IP Library › Granted Patent US 10,954,215
Granted Patent B2
US 10,954,215 · App. 16/469,075 · Granted Mar 23, 2021

Compounds as modulators of ROR gamma

Inventors: Robert Owen Hughes (Newtown, CT); Xiang Li (New Milford, CT); Peter Allen Nemoto (Southbury, CT); Lana Louise Smith Keenan (Ridgefield, CT); Lifen Wu (New Milford, CT); Zhaoming Xiong (Ridgefield, CT)
Assignee: Boehringer Ingelheim International GmbH
C07D401/14A61P37/02C07D207/16C07D401/04C07D401/10C07D401/12C07D403/04C07D409/04C07D413/04C07D417/04C07D491/107
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Quick Facts
Patent No.
US 10,954,215
App. No.
16/469,075
Granted
Mar 23, 2021
Kind
B2
Abstract

The present invention encompasses compounds of the formula (I) wherein the variables are defined herein which are suitable for the modulation of RORγ and the treatment of diseases related to the modulation of RORγ. The present invention also encompasses processes of making compounds of formula (I) and pharmaceutical preparations containing them.

Claims (43)

1. A compound of formula I

wherein:

R 2′ is H; and

R 1 and R 2 are independently selected from benzothiophen-3-yl, isoquinolinyl, [1,2,4]-oxadiazolyl, phenyl, pyrazolyl, pyridyl, thiazolyl, 1H-[1,2,4]triazolyl and 2H-[1,2,3]triazolyl, wherein when R 1 is phenyl, then R 2 is other than phenyl;

or

R 2 and R 2′ form a spiro benzofuran-3-one ring; and

R 1 is selected from C 1-6 alkyl, benzothiophen-3-yl, isoquinolinyl, [],2,41-oxadiazolyl, phenyl, pyrazolyl, pyridyl, thiazolyl, 1H-[1,2,4]triazolyl and 2H-[1,2,3]triazolyl;

wherein R 1 and R 2 are each optionally substituted by one to two groups independently selected from C 1-4 alkyl, C 3-5 cycloalkyl, cyclopropylmethyl, —CF 3 , halogen, —OCF 3 , —OH, -OCH 3 and phenyl;

R 3 is selected from phenyl, pyridyl and pyrimidinyl;

wherein R 3 is substituted with a group selected from —SO 2 C 1-3 alkyl and —SO 2 NHC 1-3 alkyl;

or an enantiomer or a salt thereof.

2. The compound of formula (I) according to claim 1 , wherein R 2′ is H; and

R 1 and R 2 are independently selected from benzothiophen-3-yl, isoquinolin-5-yl, [1,2,4]-oxadiazol-5-yl, phenyl, 4- and 5-pyrazolyl, 2- and 3-pyridyl, thiazol-2-yl, 1H-[1,2,4]triazol-5-yl and 2H-[1,2,3]triazol-5-yl, wherein when R 1 is phenyl, then R 2 is other than phenyl;

or

R 2 and R 2′ may form a spiro benzofuran-3-one ring; and

R 1 is selected from isopropyl, benzothiophen-3-yl, isoquinolin-5-yl, [1,2,41]-oxadiazol-5-yl, phenyl, 4- and 5-pyrazolyl, 2- and 3-pyridyl, thiazol-2-yl, 1H-[1,2,4]triazol-5-yl and 2H-[1,2,3]triazol-5-yl;

R 1 and R 2 are each optionally substituted by one to two groups independently selected from C 1-4 alkyl, C 3-5 cycloalkyl, cyclopropylmethyl, —CF 3 , Cl, —OCF 3 , —OH, -OCH 3 and phenyl;

R 3 is selected from phenyl, 2- and 3-pyridyl and 2-pyrimidinyl;

wherein R 3 is substituted with a group selected from —SO 2 CH 2 CH 3 and —SO 2 NHCH 3 ;

or an enantiomer or a salt thereof.

3. The compound of formula (I) according to claim 1 , wherein R 2′ is H; and

R 1 and R 2 are independently selected from benzothiophen-3-yl, isoquinolin-5-yl, phenyl, 4- and 5-pyrazolyl, 2-pyridyl and 1H-[1,2,4]triazol-5-yl, wherein when R 1 is phenyl, then R 2 other than phenyl;

or

R 2 and R 2′ may form a spiro benzofuran-3-one ring; and

R 1 is selected from isopropyl, benzothiophen-3-yl, isoquinolin-5-yl, phenyl, 4- and 5-pyrazolyl, 2-pyridyl and 1H-[1,2,4]triazol-5-yl;

wherein R 1 and R 2 are each optionally substituted by one to two groups independently selected from C 1-4 alkyl, C 3-5 cycloalkyl, cyclopropylmethyl, —CF 3 , Cl, —OCF 3 ,—OH and -OCH 3 ;

R 3 is selected from phenyl and 2-pyridyl;

wherein R 3 is substituted with a group selected from —SO 2 CH 2 CH 3 and —SO 2 NHCH 3 ;

or an enantiomer or a salt thereof.

4. The compound of formula (I) according to claim 1 , wherein R 2′ is H; and

R 1 and R 2 are independently selected from isopropyl, phenyl, 4- and 5-pyrazolyl and 2-pyridyl, wherein when R 1 is phenyl, then R 2 is other than phenyl;

or

R 2 and R 2′ may form a spiro benzofuran-3-one ring; and

R 1 is selected from isopropyl and phenyl;

wherein R 1 and R 2 are each optionally substituted by one to two groups independently selected from methyl, isopropyl, tert-butyl, cyclopropyl, cyclopentyl, —CF 3 , Cl and —OCF3;

R 3 is selected from phenyl and 2-pyridyl;

wherein R 3 is substituted with a group selected from —SO 2 CH 2 CH 3 and —SO 2 NHCH 3 ;

or an enantiomer or a salt thereof.

5. The compound according to claim 1 selected from the group consisting of

the enantiomers thereof and the pharmaceutically acceptable salts thereof.

6. A pharmaceutical composition comprising a compound according to claim 1 and a pharmaceutically acceptable excipient or carrier.

7. A method for treating an autoimmune disease or allergic disorder in a patient comprising administering to said patient a therapeutically effective amount of a compound of formula (I) according to claim 1 , or a pharmaceutically acceptable salt thereof.

8. The method according to claim 7 , wherein the autoimmune disease or allergic disorder is selected from rheumatoid arthritis, psoriasis, systemic lupus erythromatosis, lupus nephritis, scleroderma, asthma, allergic rhinitis, allergic eczema, multiple sclerosis, juvenile rheumatoid arthritis, juvenile idiopathic arthritis, type I diabetes, inflammatory bowel disease, graft versus host disease, psoriatic arthritis, reactive arthritis, ankylosing spondylitis, Crohn's disease, ulcerative colitis, uveitis and non-radiographic spondyloarthropathy.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 18, 2021
From: BOEHRINGER INGELHEIM PHARMACEUTICALS, INC.
To: BOEHRINGER INGELHEIM INTERNATIONAL GMBH
Reel/Frame 055319/0124 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 12, 2021
From: WU, LIFEN; XIONG, ZHAOMING; LI, XIANG; SMITH-KEENAN, LANA LOUISE; HUGHES, ROBERT OWEN; NEMOTO, PETER ALLEN
To: BOEHRINGER INGELHEIM PHARMACEUTICALS, INC.
Reel/Frame 055293/0533 →
Continuity (2)
Provisional Application 62433268 · Dec 13, 2016
Related Publication 20200071298A1 · Mar 5, 2020
Cited By (2)
US 12,275,742 US 12,630,560