IP Library Granted Patent US 11,040,908
Granted Patent B2
US 11,040,908 · App. 15/752,717 · Granted Jun 22, 2021

Glass fiber production method

Inventors: Takashi Nonaka (Fukushima, JP); Norio Hirayama (Fukushima, JP); Kazuaki Minami (Fukushima, JP); Yosuke Nukui (Fukushima, JP)
Assignee: Nitto Boseki Co., Ltd.
C03C13/00C03B37/075C03C3/087C03C3/091C03B2203/02
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Quick Facts
Patent No.
US 11,040,908
App. No.
15/752,717
Granted
Jun 22, 2021
Kind
B2
Abstract

Provided is a method for producing glass fiber, capable of stably performing the spinning of glass fibers without mixing of red crystals in glass fibers. When glass fibers are formed by discharging, from a nozzle tip, a molten glass obtained by melting glass raw materials mixed so as to give a glass composition including, when melted, in relation to the total amount thereof, SiO 2 in a range from 57.0 to 62.0% by mass, Al 2 O 3 in a range from 15.0 to 20.0% by mass, MgO in a range from 7.5 to 12.0% by mass, and CaO in a range from 9.0 to 16.5% by mass, and having a total content of SiO 2 , Al 2 O 3 , MgO and CaO of 98.0% by mass or more, the glass composition includes B 2 O 3 , Li 2 O, or B 2 O 3 and Li 2 O as an additive or additives capable of suppressing the generation of red crystals.

Claims (12)

1. A method for producing glass fiber, when glass fibers are formed by discharging, from a nozzle tip, a molten glass obtained by melting glass raw materials mixed so as to give a glass composition comprising, when melted, in relation to the total amount thereof, SiO 2 in a range from 57.0 to 58.8% by mass, Al 2 O 3 in a range from 18.0 to 20.0% by mass, MgO in a range from 7.5 to 12.0% by mass, and CaO in a range from 9.0 to 12.5% by mass, and having a total content of SiO 2 , Al 2 O 3 , MgO and CaO of 98.0% by mass or more, the glass composition comprises B 2 O 3 , or a combination of B 2 O 3 and Li 2 O, as an additive or additives capable of suppressing generation of red crystals,

wherein a ratio of the product between a content of the additive or additives capable of suppressing generation of red crystals (% by mass) and the content (% by mass) of CaO to the content (% by mass) of Al 2 O 3 is in a range from 0.25 to 1.00.

2. The method for producing glass fiber according to claim 1 , wherein the glass fibers each have a modified cross sectional shape in which a ratio (major axis/minor axis) of the major axis to the minor axis of the cross sectional shape falls within a range from 2.0 to 6.0.

3. The method for producing glass fiber according to claim 1 , wherein the glass fibers each have a modified cross sectional shape in which a fiber diameter defined as a diameter when a cross-sectional area is converted to a perfect circle, falls within a range from 10 to 30 μm.

4. The method for producing glass fiber according to claim 1 , wherein the glass fibers have perfect circular cross sections, and fiber diameters falling within a range of 3 μm or more to less than 10 μm.

5. The method for producing glass fiber according to claim 1 , wherein the glass raw materials mixed so as to give the glass composition are melted by using a melting furnace in which a portion in contact with the molten glass is formed of bricks containing chromium oxide.

6. The method for producing glass fiber according to claim 1 , wherein the glass composition comprises B 2 O 3 as the additive capable of suppressing the generation of red crystals, in a content of 0.5 to 1.5% by mass in relation to the total amount of the glass composition.

7. The method for producing glass fiber according to claim 1 , wherein the glass composition comprises B 2 O 3 and Li 2 O as the additives capable of suppressing the generation of red crystals, in a content of 0.5 to 1.5% by mass in relation to the total amount of the glass composition.

8. The method for producing glass fiber according to claim 1 , wherein in the glass composition, an 1000-poise temperature thereof is a temperature falling within a range from 1300 to 1370° C., a liquid phase temperature thereof is a temperature falling within a range from 1200 to 1270° C., and a working temperature range thereof is 50° C. or higher.

9. The method for producing glass fiber according to claim 1 , wherein the glass fibers each have a modified cross sectional shape in which a ratio (major axis/minor axis) of the major axis to the minor axis of the cross sectional shape falls within a range from 2.0 to 6.0, and a fiber diameter defined as a diameter when a cross-sectional area is converted to a perfect circle, falls within a range from 10 to 30 μm.

10. The method for producing glass fiber according to claim 1 , wherein the glass composition comprises CaO in a range of 10.3 to 12.5% by mass.

11. The method for producing glass fiber according to claim 1 , wherein the glass composition comprises MgO in a range of 8.8 to 12.0% by mass.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 14, 2018
From: NONAKA, TAKASHI; HIRAYAMA, NORIO; MINAMI, KAZUAKI; NUKUI, YOSUKE
To: NITTO BOSEKI CO., LTD.
Reel/Frame 044929/0490 →
Continuity (1)
Related Publication 20180237335A1 · Aug 23, 2018
Cited By (1)
US 12,600,665