IP Library › Granted Patent US 11,733,192
Granted Patent B2
US 11,733,192 · App. 16/574,012 · Granted Aug 22, 2023

Switchable single-walled carbon nanotube-polymer composites for CO

Inventors: Timothy Swager (Newton, MA); Bora Yoon (Cambridge, MA); Gary Walsh (Cambridge, MA)
Assignee: Massachusetts Institute of Technology
G01N27/126C08F226/06C08K3/041G01N27/127G01N33/004C08K2201/001C08K2201/011
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Quick Facts
Patent No.
US 11,733,192
App. No.
16/574,012
Granted
Aug 22, 2023
Kind
B2
Abstract

A sensor for carbon dioxide can include an amidine functional group.

Claims (26)

1. A composition comprising:

a polymer including a pyridyl amino side chain and an alkylazide side chain;

a conductive material associated with the polymer.

2. The composition of claim 1 , wherein the conductive material includes a carbon nanotube, a conductive polymer, an inorganic semiconductor, a metal oxide, a carbon fiber, a carbon particle, graphite, graphene, carbon paste, metal particles, conducting ink, or combinations thereof.

3. The composition of claim 1 , wherein the polymer is a copolymer of an amine-containing monomer and an alkylazide monomer.

4. The composition of claim 1 wherein the polymer is a copolymer of vinyl pyridine and alkylazido vinyl benzene.

5. A sensor for detecting carbon dioxide comprising:

a substrate; and

a composition of claim 1 on the substrate.

6. The sensor of claim 5 , wherein the amidine-functional polymer is immobilized on a surface of the substrate.

7. The sensor of claim 5 , wherein the carbon conductive material includes a carbon nanotube.

8. The sensor of claim 5 , wherein the amidine-functional polymer is a random copolymer.

9. The sensor of claim 5 , wherein the amidine-functional polymer is a copolymer of an amine-containing monomer and an amidine-functional monomer.

10. The sensor of claim 9 , wherein the amine-containing monomer is a vinyl pyridine.

11. The sensor of claim 10 , wherein the vinyl pyridine is quaternized.

12. A method of detecting carbon dioxide comprising:

exposing a composition of claim 1 to a sample; and

measuring the conductivity change of the composition.

13. The method of claim 12 , wherein the amidine-functional polymer is immobilized on a surface of a substrate.

14. A method of preparing a sensor for detecting an analyte comprising:

linking a composition of claim 1 to a substrate;

quaternizing the amino side chain; and

functionalizing the alkylazide side chain.

15. The method of claim 14 , wherein functionalizing the alkylazide side chain includes introducing an amidine-functional group to the side chain.

16. A composition comprising a polymer including amino side chain and an alkylazide side chain, and a conductive material associated with the polymer wherein the polymer is a copolymer of an amine-containing monomer and an alkylazide monomer and wherein the amine-containing monomer is a vinyl pyridine.

17. A composition comprising a polymer including amino side chain and an alkylazide side chain, and a conductive material associated with the polymer wherein the polymer is a copolymer of an amine-containing monomer and an alkylazide monomer and wherein the alkylazide monomer is an alkylazido vinyl benzene.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 29, 2023
From: YOON, BORA
To: MASSACHUSETTS INSTITUTE OF TECHNOLOGY
Reel/Frame 064112/0164 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 27, 2023
From: WALSH, GARY F.
To: THE GOVERNMENT OF THE UNITED STATES, AS REPRESENTED BY THE SECRETARY OF THE ARMY
Reel/Frame 064068/0005 →
Continuity (2)
Provisional Application 62732541 · Sep 17, 2018
Related Publication 20200088668A1 · Mar 19, 2020