IP Library › Granted Patent US 6,855,490
Granted Patent B2
US 6,855,490 · App. 09/834,240 · Granted Feb 15, 2005

Method for attaching biological molecules to a glass surface

Assignee: Medical Discovery Partners LLC
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Quick Facts
Patent No.
US 6,855,490
App. No.
09/834,240
Granted
Feb 15, 2005
Kind
B2
Abstract

The invention describes a method for attaching biological molecules, such as proteins, nucleic acids, and carbohydrates to a glass surface. In particular, a covalent attachment method is described wherein a glass surface is first activated with a water-stable form of an isocyanate, termed a protected isocyanate. The protecting group of the isocyanate moiety is displaced by amines, hydroxyl, or carboxyl groups of biological molecules, leading to covalent attachment to the glass surface.

Claims (36)

1. A method for attaching a biological molecule to a glass surface comprising the steps of:

a) providing a silane-treated glass surface having an end-capped amino group;

b) reacting said end-capped amino group with a phosgene equivalent to form a protected isocyanate group; and

c) reacting said protected isocyanate group with a biological molecule,

thereby forming a covalent coupling and attaching said biological molecule to the glass surface.

2. The method of claim 1 further comprising reacting a glass surface with an aminosilane thereby forming the silane-treated glass surface having an end-capped amino group.

3. The method of claim 1 wherein the phosgene equivalent is a carbonyl diimidazole or a ketoxime carbonate.

4. The method of claim 3 wherein the carbonyl diimidazole is 1,1-carbonyldiimidazole.

5. The method of claim 3 wherein the ketoxime carbonate is methyl ethyl ketoxime carbonate.

6. The method of claim 1 wherein the biological molecule is selected from the group consisting of proteins, peptides, nucleic acids and carbohydrates.

7. The method of claim 1 wherein the glass surface is a microscope slide surface.

8. A method for attaching a biological molecule to a glass surface comprising the steps of:

a) providing a silane-treated glass surface having an end-capped amino group;

b) reacting said amino group with a phosgene equivalent to form an end-capped group, said end-capped group including a functional group represented by the following structural formula:

>N—C(O)—N<

or by the following structural formula:

>N—C(O)—O—N<;

and

c) reacting said end-capped group with a biological molecule, thereby forming a covalent coupling and attaching said biological molecule to the glass surface.

9. The method of claim 8 wherein the phosgene equivalent is a carbonyl diimidazole or a ketoxime carbonate.

10. The method of claim 9 wherein the carbonyl diimidazole is 1,1-carbonyldiimidazole.

11. The method of claim 9 wherein the ketoxime carbonate is methyl ethyl ketoxime carbonate.

12. The method of claim 8 wherein said end-capped group is represented by the following structural formula:

13. The method of claim 8 wherein said end-capped group is represented by the following structural formula:

14. A method for attaching a biological molecule to a silane-treated glass surface comprising the steps of:

a) reacting an end-capped amino group on said silane-treated glass surface with a phosgene equivalent to form a protected isocyanate group; and

b) reacting said protected isocyanate group with a biological molecule,

thereby forming a covalent coupling and attaching said biological molecule to said silane-treated glass surface.

15. A method for attaching a biological molecule to a silane-treated glass surface comprising the steps of:

a) reacting an amino group on said silane-treated glass surface with a phosgene equivalent to form an end-capped group, said end-capped group including a functional group represented by the following structural formula:

>N—C(O)—N<

or by the following structural formula:

>N—C(O)—O—N<;

and

b) reacting said end-capped group with a biological molecule, thereby forming a covalent coupling and attaching said biological molecule to said silane-treated glass surface.

16. The method of claim 8 wherein the glass surface is a microscope slide surface.

Assignments (6)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 22, 2008
From: MEDICAL DISCOVERY PARTNERS, LLC
To: LAB VISION CORPORATION
Reel/Frame 021561/0476 →
CONFIRMATORY LICENSE Recorded Jun 24, 2008
From: MEDICAL DISCOVERY PARTNERS, LLC
To: NATIONAL INSTITUTES OF HEALTH (NIH), U.S. DEPT. OF HEALTH AND HUMAN SERVICES (DHHS), U.S. GOVERNMENT
Reel/Frame 021142/0660 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 3, 2004
From: CYTOLOGIX CORPORATION
To: MEDICAL DISCOVERY PARTNERS, LLC
Reel/Frame 015059/0696 →
TERMINATION OF SECURITY AGREEMENT Recorded Aug 22, 2002
From: OXFORD BIOSCIENCE PARTNERS III L.P.
To: CYTOLOGIX CORPORATION
Reel/Frame 013211/0579 →
SECURITY AGREEMENT Recorded Jun 17, 2002
From: CYTOLOGIX CORPORATION
To: OXFORD BIOSCIENCE PARTNERS III L.P.
Reel/Frame 013000/0685 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Apr 12, 2001
From: SOMPURAM, SESHI R.; RAMANATHAN, HALASYA
To: CYTOLOGIX CORPORATION
Reel/Frame 011704/0911 →
Continuity (3)
Continuation 0954985500 · Apr 14, 2000
Continuation In Part 0929135100 · Apr 14, 1999
Related Publication 20030166261A1 · Sep 4, 2003