IP Library › Granted Patent US 11,851,519
Granted Patent B2
US 11,851,519 · App. 16/637,601 · Granted Dec 26, 2023

Method for producing purified polytetrafluoroethylene aqueous dispersion liquid, method for producing modified polytetrafluoroethylene powder, method for producing polytetrafluoroethylene molded body, and composition

Inventors: Takahiro Taira (Osaka, JP); Kazuhiro Mishima (Osaka, JP); Chiaki Okui (Osaka, JP); Tadao Hayashi (Osaka, JP); Hirotoshi Yoshida (Osaka, JP); Yuuji Tanaka (Osaka, JP); Masayoshi Miyamoto (Osaka, JP); Taku Yamanaka (Osaka, JP); Taketo Kato (Osaka, JP)
Assignee: DAIKIN INDUSTRIES, LTD.
C08F6/06C08F6/16C08F6/24
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Quick Facts
Patent No.
US 11,851,519
App. No.
16/637,601
Granted
Dec 26, 2023
Kind
B2
Abstract

A method for producing an aqueous dispersion of purified polytetrafluoroethylene, the method including: removing or reducing a compound represented by Formula (1) or (2) below from an aqueous dispersion of polytetrafluoroethylene obtained using a hydrocarbon surfactant: (H—(CF 2 ) m —COO) p M 1 ; or  Formula (1): (H—(CF 2 ) n —SO 3 ) q M 2 .  Formula (2): Also disclosed is a composition containing polytetrafluoroethylene substantially free from a compound represented by Formula (3) below and a molded body including the composition: (H—(CF 2 ) 8 —SO 3 ) q M 2 .  Formula (3):

Claims (17)

1. A method for producing powder of refined polytetrafluoroethylene, the method comprising: removing or reducing a compound represented by Formula (1) or (2) below from polytetrafluoroethylene powder obtained by a production method including performing emulsion polymerization of tetrafluoroethylene in an aqueous medium in the presence of a hydrocarbon surfactant to thereby generate the compound represented by Formula (1) or (2):

(H—(CF 2 ) m —COO) p M 1   Formula (1):

wherein m is 3 to 19, M 1 is H, a metal atom, NR 5 4 (where R 5 s may be the same as or different from each other and are each H or an organic group having 1 to 10 carbon atoms), an imidazolium optionally having a substituent, a pyridinium optionally having a substituent, or a phosphonium optionally having a substituent, and p is 1 or 2; or

(H—(CF 2 ) n —SO 3 ) q M 2   Formula (2):

wherein n is 4 to 20, M 2 is H, a metal atom, NR 5 4 (where R 5 s may be the same as or different from each other and are each H or an organic group having 1 to 10 carbon atoms), an imidazolium optionally having a substituent, a pyridinium optionally having a substituent, or a phosphonium optionally having a substituent, and q is 1 or 2.

2. The method for producing powder of refined polytetrafluoroethylene according to claim 1 , wherein the removal or reduction of a compound represented by Formula (1) or (2) above comprises heating the polytetrafluoroethylene powder obtained using the hydrocarbon surfactant at a temperature of 160° C. or more.

3. A method for producing a molded body of polytetrafluoroethylene, the method comprising:

a step (1a) of mixing a polytetrafluoroethylene powder that is produced using a hydrocarbon surfactant by a production method including performing emulsion polymerization of tetrafluoroethylene in an aqueous medium in the presence of a hydrocarbon surfactant to thereby generate the compound represented by Formula (1) or (2) with an extrusion aid,

a step (1b) of subjecting the mixture thus obtained to paste extrusion molding,

a step (1c) of drying the extrudate obtained by the extrusion molding, and

a step (1d) of obtaining a molded body by firing the extrudate after drying, said method further comprising

removing or reducing a compound from any of the polytetrafluoroethylene powder, the mixture, the extrudate or the molded body represented by Formula (1) or (2) below:

(H—(CF 2 ) m —COO) p M 1   Formula (1):

wherein m is 3 to 19, M 1 is H, a metal atom, NR 5 4 (where R 5 s m a y be the same as or different from each other and are each H or an organic group having 1 to 10 carbon atoms), an imidazolium optionally having a substituent, a pyridinium optionally having a substituent, or a phosphonium optionally having a substituent, and p is 1 or 2; or

(H—(CF 2 ) n —SO 3 ) q M 2   Formula (2):

wherein n is 4 to 20, M 2 is H, a metal atom, NR 5 4 (where R 5 s may be the same as or different from each other and are each H or an organic group having 1 to 10 carbon atoms), an imidazolium optionally having a substituent, a pyridinium optionally having a substituent, or a phosphonium optionally having a substituent, and q is 1 or 2.

4. The method for producing the molded body of polytetrafluoroethylene according to claim 3 , wherein the removal or reduction of a compound represented by Formula (1) or (2) above comprises heating at a temperature of 160° C. or more.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 10, 2020
From: TAIRA, TAKAHIRO; MISHIMA, KAZUHIRO; OKUI, CHIAKI; HAYASHI, TADAO; YOSHIDA, HIROTOSHI; TANAKA, YUUJI; MIYAMOTO, MASAYOSHI; YAMANAKA, TAKU; KATO, TAKETO
To: DAIKIN INDUSTRIES, LTD.
Reel/Frame 051771/0054 →
Priority Claims (2)
JP 2017-248553 · Dec 25, 2017 · national
JP 2018-020460 · Feb 7, 2018 · national
Continuity (2)
Provisional Application 62543499 · Aug 10, 2017
Related Publication 20200255551A1 · Aug 13, 2020