IP Library Granted Patent US 11,383,985
Granted Patent B2
US 11,383,985 · App. 16/099,797 · Granted Jul 12, 2022

Hybrid silica gel made of porous silica particles

Inventors: Charles Joseph Rimsky (Greenwood, SC); Jaswinder Kumar Sharma (Oak Ridge, TN); Mahabir Singh Bhandari (Oak Ridge, TN); Panagiotis George Datskos (Knoxville, TN); Georgios Polyzos (Oak Ridge, TN)
Assignee: VKR HOLDING A/S
C01B33/155B32B5/16B32B17/068B32B17/069C01B33/14C04B26/32C04B28/003B32B2307/304B32B2307/412C01P2004/64C01P2006/17C01P2006/37C04B2111/28
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Quick Facts
Patent No.
US 11,383,985
App. No.
16/099,797
Granted
Jul 12, 2022
Kind
B2
Abstract

Compositions, methods, and articles of manufacture relating to a transparent/translucent insulating material formed by a hybrid silica gel composition made of porous silica particles joined with each other by silane crosslinking through a three dimensional silica network. In one embodiment, the hybrid silica gel includes small porous silica particles, and is made by a process that avoids energy intensive techniques.

Claims (21)

1. An insulating material, comprising:

a hybrid silica gel including a silica network of porous silica particles joined by silica cross-linkers, wherein the silica cross-linkers comprise at least partially hydrolyzed silica precursors, and wherein said hybrid silica gel has a thermal conductivity of about 0.15 W/m.K or less.

2. The material of claim 1 , wherein each of said porous silica particles has a diameter that is less than 100 nm.

3. The material of claim 2 , wherein each of said porous silica particles has a diameter that is between about 60 nm and about 100 nm.

4. The material of claim 2 , wherein each of said porous silica particles has a diameter that is no more than about 60 nm.

5. The material of claim 1 , wherein said hybrid silica gel has a thermal conductivity of about ≤0.032 W/m.K.

6. The material of claim 1 , wherein said hybrid silica gel has a thermal conductivity of about 0.15 W/m.K to about 0.022 W/m.K.

7. The material of claim 1 , wherein said silica cross-linkers include partially hydrolyzed TEOS.

8. An insulating material, comprising:

a hybrid silica gel including a silica network of porous silica particles joined by silica cross-linkers, wherein the silica cross-linkers comprise at least partially hydrolyzed silica precursors, wherein said hybrid silica gel has a visible transmittance of about 50% or more.

9. The material of claim 1 , wherein each of said porous silica particles has a small grain of about 60 nm.

10. The material of claim 1 , wherein said porous silica particles include pores that are ≤20 nm.

11. The material of claim 1 , wherein said porous silica particles include micropores and macropores, wherein said micropores are between about 1 nm to about 6 nm, and said macropores are between about 50 nm to about 100 nm.

12. The material of claim 11 , wherein said micropores are about 3.5 nm.

13. An insulating material, comprising:

a hybrid silica gel including a silica network of porous silica particles joined by silica cross-linkers, wherein the silica cross-linkers comprise at least partially hydrolyzed silica precursors, wherein said hybrid silica gel has a thermal resistance of about ≥6 hr·ft 2 ·° F./Btu.

14. The material of claim 8 , wherein said hybrid silica gel has a visible transmittance of about 99% or more.

15. A fenestration system, comprising:

a first pane of glass;

a second pane of glass, said first and second panes of glass defining an enclosed chamber;

a transparent insulating material contained within said enclosed chamber, said transparent insulating material comprising: a hybrid silica gel including a silica network of porous silica particles joined by silica cross-linkers, wherein the silica cross-linkers comprise at least partially hydrolyzed silica precursors, and wherein said hybrid silica gel has a thermal conductivity of about 0.15 W/m.K or less.

Assignments (3)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 8, 2022
From: SHARMA, JASWINDER K.; PANAGIOTIS, PANAGIOTIS G.; POLYZOS, GEORGIOS
To: UT-BATTELLE, LLC
Reel/Frame 060132/0005 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 8, 2022
From: BHANDARI, MAHABIR S.
To: UT-BATTELLE, LLC
Reel/Frame 060133/0189 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 20, 2018
From: RIMSKY, CHARLES JOSEPH
To: VKR HOLDING A/S
Reel/Frame 047557/0020 →
Continuity (2)
Provisional Application 62340630 · May 24, 2016
Related Publication 20190152789A1 · May 23, 2019