IP Library › Granted Patent US 10,253,273
Granted Patent B2
US 10,253,273 · App. 15/441,668 · Granted Apr 9, 2019

Process to obtain fuel from biomass in fluid catalytic cracking

Inventors: Andrea de Rezende Pinho (Rio de Janeiro, BR); Fabio Leal Mendes (Rio de Janeiro, BR)
Assignee: PETROLEO BRASILEIRO S.A.—PETROBRAS
C10G69/04C10G51/026C10G2300/1014C10G2300/202C10G2400/02Y02P30/20
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Quick Facts
Patent No.
US 10,253,273
App. No.
15/441,668
Granted
Apr 9, 2019
Kind
B2
Abstract

The present invention relates to a process for obtaining fuel from biomass which comprises the introduction of the catalyst ( 3 ) in the base of an cracking section ( 4 ), wherein said catalyst ( 3 ) at high temperature comes in contact with a gas stream of light hydrocarbons rich in hydrogen ( 1 ), wherein the catalyst ( 3 ) and hydrocarbon ( 1 ) then come in contact with a lignocellulosic liquid stream ( 2 ) in the same cracking section ( 4 ), creating the reaction mixture ( 5 ) that, soon after, comes into contact with the main stream containing the traditional fossil load of a FCC ( 6 ) in a second cracking section ( 7 ).

Claims (24)

1. A process to obtain fuels from biomass via fluid catalytic cracking (FCC), comprising:

introducing a gas stream comprising saturated hydrocarbons ( 1 ), a lignocellulosic liquid stream ( 2 ), and a catalyst ( 3 ) into a first reaction section ( 4 ) of a FCC reactor;

contacting the gas stream ( 1 ), the lignocellulosic liquid stream ( 2 ) and the catalyst ( 3 ) in the first reaction section ( 4 ) under first reaction conditions, which comprise a temperature in a range of from 500 to 800° C., to produce a reaction medium ( 5 ); and

contacting the reaction medium ( 5 ) with a main stream comprising a traditional fossil load ( 6 ) in a second reaction section ( 7 ) of the FCC reactor under second reaction conditions to produce reaction products ( 8 ).

2. The process according to claim 1 , characterized by separating the reaction products ( 8 ) obtained in the second reaction section ( 7 ) and subjecting the reaction products ( 8 ) to a hydrotreatment step to obtain high octane fuel.

3. The process according to claim 2 , characterized by the hydrotreatment step employing a temperature between 350° C. and 390° C. and, as a catalyst, a metal oxide totally or partially converted into sulfides (active phase) and supported on y-alumina (y-Al 2 O 3 ).

4. The process according to claim 1 , characterized by the first reaction conditions comprising a temperature in a range of from 500° C. to 700° C., a pressure in a range of from 200 kPa to 400 kPa, a catalyst/biomass ratio in a range of from 10 to 40,and a contact time in a range of from 0.1 to 0.9 seconds.

5. The process according to claim 1 , characterized by the second reaction conditions comprising a speed space in a range of from 200 h−1 to 400 h−1, a contact time in a range of from 1.5 to 3.0 seconds, a temperature in a range of from 500° C. and 620° C. and a catalyst/hydrocarbons ratio in a range of from 5 to 20.

6. The process according to claim 1 , characterized in that the lignocellulosic liquid stream ( 2 ) is derived from the pulp and paper industry.

7. The process according to claim 1 , characterized in that the lignocellulosic liquid stream ( 2 ) is obtained by fast pyrolysis processing units.

8. The process according to claim 1 , characterized in that the biomass corresponds to 0.1 to 10% by weight relative to a total amount of load added to the FCC reactor.

9. The process according to claim 1 , characterized by the traditional fossil load ( 6 ) being a petroleum refinery stream having a hydrogen content of at least 10% by weight based on a total weight of the traditional fossil load ( 6 ).

10. The process according to claim 1 , characterized in that the gas stream ( 1 ) comprises one or more saturated hydrocarbons selected from the group consisting of propane, butane, ethane, pentane and hexane.

11. The process according to claim 10 , characterized in that the stream ( 1 ) corresponds to 0.1 to 10% by weight relative to the total amount load added to the FCC reactor.

12. The process according to claim 1 , characterized in that the catalyst ( 3 ) is a solid acid catalyst.

13. The process according to claim 12 , characterized in that the solid acid catalyst is a zeolitic catalyst.

14. The process according to claim 1 , wherein the lignocellulosic liquid stream ( 2 ) is obtained from a Kraft process.

15. The process according to claim 1 , characterized by the traditional fossil load ( 6 ) having a hydrogen content of at least 10% by weight based on a total weight of the traditional fossil load ( 6 ).

16. The process according to claim 1 , characterized by the first reaction section ( 4 ) of the FCC reactor being located at a base of a riser.

17. A process to obtain fuels from biomass via fluid catalytic cracking (FCC), comprising:

introducing a gas stream comprising saturated hydrocarbons (1), a lignocellulosic liquid stream (2), and a catalyst (3) into a first reaction section (4) of a FCC reactor;

contacting the gas stream (1), the lignocellulosic liquid stream (2) and the catalyst (3) in the first reaction section (4) under first reaction conditions, which comprise a temperature in a range of from 500 to 800° C., to produce a reaction medium (5);

contacting the reaction medium (5) with a main stream comprising a traditional fossil load (6) in a second reaction section (7) of the FCC reactor under second reaction conditions to produce reaction products (8); and

separating the reaction products (8) obtained in the second reaction section (7) and subjecting the reaction products (8) to a hydrotreatment step to obtain gasoline with a Research Octane Number (RON) above 90.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 15, 2018
From: PINHO, ANDREA DE REZENDE; MENDES, FABIO LEAL
To: PETROLEO BRASILEIRO S.A.-PETROBRAS
Reel/Frame 046839/0783 →
Priority Claims (1)
BR 10 2016 003995-9 · Feb 24, 2016 · national
Continuity (1)
Related Publication 20170240824A1 · Aug 24, 2017