IP Library Granted Patent US 10,975,320
Granted Patent B2
US 10,975,320 · App. 16/505,428 · Granted Apr 13, 2021

Processes for producing high biogenic concentration Fischer-Tropsch liquids derived from municipal solid wastes (MSW) feedstocks

Inventors: Peter G. Tiverios (Anderson, SC); Stephen H. Lucas (Foristell, MO); Lewis L. Rich (Seneca, SC)
Assignee: Fulcrum BioEnergy, Inc.
C10L1/04B01J8/00B01J19/0006C07C29/1518C10G2/32C10G2/34C10G47/00C10J3/26C10J3/466C10J3/485C10J3/721C10J3/82C10K1/004C10K1/005C10K1/101C10K1/16C10K3/001C10K3/04C10L1/08B01J2208/00115C10J2300/0903C10J2300/0906C10J2300/0946C10J2300/0959C10J2300/0976C10J2300/1628C10J2300/1634C10J2300/1643C10J2300/1659C10J2300/1665C10J2300/1671C10J2300/1675C10J2300/1815C10J2300/1853C10L2200/0469C10L2200/0492C10L2270/023C10L2270/026C10L2270/04C10L2290/04C10L2290/10C10L2290/42C10L2290/54C10L2290/543Y02E20/16Y02E50/10Y02E50/30Y02P20/129Y02P20/133Y02P30/00
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Quick Facts
Patent No.
US 10,975,320
App. No.
16/505,428
Granted
Apr 13, 2021
Kind
B2
Abstract

Processes for producing high biogenic concentration Fischer-Tropsch liquids derived from the organic fraction of municipal solid wastes (MSW) feedstock that contains a relatively high concentration of biogenic carbon (derived from plants) and a relatively low concentration of non-biogenic carbon (derived from fossil sources) wherein the biogenic content of the Fischer-Tropsch liquids is the same as the biogenic content of the feedstock.

Claims (24)

1. A transportation fuel or fuel additive derived from municipal solid wastes (MSW) that contain materials that are produced from biogenic derived carbon materials and non-biogenic derived carbon materials, the transportation fuel or fuel additive derived from a process comprising the steps of:

a) in a feedstock processing step, removing some of the non-biogenic derived carbon materials and non-carbonaceous materials from municipal solid wastes to produce a processed MSW feedstock that contains a higher concentration of biogenic carbon materials than non-biogenic carbon materials; and

b) converting the processed MSW feedstock into Fischer-Tropsch liquids in a bio-refinery while maintaining a greater concentration of biogenic carbon than non-biogenic carbon; and

c) upgrading the Fischer-Tropsch liquids into a transportation fuel or fuel additive while maintaining a greater concentration of biogenic carbon than non-biogenic carbon.

2. The transportation fuel or fuel additive derived by the process according to claim 1 wherein the step of converting the processed MSW feedstock into Fischer-Tropsch liquids in the bio-refinery, further comprises: converting the processed MSW feedstock in a gasification island.

3. The transportation fuel or fuel additive derived by the process according to claim 1 wherein, in the feedstock processing step, more than about 10% of the non-biogenic derived carbon materials are removed.

4. The transportation fuel or fuel additive derived by the process according to claim 1 wherein, in the feedstock processing step, up to about 80% of the non-biogenic derived carbon materials are removed.

5. The transportation fuel or additive derived by the process according to claim 1 wherein in the feedstock processing step, between about 10% and about 90% of the non-biogenic derived carbon materials are removed.

6. The transportation fuel or fuel additive derived by the process according to claim 1 wherein the converting step is comprised of three stages carried out in a gasification island:

1) steam reforming the processed feedstock in a steam reformer configured to dry, volatilize and gasify the processed feedstock to produce syngas containing CO, H 2 , H 2 O and CO 2 , unreacted char, inert solids and unreacted hydrocarbons;

2) further gasifying in a sub-stoichiometric carbon oxidation unit configured to gasify the unreacted char from the steam reformer; and

3) hydrocarbon reforming in a hydrocarbon reforming unit configured to convert remaining char, hydrocarbons and tars into syngas.

7. The transportation fuel or fuel additive derived by the process according to claim 6 , further comprising:

conditioning the syngas in a syngas conditioning unit configured to receive the syngas from the gasification island and remove contaminants, remove/recover CO 2 and provide a biogenic CO 2 recycle stream for recycling high biogenic CO 2 to the gasification island for biogenic carbon conservation and to adjust the H 2 :CO 2 ratio in the syngas to a predetermined value; and

converting the syngas into Fischer-Tropsch liquids in one or more F-T reactors;

separating the F-T liquids in a separation system into heavy F-T liquids (HFTL) and medium F-T liquids (MFTL); and

upgrading the separated F-T liquids in an upgrading system comprising a hydrotreating/hydrocracking reactor and fractionation system configured to upgrade the HFTL and MFTL into a transportation fuel.

8. The transportation fuel or fuel additive derived by the process according to claim 1 , wherein the fuel or fuel additive is added to fossil based fuels.

9. The transportation fuel or fuel additive derived by the process according to claim 1 , wherein the fuel or fuel additive is added to jet fuel.

10. The transportation fuel or fuel additive derived by the process according to claim 1 , wherein the fuel or fuel additive is added to the jet fuel at a percentage of up to 50%.

11. The transportation fuel or fuel additive derived by the process according to claim 1 , wherein the fuel or fuel additive is added to diesel fuel.

12. The transportation fuel or fuel additive derived by the process according to claim 1 , wherein the fuel or fuel additive classifies the transportation fuel or fuel additive as a cellulosic biofuel which generates a renewable identification number (RIN) for said transportation fuel or fuel additive.

13. The transportation fuel or fuel additive of claim 12 wherein the RIN is a form of compliance credits under a renewable fuel standard (RFS) program.

14. The transportation fuel or fuel additive of claim 13 wherein the transportation fuel or fuel additive is blended into fossil derived fuels to establish a RIN credit.

Assignments (5)
CHANGE OF NAME Recorded Aug 27, 2024
From: NUVEEN EIC ADMINISTRATION LLC
To: PCL ADMINISTRATION LLC
Reel/Frame 068788/0916 →
AFFIDAVIT OF OWNERSHIP TO CORRECT ERROR MADE IN A PREVIOUSLY RECORDED DOCUMENT THAT ERRONEOUSLY AFFECTS THE IDENTIFIED PATENTS AND APPLICATION(S). Recorded Jan 2, 2024
From: FULCRUM BIOENERGY, INC.
To: FULCRUM BIOENERGY, INC.
Reel/Frame 066179/0612 →
SECURITY INTEREST Recorded Jun 23, 2023
From: FULCRUM BIOENERGY, INC.
To: NUVEEN EIC ADMINISTRATION LLC, AS ADMINISTRATIVE AGENT
Reel/Frame 064048/0126 →
AFFIDAVIT OF OWNERSHIP Recorded Jun 5, 2023
From: FULCRUM BIOENERGY, INC.
To: THERMOCHEM RECOVERY INTERNATIONAL, INC.
Reel/Frame 063860/0316 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jul 11, 2019
From: LUCAS, STEPHEN H.; TIVERIOS, PETER G.; RICH, LEWIS L.
To: FULCRUM BIOENERGY, INC.
Reel/Frame 049727/0295 →
Continuity (9)
Continuation 15791045 · Oct 23, 2017
Continuation 15682368 · Aug 21, 2017
Continuation 15077782 · Mar 22, 2016
Division 14842729 · Sep 1, 2015
Continuation 14799522 · Jul 14, 2015
Continuation In Part 14138635 · Dec 23, 2013
Continuation 13023505 · Feb 8, 2011
Provisional Application 61302516 · Feb 8, 2010
Related Publication 20190345400A1 · Nov 14, 2019
Cited By (6)
US 12,187,969 US 12,203,040 US 12,221,587 US 12,252,655 US 12,480,061 US 12,655,359