; TOH, CHEE TAT
To: NATIONAL UNIVERSITY OF SINGAPORE
Reel/Frame 051793/0677 →
Priority Claims (1)
WO PCT/SG2018/050082 · Feb 23, 2018 · international
Continuity (4)
Continuation In Part 15901099 · Feb 21, 2018
Provisional Application 62549680 · Aug 17, 2017
Provisional Application 62463112 · Feb 24, 2017
Related Publication 20180337411A1 · Nov 22, 2018
Cited By (3)
US 12,264,070 US 12,365,590 US 12,431,350