IP Library Granted Patent US 9,347,006
Granted Patent B2
US 9,347,006 · App. 14/149,274 · Granted May 24, 2016

Method for optimizing catalyst loading for hydrocracking process

Inventors: Omer Refa Koseoglu (Dhahran, SA); Adnan Al-Hajji (Dhahran, SA); Hendrik Muller (Dhahran, SA); Masaru Ushio (Kawasaki, JP); Koji Nakano (Fukuoka, JP)
Assignees: Saudi Arabian Oil Company; JGC Catalysts and Chemicals Ltd.; Japan Cooperation Center, Petroleum
C10G65/12B01J23/882B01J23/883B01J29/084B01J29/166B01J35/0006C10G45/04C10G45/06C10G45/10C10G45/12C10G45/32C10G45/44C10G47/02C10G49/002C10G49/02C10G49/04C10G49/06C10G49/08C10G2300/202
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Quick Facts
Patent No.
US 9,347,006
App. No.
14/149,274
Granted
May 24, 2016
Kind
B2
Abstract

The invention relates to a method for optimizing layered catalytic processes. This is accomplished by testing various catalysts with a compound found in a feedstock to be tested, to determine the facility of the catalyst in hydrogenating, hydrosulfurizing, or hydrodenitrogenating the molecule, and hence the feedstock. In a preferred embodiment, the Double Bond Equivalence of the feedstock and molecule are determined, and catalysts are pre-selected based upon their known ability to work with materials of this DBE value.

Claims (15)

1. A method for optimizing a layered hydrocracking catalytic process, comprising (i) contacting a model compound capable of (a) being hydrocracked as well as at least one of (ii) hydrogenation, hydrosulfurization and hydrodenitrogenation to a plurality of catalysts to determine an optimal catalyst for each of (i) and (ii), (b) following by layering the optimal catalysts for each of (i) and (ii) in a reaction chamber based on their activity reacting with said model compound, and (c) contacting a feedstock to the layered catalysts under condition favoring formation of lower weight hydrocarbon from said hydrocarbon containing feedstock, wherein said model compound boils in the range of 180° C.-520° C. and is selected from the group consisting of methylnaphthalene, dibenzothiophene, an alkylated or naphtalated derivative thereof, a basic nitrogen compound and a carbazole molecule.

2. The method of claim 1 , further comprising determining double bond equivalence (DBE,) of said feedstock, and contacting said model compound to a plurality of catalysts suitable for hydrocracking a substance with a DBE of said feedstock, to determine an optimum hydrocracking catalyst for said feedstock.

3. The method of claim 2 , further comprising contacting said model compound to a second plurality of catalysts suitable for hydrogenerating, hydrodesulfurizing, or hydrodenitrogenating a substance with a DBE value less than said feedstock to determine an optimal, second catalyst.

4. The method of claim 2 , wherein said hydrocarbons contained in said feedstock have a double bond equivalency of 24 or less.

5. The method of claim 2 , wherein said feedstock has a double bond equivalency of 24 or less, and at least one of said catalysts for VGO hydrocracking catalyst.

6. The method of claim 2 , wherein said feedstock has a double bond equivalency of 25 or more, and at least one of said catalysts is a catalyst designed for heavy feedstock.

7. The method of claim 1 , comprising contacting said hydrocarbon containing feedstock to said reaction chamber at a temperature of from 350° C. to 450° C.

8. The method of claim 1 , comprising contacting said hydrocarbon containing feedstock to said reaction chamber at a hydrogen feed rate less than 2500 liters per liter of feedstock.

9. The method of claim 1 , comprising contacting said hydrocarbon containing feedstock to said reaction vessel at a pressure of from 100 bars to 200 bars.

10. The method of claim 1 , wherein at least one of said catalysts contains a metal from Group VI, VII or VIIIB of the periodic table, or is a noble metal.

11. The method of claim 10 , wherein said metal is Co, Ni, W, Mo, Pt, or Pd.

12. The method of claim 1 , wherein at least one of said catalysts contains amorphous alumina, silica-alumina, titanium, Y zeolite, or at least one a transition metal inserted Y zeolite.

13. The method of claim 12 , wherein said transition metal is Zr, Ti, Hf and combination thereof.

14. The method of claim 1 , wherein said molecule is capable of being at least two of hydrogenated, hydrodesulfurized, and Itydrodenitrogenated.

15. The method of claim 1 , wherein said molecule is capable of being hydrogenated, hdrodesulfurized, and hydrodenitrogenated.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jul 14, 2014
From: USHIO, MASARU; NAKANO, KOJI
To: JGC CATALYSTS AND CHEMICALS LTD.; JAPAN COOPERATION CENTER, PETROLEUM
Reel/Frame 033305/0133 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 19, 2014
From: KOSEOGLU, OMER REFA; AL-HAJJI, ADNAN; MULLER, HENDRIK
To: SAUDI ARABIAN OIL COMPANY
Reel/Frame 032469/0475 →
Continuity (2)
Provisional Application 61750152 · Jan 8, 2013
Related Publication 20140190868A1 · Jul 10, 2014