IP Library Granted Patent US 11,559,782
Granted Patent B2
US 11,559,782 · App. 16/650,949 · Granted Jan 24, 2023

Reactive media

Inventors: Donald A. Luke (Valrico, FL); Timothy M. Luke (Valrico, FL)
Assignee: Phosphorus Free Water Solutions, LLC
B01J20/043B01J20/041B01J20/12B01J20/3078C02F1/288C04B35/18C04B35/22C04B35/62695
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Quick Facts
Patent No.
US 11,559,782
App. No.
16/650,949
Granted
Jan 24, 2023
Kind
B2
Abstract

Various embodiments of the present invention relate to reactive media including calcium. A reactive media includes a vitrified calcium silicate comprising reactive calcium. Various embodiments of the reactive media described herein are useful for removal of anionic impurities such as phosphate from water.

Claims (48)

1. A method of using a reactive media, the method comprising:

contacting water comprising an anionic material with the reactive media to form a solid calcium salt, wherein the reactive media comprises a vitrified reactive media starting material mixture, the reactive media starting material mixture comprising an organic material comprising peat, wherein the reactive media comprises

a ceramic; and

a reactive calcium available to form a solid calcium salt with the anionic material.

2. The method of claim 1 , wherein the ceramic comprises a calcium silicate, an iron silicate, an aluminum silicate, an other silicate, or a combination thereof.

3. The method of claim 1 , wherein the reactive calcium as CaO is about 14 wt % to about 18 wt % of the reactive media.

4. The method of claim 1 , wherein the reactive calcium is comprised in a calcium material that is a calcium salt, an inorganic calcium compound, or a combination thereof.

5. The method of claim 4 , wherein the calcium material reacts with the anionic material to form the solid calcium salt at a pH of about 9 to about 14.

6. The method of claim 4 , wherein the calcium material is CaO, Ca(OH) 2 , or a combination thereof.

7. The method of claim 4 , wherein the anionic material comprises an anionic impurity, wherein the calcium material reacts with the anionic impurity to form the solid calcium salt.

8. The method of claim 1 , wherein about 0.01 wt % to about 30 wt % of the reactive media is magnesium.

9. The method of claim 1 , wherein the reactive media comprises:

the ceramic that is about 80 wt % to about 99 wt % of the reactive media; and

the reactive calcium that is available to form a solid calcium salt at pH of about 9 to about 14 with phosphate or carbonate in aqueous solution, wherein the reactive calcium as CaO is about 14 wt % to about 18 wt % of the reactive media, wherein the reactive calcium is in the form of a water-soluble salt or inorganic compound including the reactive calcium.

10. The method of claim 9 , wherein during the contacting of the water comprising the anionic material with the reactive media the water comprising the anionic material has a pH of about 9 to about 14.

11. The method of claim 1 , wherein the method further comprises:

heating the reactive media starting material mixture, to provide the reactive media.

12. The method of claim 1 , wherein the reactive media starting material comprises a clay source, a calcium source, a magnesium source, and the organic material, wherein optionally the calcium source and the magnesium source are the same.

13. The method of claim 1 , wherein the reactive media starting material comprises a non-clumping clay, CaO, doloinitic limestone, the peat, and water.

14. The method of claim 11 , wherein the temperature used during formation of the reactive media from the reactive media starting material does not exceed about 1,070° C.

15. The method of claim 1 , wherein the method further comprises:

heating a reactive media starting material mixture comprising about 83% to about 90 mol % Si relative to a total amount of Si and Ca in the reactive media starting material mixture to a temperature that does not exceed about 1,070° C., to at least partially vitrify the reactive media starting material and provide the reactive media.

16. The method of claim 1 , wherein the method further comprises:

heating a reactive media starting material mixture comprising a non-clumping clay, dolomitic limestone, CaO, and the peat, to at least partially vitrify the reactive media starting material and provide the reactive media.

17. The method of claim 1 , wherein the method further comprises:

heating a reactive media starting material mixture to at least partially vitrify the reactive media starting material and provide the reactive media, wherein

about 50 wt % to about 80 wt % of the reactive media starting material mixture is a non-clumping clay,

about 5 wt % to about 20 wt % of the reactive media starting material mixture is dolomitic limestone, such that about 0.1 wt % to about 5 wt % of the reactive media starting material is magnesium,

about 0.1 wt % to about 10 wt % of the reactive media starting material mixture is CaCO 3 ,

about 0.01 wt % to about 5 wt % of the reactive media starting material mixture is CaO,

about 1 wt % to about 20 wt % of the reactive media starting material mixture is the peat, and

about 0 wt % to about 30 wt % of the reactive media starting material mixture is water.

18. The method of claim 1 , wherein the method further comprises:

heating a reactive media starting material mixture to at least partially vitrify the reactive media starting material and provide the reactive media, wherein

about 50 wt % to about 80 wt % of the reactive media starting material mixture is a non-clumping clay,

about 1 wt % to about 30 wt % of the reactive media starting material mixture is dolomite,

about 0.1 wt % to about 10 wt % of the reactive media starting material mixture is CaCO 3 ,

about 0.01 wt % to about 5 wt % of the reactive media starting material mixture is CaO,

about 1 wt % to about 20 wt % of the reactive media starting material mixture is the peat, and

about 0 wt % to about 30 wt % of the reactive media starting material mixture is water.

19. A method of using a reactive media, the method comprising:

contacting water comprising an anionic material with the reactive media to form a solid calcium salt, wherein the reactive media comprises a vitrified reactive media starting material mixture, the reactive media starting material mixture comprising a non-clumping clay, CaO, dolomitic limestone, peat, and water, wherein the reactive media comprises

a ceramic; and

a reactive calcium available to form a solid calcium salt with the anionic material.

20. A method of using a reactive media; the method comprising:

contacting water comprising an anionic material with the reactive media to form a solid calcium salt, wherein the reactive media comprises a vitrified reactive media starting material mixture, the reactive media starting material mixture comprises about 83% to about 90 mol % Si relative to a total amount of Si and Ca in the reactive media starting material mixture, wherein the reactive media comprises

a ceramic; and

a reactive calcium available to form a solid calcium salt with the anionic material.

Assignments (2)
CHANGE OF NAME Recorded May 30, 2023
From: PHOSPHORUS FREE WATER SOLUTIONS, LLC
To: NUQUATIC, LLC
Reel/Frame 063801/0518 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Apr 30, 2020
From: LUKE, DONALD A; LUKE, TIMOTHY M
To: PHOSPHORUS FREE WATER SOLUTIONS, LLC
Reel/Frame 052532/0630 →
Continuity (2)
Provisional Application 62566858 · Oct 2, 2017
Related Publication 20200290012A1 · Sep 17, 2020