IP Library Granted Patent US 12,131,970
Granted Patent B2
US 12,131,970 · App. 16/618,697 · Granted Oct 29, 2024

Liquid resin composition for sealing and electronic component apparatus

Inventors: Hidetoshi Inoue (Tokyo, JP); Takayuki Matsuzaki (Tokyo, JP); Hisato Takahashi (Tokyo, JP); Tsuyoshi Kamimura (Niigata, JP); Haruyuki Yoshii (Niigata, JP)
Assignees: Resonac Corporation; Namics Corporation
H01L23/295C08G59/226C08G59/245C08G59/5073C08K3/36C08K7/18C09K3/1025C08G2190/00C09K2200/0247C09K2200/0647
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Quick Facts
Patent No.
US 12,131,970
App. No.
16/618,697
Granted
Oct 29, 2024
Kind
B2
Abstract

A liquid resin composition for sealing contains an aliphatic epoxy compound (A), an epoxy compound (B) having an aromatic ring in a molecule, a nitrogen-containing heterocyclic compound (C), and an inorganic filler (D), wherein a percentage content of the inorganic filler (D) is 77% by mass or more with respect to a total mass of the composition.

Claims (29)

1. A liquid resin composition for sealing, comprising:

an aliphatic epoxy compound (A),

an epoxy compound (B) having an aromatic ring in a molecule,

a nitrogen-containing heterocyclic compound (C),

a curing agent other than the nitrogen-containing heterocyclic compound (C), and

an inorganic filler (D);

wherein the nitrogen-containing heterocyclic compound (C) is present in an amount within a range of from 2 parts by mass to 12 parts by mass with respect to 100 parts by mass in total of epoxy compounds;

wherein the curing agent other than the nitrogen-containing heterocyclic compound (C) is a liquid acid anhydride, a liquefied phenol, or an aromatic amine, and the curing agent other than the nitrogen-containing heterocyclic compound (C) is present in an amount of less than 0.1 equivalent with respect to 1 equivalent of epoxy compounds in the liquid resin composition; and

wherein the inorganic filler (D) is at least one selected from the group consisting of silicas, calcium carbonate, clay, alumina, silicon nitride, silicon carbide, boron nitride, calcium silicate, potassium titanate, aluminum nitride, beryllia, zirconia, zircon, forsterite, steatite, spinel, mullite, titania, aluminum hydroxide, magnesium hydroxide, zinc borate, and zinc molybdate, and the inorganic filler (D) is present in an amount of at least 77% by mass with respect to a total mass of the composition.

2. The liquid resin composition for sealing according to claim 1 , wherein the aliphatic epoxy compound (A) comprises a compound represented by the following Formula (I):

wherein, in Formula (I), n is an integer from 1 to 15.

3. The liquid resin composition for sealing according to claim 2 , wherein a number-average molecular weight of the compound represented by Formula (I) is from 200 to 10000.

4. The liquid resin composition for sealing according to claim 3 , wherein the epoxy compound (B) having an aromatic ring in a molecule comprises at least one of N,N-diglycidylorthotoluidine or N,N-bis(2,3-epoxypropyl)-4-(2,3-epoxypropoxy)aniline.

5. The liquid resin composition for sealing according to claim 4 , further comprising a coupling agent (E).

6. The liquid resin composition for sealing according to claim 3 , further comprising a coupling agent (E).

7. The liquid resin composition for sealing according to claim 2 , wherein the epoxy compound (B) having an aromatic ring in a molecule comprises at least one of N,N-diglycidylorthotoluidine or N,N-bis(2,3-epoxypropyl)-4-(2,3-epoxypropoxy)aniline.

8. The liquid resin composition for sealing according to claim 7 , further comprising a coupling agent (E).

9. The liquid resin composition for sealing according to claim 2 , further comprising a coupling agent (E).

10. The liquid resin composition for sealing according to claim 1 , wherein a number-average molecular weight of the aliphatic epoxy compound (A) is from 200 to 10000.

11. The liquid resin composition for sealing according to claim 10 , wherein the epoxy compound (B) having an aromatic ring in a molecule comprises at least one of N,N-diglycidylorthotoluidine or N,N-bis(2,3-epoxypropyl)-4-(2,3-epoxypropoxy)aniline.

12. The liquid resin composition for sealing according to claim 11 , further comprising a coupling agent (E).

13. The liquid resin composition for sealing according to claim 10 , further comprising a coupling agent (E).

14. The liquid resin composition for sealing according to claim 1 , wherein the epoxy compound (B) having an aromatic ring in a molecule comprises at least one of N,N-diglycidylorthotoluidine or N,N-bis(2,3-epoxypropyl)-4-(2,3-epoxypropoxy)aniline.

15. The liquid resin composition for sealing according to claim 14 , further comprising a coupling agent (E).

16. The liquid resin composition for sealing according to claim 1 , further comprising a coupling agent (E).

17. The liquid resin composition for sealing according to claim 1 , wherein a percentage content of the aliphatic epoxy compound (A) is from 3% by mass to 40% by mass with respect to the total amount of compounds having an epoxy group, included in the liquid resin composition for sealing.

18. The liquid resin composition for sealing according to claim 17 , wherein the epoxy compound (B) having an aromatic ring in a molecule comprises at least one of N,N-diglycidylorthotoluidine or N,N-bis(2,3-epoxypropyl)-4-(2,3-epoxypropoxy)aniline.

19. The liquid resin composition for sealing according to claim 1 , wherein a percentage content of the aliphatic epoxy compound (A) is from 10% by mass to 30% by mass with respect to the total amount of compounds having an epoxy group, included in the liquid resin composition for sealing.

20. An electronic component apparatus, comprising an element sealed with the liquid resin composition for sealing according to claim 1 .

Assignments (6)
CHANGE OF ADDRESS Recorded Feb 9, 2024
From: RESONAC CORPORATION
To: RESONAC CORPORATION
Reel/Frame 066547/0677 →
CHANGE OF NAME Recorded Mar 10, 2023
From: SHOWA DENKO MATERIALS CO., LTD.
To: RESONAC CORPORATION
Reel/Frame 063052/0423 →
CHANGE OF NAME Recorded Mar 7, 2023
From: SHOWA DENKO MATERIALS CO., LTD.
To: RESONAC CORPORATION
Reel/Frame 062901/0765 →
CHANGE OF NAME Recorded Mar 6, 2023
From: HITACHI CHEMICAL COMPANY, LTD.
To: SHOWA DENKO MATERIALS CO., LTD.
Reel/Frame 062956/0775 →
CHANGE OF NAME Recorded Nov 18, 2022
From: HITACHI CHEMICAL CO., LTD.
To: SHOWA DENKO MATERIALS CO., LTD.
Reel/Frame 061967/0148 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 2, 2019
From: INOUE, HIDETOSHI; MATSUZAKI, TAKAYUKI; TAKAHASHI, HISATO; KAMIMURA, TSUYOSHI; YOSHII, HARUYUKI
To: HITACHI CHEMICAL COMPANY, LTD.; NAMICS CORPORATION
Reel/Frame 051152/0904 →