IP Library › Granted Patent US 11,559,839
Granted Patent B2
US 11,559,839 · App. 16/481,141 · Granted Jan 24, 2023

Method and apparatus for producing nanoscale materials

Inventors: Davide Mariotti (Belfast, GB); Paul Maguire (Belfast, GB)
Assignee: University of Ulster
B22F9/24B22F1/05B22F1/054B22F1/056B22F1/0545B22F2301/255B22F2304/10B22F2999/00B82Y30/00C01P2004/64H05H2245/50
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Quick Facts
Patent No.
US 11,559,839
App. No.
16/481,141
Granted
Jan 24, 2023
Kind
B2
Abstract

A method of producing nanoscale materials comprising the steps of entraining liquid droplets containing at least one nanoparticle precursor within a gaseous stream, and passing said gaseous stream containing said liquid droplets through a non-thermal equilibrium plasma whereby said plasma interacts with said at least one nanoparticle precursor to produce nanoparticles within said droplets without substantial evaporation of the droplets and conveying the thus produced nanoparticles within said gaseous stream downstream of said plasma.

Claims (20)

1. A method of producing nanoscale materials comprising the steps of:

entraining, within a gaseous stream, liquid droplets comprising a liquid carrier, said droplets containing at least one nanoparticle precursor;

passing said gaseous stream, containing said liquid droplets, through a non-thermal equilibrium plasma, whereby said plasma interacts with said at least one nanoparticle precursor to produce nanoparticles within said droplets without substantial evaporation of the droplets; and

conveying the thus produced nanoparticles within said gaseous stream downstream of said plasma.

2. The method of claim 1 , wherein said nanoparticles are conveyed within said gaseous stream for direct use.

3. The method of claim 1 , wherein the temperature of the gaseous stream when exposed to the plasma does not exceed 100° C.

4. The method of claim 1 , wherein said droplets have a diameter within the range of 1 μm to 100 μm.

5. The method of claim 1 , wherein said droplets have a diameter within the range 1 μm to 60 μm.

6. The method of claim 1 , wherein said droplets have a diameter within the range 10 μm to 20 μm.

7. The method of claim 1 , wherein the flow rate of said gaseous stream is configured to provide a droplet velocity of between 0.01 m/s and 30 m/s.

8. The method of claim 1 , wherein the flow rate of said gaseous stream is configured to provide a droplet velocity of between 0.1 m/s and 2 m/s.

9. The method of claim 1 , wherein the average droplet volume is approximately one picolitre.

10. The method of claim 1 wherein the exposure time of each droplet to the plasma is approximately 120 microseconds.

11. The method of claim 1 , wherein the liquid carrier is water.

12. The method of claim 1 , wherein the nanoparticle precursor is a metal salt.

13. The method of claim 12 , wherein the nanoparticle precursor is a gold salt.

14. The method of claim 13 , wherein the nanoparticle precursor comprises HAuCl 4 .

15. The method of claim 1 , wherein said gaseous stream is constrained to flow within a passage having a diameter of between 0.5 mm and 10 mm.

16. The method of claim 1 , wherein said gaseous stream is constrained to flow within a passage having a diameter of approximately 2 mm.

17. The method of claim 1 , wherein said droplets are injected into said gaseous stream using a nebuliser, atomiser or piezoelectric based droplet generator.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 27, 2019
From: MARIOTTI, DAVIDE; MAGUIRE, PAUL
To: UNIVERSITY OF ULSTER
Reel/Frame 050185/0407 →
Priority Claims (1)
GB 1701292 · Jan 26, 2017 · national
Continuity (1)
Related Publication 20190358708A1 · Nov 28, 2019