IP Library › Granted Patent US 11,498,850
Granted Patent B2
US 11,498,850 · App. 16/912,039 · Granted Nov 15, 2022

Solid electrolyte material and battery

Inventors: Tetsuya Asano (Nara, JP); Akihiro Sakai (Nara, JP); Yusuke Nishio (Osaka, JP); Masashi Sakaida (Hyogo, JP); Akinobu Miyazaki (Osaka, JP); Shinya Hasegawa (Kyoto, JP)
Assignee: PANASONIC INTELLECTUAL PROPERTY MANAGEMENT CO., LTD.
C01F17/36H01M10/0525H01M10/0562H01M2300/008
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Quick Facts
Patent No.
US 11,498,850
App. No.
16/912,039
Granted
Nov 15, 2022
Kind
B2
Abstract

A solid electrolyte material contains Li; Y; at least one selected from the group consisting of Mg, Ca, Sr, Ba, Zn, Zr, Nb, and Ta; and at least one selected from the group consisting of Cl, Br, and I. An X-ray diffraction pattern of the solid electrolyte material obtained using Cu—Kα radiation as an X-ray source includes peaks in a range of diffraction angles 2θ of 30° or more and 33° or less, in a range of diffraction angles 2θ of 39° or more and 43° or less, and in a range of diffraction angles 2θ of 47° or more and 51° or less.

Claims (37)

1. A solid electrolyte material comprising:

Li;

Y;

at least one selected from the group consisting of Mg, Ca, Sr, Ba, Zn, Zr, Nb, and Ta; and

at least one selected from the group consisting of Cl, Br, and I,

wherein an X-ray diffraction pattern of the solid electrolyte material obtained using Cu—Kα radiation as an X-ray source includes peaks in a range of diffraction angles 2θ of 30° or more and 33° or less, in a range of diffraction angles 2θ of 39° or more and 43° or less, and in a range of diffraction angles 2θ of 47° or more and 51° or less.

2. The solid electrolyte material according to claim 1 , wherein the X-ray diffraction pattern further includes a peak in a range of diffraction angles 2θ of 15° or more and 18° or less.

3. The solid electrolyte material according to claim 1 , wherein

the solid electrolyte material contains a sublattice of the at least one selected from the group consisting of Cl, Br, and I, and

the sublattice has a hexagonal closest packed structure or a distorted hexagonal closest packed structure.

4. A battery comprising:

the solid electrolyte material according to claim 1 ;

a positive electrode;

a negative electrode; and

an electrolyte layer disposed between the positive electrode and the negative electrode,

wherein at least one selected from the group consisting of the positive electrode, the negative electrode, and the electrolyte layer contains the solid electrolyte material.

5. A solid electrolyte material comprising:

Li;

Y;

at least one selected from the group consisting of Mg, Ca, Sr, Ba, Zn, Zr, Nb, and Ta; and

at least one selected from the group consisting of Cl, Br, and I, wherein

a first converted pattern, which is obtained by measuring an X-ray diffraction pattern of the solid electrolyte material by using Cu—Kα radiation as an X-ray source and converting the X-ray diffraction pattern such that a horizontal axis represents q instead of diffraction angle 2θ,

includes a reference peak in a range of q of 2.109 Å −1 or more and 2.315 Å −1 or less,

q=4π sin θ/λ where λ is a wavelength of the Cu—Kα radiation,

a second converted pattern, which is obtained by converting the X-ray diffraction pattern such that the horizontal axis represents q/q 0 instead of diffraction angle 2θ,

includes peaks in a range of q/q 0 of 1.28 or more and 1.30 or less and in a range of q/q 0 of 1.51 or more and 1.54 or less, and

q 0 is a value of q corresponding to the reference peak in the first conversion pattern.

6. The solid electrolyte material according to claim 5 , wherein the second conversion pattern includes a peak in a range of q/q 0 of 0.50 or more and 0.52 or less.

7. The solid electrolyte material according to claim 5 , wherein

the solid electrolyte material contains a sublattice of the at least one selected from the group consisting of Cl, Br, and I, and

the sublattice has a hexagonal closest packed structure or a distorted hexagonal closest packed structure.

8. A battery comprising:

the solid electrolyte material according to claim 5 ;

a positive electrode;

a negative electrode; and

an electrolyte layer disposed between the positive electrode and the negative electrode,

wherein at least one selected from the group consisting of the positive electrode, the negative electrode, and the electrolyte layer contains the solid electrolyte material.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 18, 2020
From: ASANO, TETSUYA; SAKAI, AKIHIRO; NISHIO, YUSUKE; SAKAIDA, MASASHI; MIYAZAKI, AKINOBU; HASEGAWA, SHINYA
To: PANASONIC INTELLECTUAL PROPERTY MANAGEMENT CO., LTD.
Reel/Frame 053810/0234 →
Priority Claims (1)
JP JP2018-000427 · Jan 5, 2018 · national
Continuity (2)
Continuation PCTJP2018046260 · Dec 17, 2018
Related Publication 20200328462A1 · Oct 15, 2020