IP Library › Granted Patent US 10,239,811
Granted Patent B2
US 10,239,811 · App. 15/852,719 · Granted Mar 26, 2019

Process for producing reduced coenzyme Q

Inventors: Kento Kanaya (Takasago, JP); Hiroko Okatsu (Takasago, JP)
Assignee: KANEKA CORPORATION
C07C46/00C07C41/26C07C46/08C07C46/10C12P7/66
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Quick Facts
Patent No.
US 10,239,811
App. No.
15/852,719
Granted
Mar 26, 2019
Kind
B2
Abstract

A process for producing reduced coenzyme Q 10 includes removing moisture from an aqueous suspension including a reduced coenzyme Q 10 -containing microbial cell or a disrupted cell thereof such that a de-moisturized substance is obtained and in contact with an oxidizing atmosphere, and that an oxidized coenzyme Q 10 is produced in an amount of 50 mass % or more relative to a total amount of the oxidized and reduced coenzymes Q 10 , and reducing the oxidized coenzyme Q 10 outside a microbial cell such that a reduced coenzyme Q 10 is recovered.

Claims (40)

1. A process for producing reduced coenzyme Q 10 , comprising:

removing moisture from an aqueous suspension comprising a reduced coenzyme Q 10 -containing microbial cell or a disrupted cell thereof such that a de-moisturized substance is obtained and in contact with an oxidizing atmosphere, and that an oxidized coenzyme Q 10 is produced in an amount of 50 mass % or more relative to the total amount of the oxidized and reduced coenzymes Q 10 ; and

reducing the oxidized coenzyme Q 10 outside a microbial cell such that a reduced coenzyme Q 10 is recovered.

2. The process of claim 1 , wherein the aqueous suspension, before the removing of the moisture, includes the reduced coenzyme Q 10 in an amount of not less than 50 mass % relative to the total amount of the oxidized and the reduced coenzymes Q 10 .

3. The process of claim 1 , wherein the de-moisturized substance has a moisture content of not greater than 30 mass % after the removing of the moisture.

4. The process of claim 1 , wherein the aqueous suspension has a pH of greater than 4 before the removing of the moisture.

5. The process of claim 1 , wherein the removing of the moisture comprises drying the aqueous suspension under an oxidizing atmosphere, or

drying the aqueous suspension under an oxidizing atmosphere and preservation for 1 to 30 days under an oxidizing atmosphere.

6. The process of claim 5 , wherein the removing of the moisture is conducted at a temperature of not lower than 50° C.

7. The process of claim 1 , wherein the removing of the moisture is conducted such that the oxidized coenzyme Q 10 is produced in an amount of 80 mass % or more relative to the total amount of the oxidized and the reduced coenzymes Q 10 .

8. The process of claim 1 , further comprising:

extracting the oxidized coenzyme Q 10 produced, before the reducing of the oxidized coenzyme Q 10 ,

wherein the removing of the moisture comprises drying the aqueous suspension under an oxidizing atmosphere.

9. A process for producing oxidized coenzyme Q 10 , comprising:

removing moisture from an aqueous suspension comprising reduced coenzyme Q 10 -containing a microbial cell or a disrupted cell thereof such that a de-moisturized substance is obtained; and

preserving the de-moisturized substance for 1 to 30 days in an oxidizing atmosphere such that an oxidized coenzyme Q 10 is produced.

10. The process of claim 9 , further comprising:

extracting the oxidized coenzyme Q 10 produced;

separating an extract including the oxidized coenzyme Q 10 from the microbial cell or the disrupted cell thereof; and

purifying a separated extract including the oxidized coenzyme Q 10 by at least one of column chromatography and crystallization.

11. The process of claim 10 , further comprising:

oxidizing with an oxidizing agent a residual reduced coenzyme Q 10 included in the separated extract.

12. The process of claim 9 , wherein the de-moisturized substance has a moisture content of not greater than 30 mass % after the removing of the moisture.

13. The process of claim 9 , wherein the aqueous suspension has a pH of greater than 4 before the removing of the moisture.

14. The process of claim 9 , wherein the removing of the moisture comprises drying the aqueous suspension under an oxidizing atmosphere.

15. The process of claim 1 , further comprising, before the reducing of the oxidized coenzyme Q 10 :

extracting the oxidized coenzyme Q 10 produced;

separating an extract including the oxidized coenzyme Q 10 from the microbial cell or the disrupted cell thereof; and

purifying a separated extract including the oxidized coenzyme Q 10 by at least one of column chromatography and crystallization,

wherein the removing of the moisture comprises drying the aqueous suspension under an oxidizing atmosphere.

16. The process of claim 9 , wherein the preserving is for 5 to 20 days.

17. The process of claim 9 , wherein the preserving is for 10 to 18 days.

18. The process of claim 1 , wherein the removing of the moisture comprises drying the aqueous suspension under an oxidizing atmosphere and preservation for 1 to 30 days under an oxidizing atmosphere.

19. The process of claim 1 , wherein the reducing of the oxidized coenzyme Q 10 is conducted such that not less than 98 mass % of reduced coenzyme Q 10 is obtained with respect to the total amount of the oxidized and reduced coenzymes Q 10 .

20. The process of claim 19 , wherein the reducing of the oxidized coenzyme Q 10 is conducted such that not less than 99 mass % of reduced coenzyme Q 10 is obtained with respect to the total amount of the oxidized and reduced coenzymes Q 10 .

21. The process of claim 9 , wherein the preserving of the de-moisturized substance is conducted such that the oxidized coenzyme Q 10 is produced in an amount of 50 mass % or more relative to the total amount of the oxidized and reduced coenzymes Q 10 .

22. A process for producing reduced coenzyme Q 10 , comprising:

producing oxidized coenzyme Q 10 by the process of claim 9 ;

extracting the oxidized coenzyme Q 10 produced; and

reducing the oxidized coenzyme Q 10 outside a microbial cell such that a reduced coenzyme Q 10 is recovered.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 26, 2017
From: KANAYA, KENTO; OKATSU, HIROKO
To: KANEKA CORPORATION
Reel/Frame 044484/0397 →
Priority Claims (1)
JP 2015-125965 · Jun 23, 2015 · national
Continuity (2)
Continuation In Part PCTJP2016068612 · Jun 23, 2016
Related Publication 20180134644A1 · May 17, 2018
Cited By (1)
US 12,226,374