IP Library Granted Patent US 11,613,553
Granted Patent B2
US 11,613,553 · App. 17/198,829 · Granted Mar 28, 2023

Methods of preparing 1′-cyano nucleosides

Inventors: Pavel R. Badalov (Edmonton, CA); Stacy Bremner (Edmonton, CA); Matthew R. Chin (Danvers, MA); Detian Gao (Edmonton, CA); Nolan Griggs (San Mateo, CA); Lars V. Heumann (Redwood City, CA); Chiajen Lai (Livermore, CA); Robert R. Milburn (Belmont, CA); Sankar Mohan (Edmonton, CA); Sean T. Neville (San Mateo, CA); Bing Shi (Redwood City, CA); Andrew C. Stevens (Edmonton, CA); Nicholas A. J. Uhlig (Edmonton, CA); Tiago Vieira (Edmonton, CA); Todd A. Wenderski (Hayward, CA)
Assignee: Gilead Sciences, Inc.
C07H19/23C07H1/00
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Quick Facts
Patent No.
US 11,613,553
App. No.
17/198,829
Granted
Mar 28, 2023
Kind
B2
Abstract

The present disclosure generally describes methods of preparing 1′-cyano nucleosides, such as a compound of Formula (I). For example, the compound of Formula (I) can be prepared from a compound of Formula (II-a) in a flow reactor.

Claims (32)

1. A method of preparing a compound of Formula (I):

the method comprising:

(a) adding a first input mixture to a first flow reactor, wherein the first input mixture comprises a Lewis acid, a Bronsted acid, and a compound of Formula (II-a):

wherein the first flow reactor provides a first output mixture; and

(b) adding a second input mixture to a second flow reactor, wherein the second input mixture comprises the first output mixture and a cyanating agent; wherein the second flow reactor provides a second output mixture comprising the compound of Formula (I).

2. The method of claim 1 , further comprising a solvent.

3. The method of claim 2 , wherein the solvent is dichloromethane, chloroform, dichloroethane, or chlorobenzene, or a combination thereof.

4. The method of claim 1 , wherein the Lewis acid is trimethylsilyl trifluoromethanesulfonate (TMSOTf), trimethylsilyl chloride (TMSCl), trimethylsilyl iodide (TMSI), trimethylsilyl bromide (TMSBr), tert-butyldimethylsilyl chloride (TBSCI), tert-butyldimethylsilyl bromide (TB SBr), tert-butyldimethylsilyl iodide (TBSI), triethylsilyl chloride (TESCl), triethylsilyl bromide (TESBr), triethylsilyl iodide (TESI), tert-butyldimethylsilyl trifluoromethanesulfonate (TBSOTf), or triethylsilyl trifluoromethanesulfonate (TESOTf).

5. The method of claim 1 , wherein the Bronsted acid is trifluoroacetic acid (TFA), trifluoromethanesulfonic acid, 4-fluorobenzoic acid, pivalic acid, hydrogen tetrafluoroborate (HBF 4 ), nitric acid, 4-chlorobenzoic acid, pentafluorophenol, or hydrogen hexafluorophosphate (HPF 6 ).

6. The method of claim 1 , wherein the cyanating agent is trimethylsilyl cyanide (TMSCN), tert-butyldimethylsilyl cyanide (TBSCN), triethylsilyl cyanide (TESCN), tetrabutylammonium cyanide, tetramethylammonium cyanide, or tetraethylammonium cyanide.

7. The method of claim 2 , wherein the Lewis acid is trifluoromethanesulfonate (TMSOTf), the Bronsted acid is trifluoroacetic acid, the solvent is dichloromethane, and the cyanating agent is trimethylsilyl cyanide (TMSCN).

8. The method of claim 1 , wherein the first flow reactor and the second flow reactor are both maintained at a temperature of about −30° C.

9. The method of claim 1 , further comprising:

(c) adding a third input mixture to a third reactor, wherein the third input mixture comprises trimethylsilyl chloride (TMSCl), isopropylmagnesium chloride (iPrMgCl), phenylmagnesium chloride (PhMgCl), tetrahydrofuran (THF), and a compound of Formula (IV):

wherein the third reactor provides a third output mixture; and

(d) adding a fourth input mixture to a fourth reactor, wherein the fourth input mixture comprises the third output mixture, neodymium chloride (NdCl 3 ), tetra-n-butylammonium chloride (nBu 4 NCl), and a compound of Formula (III):

wherein the fourth reactor provides a fourth output mixture comprising the compound of Formula (II-a).

10. The method of claim 1 , further comprising:

(c) adding a third input mixture to a third reactor, wherein the third input mixture comprises trimethylsilyl chloride (TMSCl), isopropylmagnesium chloride (iPrMgCl), phenylmagnesium chloride (PhMgCl), tetrahydrofuran (THF), and a compound of Formula (IV):

wherein the third reactor provides a third output mixture; and

(d) adding a fourth input mixture to a fourth reactor, wherein the fourth input mixture comprises the third output mixture, cerium chloride (CeCl 3 ), tetra-n-butylammonium bromide (nBu 4 NBr), and a compound of Formula (III):

wherein the fourth reactor provides a fourth output mixture comprising the compound of Formula (II-a).

11. The method of claim 1 , further comprising:

(c) adding a third input mixture to a third reactor, wherein the third input mixture comprises trimethylsilyl chloride (TMSCl), isopropylmagnesium chloride (iPrMgCl), phenylmagnesium chloride (PhMgCl), tetrahydrofuran (THF), and a compound of Formula (IV):

wherein the third reactor provides a third output mixture; and

(d) adding a fourth input mixture to a fourth reactor, wherein the fourth input mixture comprises the third output mixture, neodymium chloride tetrahydrofuran solvate (NdCl 3 .THF), tetra-n-butylammonium bromide (nBu 4 NBr), and a compound of Formula (III):

wherein the fourth reactor provides a fourth output mixture comprising the compound of Formula (II-a).

12. The method of claim 1 , further comprising:

(c) adding a third input mixture to a third reactor, wherein the third input mixture comprises trimethylsilyl chloride (TMSCl), isopropylmagnesium chloride (iPrMgCl), phenylmagnesium chloride (PhMgCl), tetrahydrofuran (THF), and a compound of Formula (IV):

wherein the third reactor provides a third output mixture; and

(d) adding a fourth input mixture to a fourth reactor, wherein the fourth input mixture comprises the third output mixture, neodymium chloride hexahydrate (NdCl 3 .6H 2 O), trimethyl orthoformate, tetra-n-butylammonium bromide (nBu 4 NBr), and a compound of Formula (III):

wherein the fourth reactor provides a fourth output mixture comprising the compound of Formula (II-a).

Assignments (3)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 24, 2021
From: BADALOV, PAVEL R.; GAO, DETIAN; HEUMANN, LARS V.; STEVENS, ANDREW C.; VIEIRA, TIAGO
To: GILEAD SCIENCES, INC.
Reel/Frame 056325/0331 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 24, 2021
From: NEVILLE, SEAN T.; SHI, BING
To: GILEAD SCIENCES, INC.
Reel/Frame 056325/0367 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 24, 2021
From: BREMNER, STACY; CHIN, MATTHEW R.; GRIGGS, NOLAN; LAI, CHIAJEN; MILBURN, ROBERT R.; MOHAN, SANKAR; UHLIG, NICHOLAS A.J.; WENDERSKI, TODD A.
To: GILEAD SCIENCES, INC.
Reel/Frame 056339/0327 →
Continuity (2)
Provisional Application 62988661 · Mar 12, 2020
Related Publication 20210309689A1 · Oct 7, 2021
Cited By (6)
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