IP Library Granted Patent US 11,186,753
Granted Patent B2
US 11,186,753 · App. 16/334,107 · Granted Nov 30, 2021

Shrinkable thermoplastic vulcanizate and method and article

Inventors: Wanli Wang (Katy, TX); Michael W. Bednarik (Fairlawn, OH); Peite Bao (Houston, TX); Yi Ping Ni (Shanghai, CN); Ying Ying Sun (Houston, TX)
Assignee: ExxonMobil Chemical Patents Inc.
C09J123/16B29C61/003B29C61/025B29C65/68C08J3/226C08L23/16C09J5/06B29K2021/003C08L2203/30C08L2205/025C08L2205/035C08L2310/00C09J2423/10C09J2423/16C09J2461/00C09J2491/00
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Quick Facts
Patent No.
US 11,186,753
App. No.
16/334,107
Granted
Nov 30, 2021
Kind
B2
Abstract

A process of heat shrinking an article is provided. The process includes shaping a thermoplastic vulcanizate (TPV) into an article, the TPV having: a partially vulcanized rubber dispersed in a continuous thermoplastic phase, wherein more than 5 wt % of the rubber is extractable in boiling xylene, and wherein the thermoplastic phase comprises a thermoplastic resin having a Tm>110° C. and a propylene-based elastomer (PBE) having a Tm<110° C.; and heating the article to a temperature between about 100° C. and 250° C. to shrink the article.

Claims (30)

1. A process of heat shrinking an article, the process comprising:

shaping a thermoplastic vulcanizate (TPV) into an article, the TPV comprising:

a partially vulcanized rubber dispersed in a continuous thermoplastic phase,

wherein more than 5 wt % of the rubber is extractable in boiling xylene, and

wherein the thermoplastic phase comprises a thermoplastic resin having a Tm>110° C. and a propylene-based elastomer (PBE) having a Tm<110° C.; and

heating the article to a temperature between about 100° C. and 250° C. to shrink the article.

2. A process of heat shrinking an article, the method comprising:

shaping a thermoplastic vulcanizate (TPV) into an article, the TPV comprising:

an at least partially vulcanized rubber dispersed in a continuous thermoplastic phase,

wherein the thermoplastic phase comprises a thermoplastic resin having a Tm>110° C. and a propylene-based elastomer (PBE) having a TM<110° C.; and

heating the article to a temperature between about 100° C. and 250° C. to shrink the article.

3. A process according to claim 1 , wherein the heating shrinks the article in a machine direction (MD) by at least 20%.

4. A process according to claim 3 , wherein the article is a tube, and the MD is an axial direction of the tube.

5. A process according to claim 1 , wherein the heating shrinks the article in a cross direction (CD) by no more than 5%.

6. A process according to claim 5 , wherein the article is a tube, and the cross direction is a radial or circumferential direction of the tube.

7. A process according to claim 1 , wherein the thermoplastic resin has a Tm>130° C.

8. A process according to claim 1 , wherein the PBE has a Tm<100° C., and further wherein the PBE comprises 70 to 95 wt % units derived from propylene and 5 to 30 wt % units derived from ethylene, said wt % s on the basis of the monomer-derived content of the PBE.

9. The process according to claim 1 , wherein heating the article comprises heating the article to a temperature between about 110° C. and 150° C.

10. A process according to claim 1 , wherein the heating the article comprises heating the article to the temperature for 120 seconds.

11. A process according to claim 1 , wherein more than 10 wt % of the rubber is extractable in boiling xylene.

12. A process according to claim 1 , wherein more than 15 wt % of the rubber is extractable in boiling xylene.

13. A process according to claim 1 , wherein the shaping comprises molding or extruding the TPV.

14. A process of securing two parts by heat shrinking an article, the process comprising:

disposing the article at least partially about each of the two parts to be secured, and heating the article to a temperature between 100° C. and 250° C. so as to shrink the article, thereby securing the two parts;

wherein the article comprises a TPV, the TPV comprising:

a partially vulcanized rubber dispersed in a continuous thermoplastic phase,

wherein more than 5 wt % of the rubber is extractable in boiling xylene, and

wherein the thermoplastic phase comprises a thermoplastic resin having a Tm>110° C. and a propylene-based elastomer (PBE) having a Tm<110° C.

15. A process according to claim 1 , wherein the thermoplastic resin comprises a random propylene, ethylene, butene terpolymer.

16. A process according to claim 1 , wherein the rubber is an ethylene propylene diene rubber (EPDM).

Assignments (3)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 25, 2022
From: EXXONMOBIL CHEMICAL PATENTS INC.
To: SANTOPRENE PRODUCTION PENSACOLA LLC
Reel/Frame 059248/0456 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 25, 2022
From: SANTOPRENE PRODUCTION PENSACOLA LLC
To: CELANESE INTERNATIONAL CORPORATION
Reel/Frame 059248/0673 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jul 16, 2019
From: WANG, WANLI; BEDNARIK, MICHAEL W.; BAO, PEITE; NI, YI PING; SUN, YING YING
To: EXXONMOBIL CHEMICAL PATENTS INC.
Reel/Frame 049760/0757 →
Continuity (2)
Provisional Application 62399080 · Sep 23, 2016
Related Publication 20190256746A1 · Aug 22, 2019