IP Library Granted Patent US 10,815,593
Granted Patent B2
US 10,815,593 · App. 13/675,414 · Granted Oct 27, 2020

Viscosity modified formaldehyde-free binder compositions

Inventors: Zhihua Guo (Centennial, CO); Uranchimeg Lester (Littleton, CO); Jawed Asrar (Englewood, CO); Kiarash Alavi Shooshtari (Littleton, CO); Mingfu Zhang (Highlands Ranch, CO)
Assignee: Johns Manville
D04H13/008C08K7/14C08L3/02C08L61/20C08L61/24C08L61/32C09J101/28C09J101/286C09J103/02C09J105/00D04H1/4218D04H1/4242D04H1/587D04H1/64D21H13/40D21H17/20D21H23/48Y10T442/604
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Quick Facts
Patent No.
US 10,815,593
App. No.
13/675,414
Granted
Oct 27, 2020
Kind
B2
Abstract

Viscosity-modified carbohydrate binder compositions are described. The binder compositions may include a carbohydrate, a nitrogen-containing compound, and a thickening agent. The binder compositions may have a Brookfield viscosity of 7 to 50 centipoise at 20° C. The thickening agents may include modified celluloses such as hydroxyethyl cellulose (HEC) and carboxymethyl cellulose (CMC), and polysaccharides such as xanthan gum, guar gum, and starches.

Claims (30)

1. A carbohydrate binder composition comprising a reducing sugar, a nitrogen-containing compound, and a thickening agent, wherein:

the nitrogen-containing compound is a reaction product of urea (H 2 N—CO—NH 2 ) and glyoxal,

the binder composition has a Brookfield viscosity of 7 to 50 centipoise at 20° C. as measured with a Brookfield viscometer using spindle 18 at 60 rpm,

the binder composition is formaldehyde-free and forms a polymerization product, and

the thickening agent has a concentration of 0.03 wt. % to 0.3 wt. % of the binder composition.

2. The carbohydrate binder composition of claim 1 , wherein the reducing sugar is chosen from dextrose, fructose, allose, galactose, xylose, ribose, maltose, cellobiose, and lactose.

3. The carbohydrate binder composition of claim 1 , wherein the reaction product comprises 4,5-dihydroxyimidazolidin-2-one.

4. The carbohydrate binder composition of claim 1 , wherein the binder composition further comprises a reaction product of an organic anhydride and an alkanol amine.

5. The carbohydrate binder composition of claim 1 , wherein the thickening agent comprises a modified cellulose.

6. The carbohydrate binder composition of claim 5 , wherein the modified cellulose is chosen from carboxymethyl cellulose (CMC), and hydroxyethyl cellulose (HEC).

7. The carbohydrate binder composition of claim 1 , wherein the thickening agent comprises a polysaccharide.

8. The carbohydrate binder composition of claim 7 , wherein the polysaccharide is chosen from xanthan gum, guar gum, and starch.

9. The carbohydrate binder composition of claim 1 , wherein the thickening agent comprises acrylic acid.

10. The carbohydrate binder composition of claim 1 , wherein:

the reducing sugar comprises dextrose;

the nitrogen-containing compound is 4,5-dihydroxyimidazolidin-2-one; and

the thickening agent comprises hydroxyethyl cellulose, wherein the hydroxyethyl cellulose has a concentration of 0.05 wt. % to 0.3 wt. % of the binder composition.

11. The carbohydrate binder composition of claim 1 , wherein:

the reducing sugar comprises dextrose;

the nitrogen-containing compound is 4,5-dihydroxyimidazolidin-2-one; and

the thickening agent comprises xanthan gum, wherein the xanthan gum has a concentration of 0.03 wt. % to 0.2 wt. % of the binder composition.

12. A blended carbohydrate binder composition comprising a reducing sugar, a nitrogen-containing compound, and a second binder composition, wherein:

the nitrogen-containing compound is a reaction product of urea (H 2 N—CO—NH 2 ) and glyoxal,

the blended carbohydrate binder composition has a Brookfield viscosity of 7 to 50 centipoise at 20° C. as measured with a Brookfield viscometer using spindle 18 at 60 rpm,

the second binder composition is formaldehyde-free and forms a polymerization product, and

the blended carbohydrate binder composition comprises a thickening agent at a concentration from 0.03 wt. % to 0.3 wt. % of the blended carbohydrate binder composition.

13. The blended carbohydrate binder composition of claim 12 , wherein the second binder composition is selected from the group consisting of a latex binder composition and a solution polymer binder composition.

14. The carbohydrate binder composition of claim 1 , wherein the binder composition is an aqueous solution.

15. The blended carbohydrate binder composition of claim 12 , wherein the second binder composition is a solution polymer binder composition.

16. The carbohydrate binder composition of claim 1 , wherein the molar ratio of the nitrogen-containing compound to the reducing sugar is in a range from 1:4 to 1:10.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 30, 2012
From: GUO, ZHIHUA; LESTER, URANCHIMEG; ASRAR, JAWED; SHOOSHTARI, KIARASH ALAVI; ZHANG, MINGFU
To: JOHNS MANVILLE
Reel/Frame 029380/0163 →
Continuity (1)
Related Publication 20140134909A1 · May 15, 2014
Cited By (3)
US 12,297,342 US 12,343,974 US 12,578,051