IP Library › Granted Patent US 10,882,937
Granted Patent B2
US 10,882,937 · App. 16/312,040 · Granted Jan 5, 2021

Polymer having a small average particle size

Inventors: Attyah Saeed Al-Zhrani (Riyadh, SA); Mohammed Zerfa (Riyadh, SA); Faisal Alhareeki (Riyadh, SA)
Assignee: SABIC GLOBAL TECHNOLOGIES B.V.
C08F220/26C08K5/0016C08L27/06C08L29/04C08F220/282C08F2800/20C08L2201/54C08L2205/14
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Quick Facts
Patent No.
US 10,882,937
App. No.
16/312,040
Granted
Jan 5, 2021
Kind
B2
Abstract

The present invention relates to a polymer comprising: (a) polymeric units derived from vinyl chloride, vinyl acetate, styrene, methyl methacrylate, acrylonitrile, or combinations thereof; and (b) polymeric units derived from one or more compounds according to formula I: wherein: R1 is CH 3 or H; R2 is a moiety comprising 1-20 carbon atoms; and n is an integer from 1-10; wherein the polymer has an average particle size of 10-80 μm expressed as D 50 determined in accordance with ISO 9276-2 (2014); and a porosity of ≤0.20 ml/g as determined as the quantity of di(2-ethylhexyl)phthalate in ml absorbed by 1 g of polymer upon subjecting the polymer at 23° C. to vacuum, submerging in di(2-ethylhexyl)phthalate for 10 min, and subsequently centrifuging at 2000 rpm for 45 min. Such polymer may be used as viscosity reducing agent in PVC plastisol compositions.

Claims (44)

1. A polymer comprising:

(a) polymeric units derived from vinyl chloride, vinyl acetate, styrene, methyl methacrylate, acrylonitrile, or combinations thereof; and

(b) polymeric units derived from one or more compounds according to formula I:

formula I

wherein:

R1 is CH 3 or H;

R2 is a moiety comprising 1-20 carbon atoms; and

n is an integer from 1-10;

wherein the polymer has

an average particle size of 10-80 μm expressed as D 50 determined in accordance with ISO 9276-2 (2014); and

a porosity of ≤0.20 ml/g as determined as the quantity of di(2-ethylhexyl)phthalate in ml absorbed by 1 g of polymer upon subjecting the polymer at 23° C. to vacuum, submerging in di(2-ethylhexyl)phthalate for 10 min, and subsequently centrifuging at 2000 rpm for 45 min.

2. A polymer according to claim 1 , wherein R2 is a moiety comprising at least one hydroxyl moiety.

3. A polymer according to claim 1 , wherein the polymer comprises ≥500 ppm of units (b), with regard to the total weight of the polymer.

4. A polymer according to claim 1 , wherein the polymeric units (a) are derived from vinyl chloride.

5. A polymer according to claim 1 , wherein the polymeric units (b) are derived from one or more compounds selected from glycerol (meth)acrylate, 2-hydroxyethyl (meth)acrylate, 2-hydroxypropyl (meth)acrylate, tetritol mono(meth)acrylate, xylitol mono(meth)acrylate, sorbitol mono(meth)acrylate, polyethyleneglycol (meth)acrylate, polypropyleneglycol (meth)acrylate, or combinations thereof.

6. A polymer according to claim 1 , wherein the polymeric units (b) are derived from glycerol (meth)acrylate.

7. A polymer according to claim 1 , wherein the polymer is produced in a suspension polymerisation process.

8. A polymer according to claim 7 , wherein the suspension polymerisation process comprises reacting a reaction mixture comprising:

a quantity of a reaction medium;

a quantity of vinyl chloride, vinyl acetate, styrene, methyl methacrylate, acrylonitrile, or combinations thereof; and

a quantity of one or more compounds according to formula I:

formula I

wherein:

R1 is CH 3 or H;

R2 is a moiety comprising 1-20 carbon atoms; and

n is an integer from 1-10.

9. A polymer according to claim 7 , wherein the suspension polymerisation process comprises reacting a reaction mixture comprising:

a quantity of a reaction medium;

a quantity of vinyl chloride, vinyl acetate, styrene, methyl methacrylate, acrylonitrile, or combinations thereof; and

a quantity of one or more compounds selected from glycerol (meth)acrylate, 2-hydroxyethyl (meth)acrylate, 2-hydroxypropyl (meth)acrylate, tetritol mono(meth)acrylate, xylitol mono(meth)acrylate, sorbitol mono(meth)acrylate, polyethyleneglycol (meth)acrylate, polypropyleneglycol (meth)acrylate, or combinations thereof.

10. A polymer according to claim 7 , wherein the suspension polymerisation process comprises reacting a reaction mixture comprising:

a quantity of a reaction medium;

a quantity of vinyl chloride, vinyl acetate, styrene, methyl methacrylate, acrylonitrile, or combinations thereof; and

a quantity of ≥500 ppm by weight, with regard to the weight of the quantity of vinyl chloride, vinyl acetate, styrene, methyl methacrylate, acrylonitrile, or combinations thereof, of a one or more compounds selected from glycerol (meth)acrylate, 2-hydroxyethyl (meth)acrylate, 2-hydroxypropyl (meth)acrylate, tetritol mono(meth)acrylate, xylitol mono(meth)acrylate, sorbitol mono(meth)acrylate, polyethyleneglycol (meth)acrylate, polypropyleneglycol (meth)acrylate, or combinations thereof.

11. A polymer according to claim 7 , wherein the suspension polymerisation process comprises reacting a reaction mixture comprising:

a quantity of a reaction medium;

a quantity of vinyl chloride; and

a quantity of ≥500 ppm by weight, with regard to the weight of the quantity of vinyl chloride, of a glycerol (meth)acrylate.

12. A method of reducing a viscosity of a plastisol composition, comprising combining the polymer according to claim 1 with the plastisol compositions.

13. A plastisol composition comprising a polymer according to any claim 1 and a polyvinyl chloride polymer having an average particle size of 1-20 μm.

14. A plastisol composition comprising 10.0-30.0 wt % of the polymer according to claim 1 with regard to the total weight of the plastisol composition.

15. A plastisol composition according claim 14 further comprising a polyvinyl chloride polymer having an average particle size of 1-20 μm.

16. A plastisol composition according claim 14 , wherein the polymeric units (a) are derived from vinyl chloride, and the polymeric units (b) are derived from one or more compounds selected from glycerol (meth)acrylate, 2-hydroxyethyl (meth)acrylate, 2-hydroxypropyl (meth)acrylate, tetritol mono(meth)acrylate, xylitol mono(meth)acrylate, sorbitol mono(meth)acrylate, polyethyleneglycol (meth)acrylate, polypropyleneglycol (meth)acrylate, or combinations thereof.

17. A polymer according to claim 16 , wherein the polymeric units (b) are derived from glycerol (meth)acrylate.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 21, 2018
From: AL-ZHRANI, ATTYAH SAEED; ZERFA, MOHAMMED; ALHAREEKI, FAISAL
To: SABIC GLOBAL TECHNOLOGIES B.V.
Reel/Frame 047838/0452 →
Priority Claims (2)
EP 16177049 · Jun 30, 2016 · regional
EP 16177051 · Jun 30, 2016 · regional
Continuity (1)
Related Publication 20190375868A1 · Dec 12, 2019