IP Library › Granted Patent US 11,950,507
Granted Patent B2
US 11,950,507 · App. 17/108,448 · Granted Apr 2, 2024

Organic electroluminescence device

Inventors: Huiqing Pang (Beijing, CN); Ru Jia (Beijing, CN); Zhihao Cui (Beijing, CN); Xiao Chen (Beijing, CN); Chuanjun Xia (Beijing, CN); Chi Yuen Raymond Kwong (Beijing, CN); Jing Wang (Beijing, CN)
Assignee: BEIJING SUMMER SPROUT TECHNOLOGY CO., LTD.
H10K85/6572H10K85/631H10K50/155
View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 11,950,507
App. No.
17/108,448
Granted
Apr 2, 2024
Kind
B2
Abstract

Disclosed is an organic electroluminescence device. The organic electroluminescence device has an organic layer having a specific combination in which a hole transporting material is doped with a p-type conductive doped material. The organic electroluminescence device can provide better device performance, such as lifetime improvement and voltage reduction.

Claims (8196)

1. An organic electroluminescence device, comprising:

an anode,

a cathode,

a light-emitting layer disposed between the anode and the cathode, and

a first organic layer disposed between the anode and the light-emitting layer,

wherein the first organic layer comprises a compound of Formula 1 and a compound of Formula 2;

wherein, in Formula 1,

X and Y are, at each occurrence identically or differently, selected from NR′, CR″R′″, O, S or Se;

Z 1 and Z 2 are, at each occurrence identically or differently, selected from O, S or Se;

R, R′, R″ and R″' are, at each occurrence identically or differently, selected from a group consisting of: hydrogen, deuterium, halogen, a nitroso group, a nitro group, an acyl group, a carbonyl group, a carboxylic acid group, an ester group, a cyano group, an isocyano group, SCN, OCN, SF 5 , a boryl group, a sulfinyl group, a sulfonyl group, a phosphoroso group, a substituted or unsubstituted alkyl group having 1 to 20 carbon atoms, a substituted or unsubstituted cycloalkyl group having 3 to 20 ring carbon atoms, a substituted or unsubstituted heteroalkyl group having 1 to 20 carbon atoms, a substituted or unsubstituted arylalkyl group having 7 to 30 carbon atoms, a substituted or unsubstituted alkoxy group having 1 to 20 carbon atoms, a substituted or unsubstituted aryloxy group having 6 to 30 carbon atoms, a substituted or unsubstituted alkenyl group having 2 to 20 carbon atoms, a substituted or unsubstituted alkynyl group having 2 to 20 carbon atoms, a substituted or unsubstituted aryl group having 6 to 30 carbon atoms, a substituted or unsubstituted heteroaryl group having 3 to 30 carbon atoms, a substituted or unsubstituted alkylsilyl group having 3 to 20 carbon atoms, a substituted or unsubstituted arylsilyl group having 6 to 20 carbon atoms, and combinations thereof;

each R is identical or different, and at least one of R, R′, R″ and R′″ is a group having at least one electron-withdrawing group; and

in Formula 1, adjacent substituents are optionally joined to form a ring;

wherein, in Formula 2,

X 1 to X 8 are, at each occurrence identically or differently, selected from CR 1 or N;

L is, at each occurrence identically or differently, selected from a substituted or unsubstituted arylene group having 6 to 30 carbon atoms, a substituted or unsubstituted heteroarylene group having 3 to 30 carbon atoms, or combinations thereof;

Ar 1 and Ar 2 are, at each occurrence identically or differently, selected from a substituted or unsubstituted aryl group having 6 to 30 carbon atoms or a substituted or unsubstituted heteroaryl group having 3 to 30 carbon atoms;

R 1 is, at each occurrence identically or differently, selected from a group consisting of:

hydrogen, deuterium, halogen, a substituted or unsubstituted alkyl group having 1 to 20 carbon atoms, a substituted or unsubstituted cycloalkyl group having 3 to 20 ring carbon atoms, a substituted or unsubstituted heteroalkyl group having 1 to 20 carbon atoms, a substituted or unsubstituted arylalkyl group having 7 to 30 carbon atoms, a substituted or unsubstituted alkoxy group having 1 to 20 carbon atoms, a substituted or unsubstituted aryloxy group having 6 to 30 carbon atoms, a substituted or unsubstituted alkenyl group having 2 to 20 carbon atoms, a substituted or unsubstituted aryl group having 6 to 30 carbon atoms, a substituted or unsubstituted heteroaryl group having 3 to 30 carbon atoms, a substituted or unsubstituted alkylsilyl group having 3 to 20 carbon atoms, a substituted or unsubstituted arylsilyl group having 6 to 20 carbon atoms, a substituted or unsubstituted amino group having 0 to 20 carbon atoms, an acyl group, a carbonyl group, a carboxylic acid group, an ester group, a nitrile group, an isonitrile group, a sulfanyl group, a sulfinyl group, a sulfonyl group, a phosphino group, and combinations thereof; and

in Formula 2, adjacent substituents are optionally joined to form a ring.

2. The organic electroluminescence device according to claim 1 , wherein X and Y are, at each occurrence identically or differently, selected from CR″R′″ or NR′, and R′, R″ and R′″ are a group having at least one electron-withdrawing group; optionally, R, R′, R″ and R′″ are a group having at least one electron-withdrawing group.

3. The organic electroluminescence device according to claim 1 , wherein X and Y are, at each occurrence identically or differently, selected from O, S or Se, and at least one of R is a group having at least one electron-withdrawing group; optionally, all of R are groups having at least one electron-withdrawing group.

4. The organic electroluminescence device according to claim 1 , wherein the Hammett constant of the electron-withdrawing group is greater than or equal to 0.05, optionally is greater than or equal to 0.3, and optionally is greater than or equal to 0.5.

5. The organic electroluminescence device according to claim 1 , wherein the electron-withdrawing group is selected from a group consisting of: halogen, a nitroso group, a nitro group, an acyl group, a carbonyl group, a carboxylic acid group, an ester group, a cyano group, an isocyano group, SCN, OCN, SF 5 , a boryl group, a sulfinyl group, a sulfonyl group, a phosphoroso group, an aza-aromatic ring group, and any one of the following groups substituted by one or more of halogen, a nitroso group, a nitro group, an acyl group, a carbonyl group, a carboxylic acid group, an ester group, a cyano group, an isocyano group, SCN, OCN, SF 5 , a boryl group, a sulfinyl group, a sulfonyl group, a phosphoroso group, and an aza-aromatic ring group: an alkyl group having 1 to 20 carbon atoms, a cycloalkyl group having 3 to 20 ring carbon atoms, a heteroalkyl group having 1 to 20 carbon atoms, an arylalkyl group having 7 to 30 carbon atoms, an alkoxy group having 1 to 20 carbon atoms, an aryloxy group having 6 to 30 carbon atoms, an alkenyl group having 2 to 20 carbon atoms, an alkynyl group having 2 to 20 carbon atoms, an aryl group having 6 to 30 carbon atoms, a heteroaryl group having 3 to 30 carbon atoms, an alkylsilyl group having 3 to 20 carbon atoms, an arylsilyl group having 6 to 20 carbon atoms, and combinations thereof;

optionally, the electron-withdrawing group is selected from a group consisting of: F, CF 3 , OCF 3 , SF 5 , SO 2 CF 3 , a cyano group, an isocyano group, SCN, OCN, a pyrimidinyl group, a triazinyl group, and combinations thereof.

6. The organic electroluminescence device according to claim 1 , wherein X and Y are, at each occurrence identically or differently, selected from a group consisting of the following structures:

wherein R 2 is, at each occurrence identically or differently, selected from a group consisting of: hydrogen, deuterium, halogen, a nitroso group, a nitro group, an acyl group, a carbonyl group, a carboxylic acid group, an ester group, a cyano group, an isocyano group, SCN, OCN, SF 5 , a boryl group, a sulfinyl group, a sulfonyl group, a phosphoroso group, a substituted or unsubstituted alkyl group having 1 to 20 carbon atoms, a substituted or unsubstituted cycloalkyl group having 3 to 20 ring carbon atoms, a substituted or unsubstituted heteroalkyl group having 1 to 20 carbon atoms, a substituted or unsubstituted arylalkyl group having 7 to 30 carbon atoms, a substituted or unsubstituted alkoxy group having 1 to 20 carbon atoms, a substituted or unsubstituted aryloxy group having 6 to 30 carbon atoms, a substituted or unsubstituted alkenyl group having 2 to 20 carbon atoms, a substituted or unsubstituted alkynyl group having 2 to 20 carbon atoms, a substituted or unsubstituted aryl group having 6 to 30 carbon atoms, a substituted or unsubstituted heteroaryl group having 3 to 30 carbon atoms, a substituted or unsubstituted alkylsilyl group having 3 to 20 carbon atoms, a substituted or unsubstituted arylsilyl group having 6 to 20 carbon atoms, and combinations thereof;

optionally, R 2 is, at each occurrence identically or differently, selected from a group consisting of: F, CF 3 , OCF 3 , SF 5 , SO 2 CF 3 , a cyano group, an isocyano group, SCN, OCN, a pentafluorophenyl group, a 4-cyanotetrafluorophenyl group, a tetrafluoropyridyl group, a pyrimidyl group, a triazinyl group, and combinations thereof;

wherein V and W are, at each occurrence identically or differently, selected from CR v R w , NR v , O, S or Se;

wherein Ar is, at each occurrence identically or differently, selected from a substituted or unsubstituted aryl group having 6 to 30 carbon atoms or a substituted or unsubstituted heteroaryl group having 3 to 30 carbon atoms;

wherein A, R a , R b , R c , R d , R e , R f , R g , R h , R v and R w are, at each occurrence identically or differently, selected from a group consisting of: hydrogen, deuterium, halogen, a nitroso group, a nitro group, an acyl group, a carbonyl group, a carboxylic acid group, an ester group, a cyano group, an isocyano group, SCN, OCN, SF 5 , a boryl group, a sulfinyl group, a sulfonyl group, a phosphoroso group, a substituted or unsubstituted alkyl group having 1 to 20 carbon atoms, a substituted or unsubstituted cycloalkyl group having 3 to 20 ring carbon atoms, a substituted or unsubstituted heteroalkyl group having 1 to 20 carbon atoms, a substituted or unsubstituted arylalkyl group having 7 to 30 carbon atoms, a substituted or unsubstituted alkoxy group having 1 to 20 carbon atoms, a substituted or unsubstituted aryloxy group having 6 to 30 carbon atoms, a substituted or unsubstituted alkenyl group having 2 to 20 carbon atoms, a substituted or unsubstituted alkynyl group having 2 to 20 carbon atoms, a substituted or unsubstituted aryl group having 6 to 30 carbon atoms, a substituted or unsubstituted heteroaryl group having 3 to 30 carbon atoms, a substituted or unsubstituted alkylsilyl group having 3 to 20 carbon atoms, a substituted or unsubstituted arylsilyl group having 6 to 20 carbon atoms, and combinations thereof;

wherein A is a group having at least one electron-withdrawing group, and for any of the structures, when one or more of R a , R b , R c , R d , R e , R f , R g , R h , R v and R w occur, at least one of R a , R b , R c , R d , R e , R f , R g , R h , R v and R w is a group having at least one electron-withdrawing group;

optionally, the group having at least one electron-withdrawing group is selected from a group consisting of: F, CF 3 , OCF 3 , SF 5 , SO 2 CF 3 , a cyano group, an isocyano group, SCN, OCN, a pentafluorophenyl group, a 4-cyanotetrafluorophenyl group, a tetrafluoropyridyl group, a pyrimidyl group, a triazinyl group, and combinations thereof;

wherein “*” represents a position where the X and Y groups are joined to a dehydrobenzodioxazole ring, a dehydrobenzodithiazole ring, or a dehydrobenzodiselenazole in Formula 1.

7. The organic electroluminescence device according to claim 1 , wherein X and Y are, at each occurrence identically or differently, selected from a group consisting of the following structures:

wherein “*” represents a position where the X and Y groups are joined to a dehydrobenzodioxazole ring, a dehydrobenzodithiazole ring, or a dehydrobenzodiselenazole in Formula 1.

8. The organic electroluminescence device according to claim 1 , wherein R is, at each occurrence identically or differently, selected from a group consisting of: hydrogen, deuterium, halogen, a nitroso group, a nitro group, an acyl group, a carbonyl group, a carboxylic acid group, an ester group, a cyano group, an isocyano group, SCN, OCN, SF 5 , a boryl group, a sulfinyl group, a sulfonyl group, a phosphoroso group, an unsubstituted alkyl group having 1 to 20 carbon atoms, an unsubstituted cycloalkyl group having 3 to 20 ring carbon atoms, an unsubstituted alkoxy group having 1 to 20 carbon atoms, an unsubstituted alkenyl group having 2 to 20 carbon atoms, an unsubstituted aryl group having 6 to 30 carbon atoms, an unsubstituted heteroaryl group having 3 to 30 carbon atoms, and any one of the following groups substituted by one or more of halogen, a nitroso group, a nitro group, an acyl group, a carbonyl group, a carboxylic acid group, an ester group, a cyano group, an isocyano group, SCN, OCN, SF 5 , a boryl group, a sulfinyl group, a sulfonyl group, and a phosphoroso group: an alkyl group having 1 to 20 carbon atoms, a cycloalkyl group having 3 to 20 ring carbon atoms, an alkoxy group having 1 to 20 carbon atoms, an alkenyl group having 2 to 20 carbon atoms, an aryl group having 6 to 30 carbon atoms, a heteroaryl group having 3 to 30 carbon atoms, and combinations thereof;

optionally, R is, at each occurrence identically or differently, selected from a group consisting of: hydrogen, deuterium, a methyl group, an isopropyl group, NO 2 , SO 2 CH 3 , SCF 3 , C 2 F 5 , OC 2 F 5 , OCH 3 , a diphenylmethylsilyl group, a phenyl group, a methoxyphenyl group, a p-methylphenyl group, a 2,6-diisopropylphenyl group, a biphenylyl group, a polyfluorophenyl group, a difluopyridyl group, a nitrophenyl group, a dimethylthiazolyl group, a vinyl group substituted by one or more of CN or CF 3 , an acetenyl group substituted by one of CN or CF 3 , a dimethylphosphoroso group, a diphenylphosphoroso group, F, CF 3 , OCF 3 , SF 5 , SO 2 CF 3 , a cyano group, an isocyano group, SCN, OCN, a trifluoromethylphenyl group, a trifluoromethoxyphenyl group, a bis(trifluoromethyl)phenyl group, a bis(trifluoromethoxy)phenyl group, a 4-cyanotetrafluorophenyl group, a phenyl or biphenylyl group substituted by one or more of F, CN or CF 3 , a tetrafluoropyridyl group, a pyrimidinyl group, a triazinyl group, a diphenylboryl group, an oxaboraanthryl group, and combinations thereof.

9. The organic electroluminescence device according to claim 8 , wherein X and Y are

10. The organic electroluminescence device according to claim 1 , wherein R is, at each occurrence identically or differently, selected from a group consisting of the following structures:

optionally, both of R in a compound represented by Formula 1 are identical;

wherein “z,?” represents a position where the R group is joined to a dehydrobenzodioxazole ring, a dehydrobenzodithiazole ring, or a dehydrobenzodiselenazole in Formula 1.

11. The organic electroluminescence device according to claim 10 , wherein the compound of Formula 1 has a structure represented by Formula 3:

wherein, in Formula 3, structures of both Z are identical, structures of both R are identical or different, and the Z, X, Y and R are respectively and correspondingly selected from atoms or groups shown in the following table;

wherein, the compound having the structure of Formula 3 is selected from a group consisting of the following compounds:

No.

Z

X

Y

R

R

Compound 1

O

A1

A1

B1

B1

Compound 2

O

A1

A1

B2

B2

Compound 3

O

A1

A1

B3

B3

Compound 4

O

A1

A1

B4

B4

Compound 5

O

A1

A1

B5

B5

Compound 6

O

A1

A1

B6

B6

Compound 7

O

A1

A1

B7

B7

Compound 8

O

A1

A1

B8

B8

Compound 9

O

A1

A1

B9

B9

Compound 10

O

A1

A1

B10

B10

Compound 11

O

A1

A1

B11

B11

Compound 12

O

A1

A1

B12

B12

Compound 13

O

A1

A1

B13

B13

Compound 14

O

A1

A1

B14

B14

Compound 15

O

A1

A1

B15

B15

Compound 16

O

A1

A1

B16

B16

Compound 17

O

A1

A1

B17

B17

Compound 18

O

A1

A1

B18

B18

Compound 19

O

A1

A1

B19

B19

Compound 20

O

A1

A1

B20

B20

Compound 21

O

A1

A1

B21

B21

Compound 22

O

A1

A1

B22

B22

Compound 23

O

A1

A1

B23

B23

Compound 24

O

A1

A1

B24

B24

Compound 25

O

A1

A1

B25

B25

Compound 26

O

A1

A1

B26

B26

Compound 27

O

A1

A1

B27

B27

Compound 28

O

A1

A1

B28

B28

Compound 29

O

A1

A1

B29

B29

Compound 30

O

A1

A1

B30

B30

Compound 31

O

A1

A1

B31

B31

Compound 32

O

A1

A1

B32

B32

Compound 33

O

A1

A1

B33

B33

Compound 34

O

A1

A1

B34

B34

Compound 35

O

A1

A1

B35

B35

Compound 36

O

A1

A1

B36

B36

Compound 37

O

A1

A1

B37

B37

Compound 38

O

A1

A1

B38

B38

Compound 39

O

A1

A1

B39

B39

Compound 40

O

A1

A1

B40

B40

Compound 41

O

A1

A1

B41

B41

Compound 42

O

A1

A1

B42

B42

Compound 43

O

A1

A1

B43

B43

Compound 44

O

A1

A1

B44

B44

Compound 45

O

A1

A1

B45

B45

Compound 46

O

A1

A1

B46

B46

Compound 47

O

A1

A1

B47

B47

Compound 48

O

A1

A1

B48

B48

Compound 49

O

A1

A1

B49

B49

Compound 50

O

A1

A1

B50

B50

Compound 51

O

A1

A1

B51

B51

Compound 52

O

A1

A1

B52

B52

Compound 53

O

A1

A1

B53

B53

Compound 54

O

A1

A1

B54

B54

Compound 55

O

A1

A1

B55

B55

Compound 56

O

A1

A1

B56

B56

Compound 57

O

A1

A1

B57

B57

Compound 58

O

A1

A1

B58

B58

Compound 59

O

A1

A1

B59

B59

Compound 60

O

A1

A1

B60

B60

Compound 61

O

A1

A1

B61

B61

Compound 62

O

A1

A1

B62

B62

Compound 63

O

A1

A1

B63

B63

Compound 64

O

A1

A1

B64

B64

Compound 65

O

A1

A1

B65

B65

Compound 66

O

A1

A1

B66

B66

Compound 67

O

A1

A1

B67

B67

Compound 68

O

A1

A1

B68

B68

Compound 69

O

A1

A1

B69

B69

Compound 70

O

A1

A1

B70

B70

Compound 71

O

A1

A1

B71

B71

Compound 72

O

A1

A1

B72

B72

Compound 73

O

A1

A1

B73

B73

Compound 74

O

A1

A1

B74

B74

Compound 75

O

A1

A1

B75

B75

Compound 76

O

A1

A1

B76

B76

Compound 77

O

A1

A1

B77

B77

Compound 78

O

A1

A1

B78

B78

Compound 79

O

A1

A1

B79

B79

Compound 80

O

A1

A1

B80

B80

Compound 81

O

A1

A1

B81

B81

Compound 82

O

A1

A1

B82

B82

Compound 83

O

A1

A1

B83

B83

Compound 84

O

A1

A1

B84

B84

Compound 85

O

A1

A1

B85

B85

Compound 86

O

A1

A1

B86

B86

Compound 87

O

A1

A1

B87

B87

Compound 88

O

A1

A1

B88

B88

Compound 89

S

A1

A1

B1

B1

Compound 90

S

A1

A1

B2

B2

Compound 91

S

A1

A1

B3

B3

Compound 92

S

A1

A1

B4

B4

Compound 93

S

A1

A1

B5

B5

Compound 94

S

A1

A1

B6

B6

Compound 95

S

A1

A1

B7

B7

Compound 96

S

A1

A1

B8

B8

Compound 97

S

A1

A1

B9

B9

Compound 98

S

A1

A1

B10

B10

Compound 99

S

A1

A1

B11

B11

Compound 100

S

A1

A1

B12

B12

Compound 101

S

A1

A1

B13

B13

Compound 102

S

A1

A1

B14

B14

Compound 103

S

A1

A1

B15

B15

Compound 104

S

A1

A1

B16

B16

Compound 105

S

A1

A1

B17

B17

Compound 106

S

A1

A1

B18

B18

Compound 107

S

A1

A1

B19

B19

Compound 108

S

A1

A1

B20

B20

Compound 109

S

A1

A1

B21

B21

Compound 110

S

A1

A1

B22

B22

Compound 111

S

A1

A1

B23

B23

Compound 112

S

A1

A1

B24

B24

Compound 113

S

A1

A1

B25

B25

Compound 114

S

A1

A1

B26

B26

Compound 115

S

A1

A1

B27

B27

Compound 116

S

A1

A1

B28

B28

Compound 117

S

A1

A1

B29

B29

Compound 118

S

A1

A1

B30

B30

Compound 119

S

A1

A1

B31

B31

Compound 120

S

A1

A1

B32

B32

Compound 121

S

A1

A1

B33

B33

Compound 122

S

A1

A1

B34

B34

Compound 123

S

A1

A1

B35

B35

Compound 124

S

A1

A1

B36

B36

Compound 125

S

A1

A1

B37

B37

Compound 126

S

A1

A1

B38

B38

Compound 127

S

A1

A1

B39

B39

Compound 128

S

A1

A1

B40

B40

Compound 129

S

A1

A1

B41

B41

Compound 130

S

A1

A1

B42

B42

Compound 131

S

A1

A1

B43

B43

Compound 132

S

A1

A1

B44

B44

Compound 133

S

A1

A1

B45

B45

Compound 134

S

A1

A1

B46

B46

Compound 135

S

A1

A1

B47

B47

Compound 136

S

A1

A1

B48

B48

Compound 137

S

A1

A1

B49

B49

Compound 138

S

A1

A1

B50

B50

Compound 139

S

A1

A1

B51

B51

Compound 140

S

A1

A1

B52

B52

Compound 141

S

A1

A1

B53

B53

Compound 142

S

A1

A1

B54

B54

Compound 143

S

A1

A1

B55

B55

Compound 144

S

A1

A1

B56

B56

Compound 145

S

A1

A1

B57

B57

Compound 146

S

A1

A1

B58

B58

Compound 147

S

A1

A1

B59

B59

Compound 148

S

A1

A1

B60

B60

Compound 149

S

A1

A1

B61

B61

Compound 150

S

A1

A1

B62

B62

Compound 151

S

A1

A1

B63

B63

Compound 152

S

A1

A1

B64

B64

Compound 153

S

A1

A1

B65

B65

Compound 154

S

A1

A1

B66

B66

Compound 155

S

A1

A1

B67

B67

Compound 156

S

A1

A1

B68

B68

Compound 157

S

A1

A1

B69

B69

Compound 158

S

A1

A1

B70

B70

Compound 159

S

A1

A1

B71

B71

Compound 160

S

A1

A1

B72

B72

Compound 161

S

A1

A1

B73

B73

Compound 162

S

A1

A1

B74

B74

Compound 163

S

A1

A1

B75

B75

Compound 164

S

A1

A1

B76

B76

Compound 165

S

A1

A1

B77

B77

Compound 166

S

A1

A1

B78

B78

Compound 167

S

A1

A1

B79

B79

Compound 168

S

A1

A1

B80

B80

Compound 169

S

A1

A1

B81

B81

Compound 170

S

A1

A1

B82

B82

Compound 171

S

A1

A1

B83

B83

Compound 172

S

A1

A1

B84

B84

Compound 173

S

A1

A1

B85

B85

Compound 174

S

A1

A1

B86

B86

Compound 175

S

A1

A1

B87

B87

Compound 176

S

A1

A1

B88

B88

Compound 177

Se

A1

A1

B1

B1

Compound 178

Se

A1

A1

B2

B2

Compound 179

Se

A1

A1

B3

B3

Compound 180

Se

A1

A1

B4

B4

Compound 181

Se

A1

A1

B5

B5

Compound 182

Se

A1

A1

B6

B6

Compound 183

Se

A1

A1

B7

B7

Compound 184

Se

A1

A1

B8

B8

Compound 185

Se

A1

A1

B9

B9

Compound 186

Se

A1

A1

B10

B10

Compound 187

Se

A1

A1

B11

B11

Compound 188

Se

A1

A1

B12

B12

Compound 189

Se

A1

A1

B13

B13

Compound 190

Se

A1

A1

B14

B14

Compound 191

Se

A1

A1

B15

B15

Compound 192

Se

A1

A1

B16

B16

Compound 193

Se

A1

A1

B17

B17

Compound 194

Se

A1

A1

B18

B18

Compound 195

Se

A1

A1

B19

B19

Compound 196

Se

A1

A1

B20

B20

Compound 197

Se

A1

A1

B21

B21

Compound 198

Se

A1

A1

B22

B22

Compound 199

Se

A1

A1

B23

B23

Compound 200

Se

A1

A1

B24

B24

Compound 201

Se

A1

A1

B25

B25

Compound 202

Se

A1

A1

B26

B26

Compound 203

Se

A1

A1

B27

B27

Compound 204

Se

A1

A1

B28

B28

Compound 205

Se

A1

A1

B29

B29

Compound 206

Se

A1

A1

B30

B30

Compound 207

Se

A1

A1

B31

B31

Compound 208

Se

A1

A1

B32

B32

Compound 209

Se

A1

A1

B33

B33

Compound 210

Se

A1

A1

B34

B34

Compound 211

Se

A1

A1

B35

B35

Compound 212

Se

A1

A1

B36

B36

Compound 213

Se

A1

A1

B37

B37

Compound 214

Se

A1

A1

B38

B38

Compound 215

Se

A1

A1

B39

B39

Compound 216

Se

A1

A1

B40

B40

Compound 217

Se

A1

A1

B41

B41

Compound 218

Se

A1

A1

B42

B42

Compound 219

Se

A1

A1

B43

B43

Compound 220

Se

A1

A1

B44

B44

Compound 221

Se

A1

A1

B45

B45

Compound 222

Se

A1

A1

B46

B46

Compound 223

Se

A1

A1

B47

B47

Compound 224

Se

A1

A1

B48

B48

Compound 225

Se

A1

A1

B49

B49

Compound 226

Se

A1

A1

B50

B50

Compound 227

Se

A1

A1

B51

B51

Compound 228

Se

A1

A1

B52

B52

Compound 229

Se

A1

A1

B53

B53

Compound 230

Se

A1

A1

B54

B54

Compound 231

Se

A1

A1

B55

B55

Compound 232

Se

A1

A1

B56

B56

Compound 233

Se

A1

A1

B57

B57

Compound 234

Se

A1

A1

B58

B58

Compound 235

Se

A1

A1

B59

B59

Compound 236

Se

A1

A1

B60

B60

Compound 237

Se

A1

A1

B61

B61

Compound 238

Se

A1

A1

B62

B62

Compound 239

Se

A1

A1

B63

B63

Compound 240

Se

A1

A1

B64

B64

Compound 241

Se

A1

A1

B65

B65

Compound 242

Se

A1

A1

B66

B66

Compound 243

Se

A1

A1

B67

B67

Compound 244

Se

A1

A1

B68

B68

Compound 245

Se

A1

A1

B69

B69

Compound 246

Se

A1

A1

B70

B70

Compound 247

Se

A1

A1

B71

B71

Compound 248

Se

A1

A1

B72

B72

Compound 249

Se

A1

A1

B73

B73

Compound 250

Se

A1

A1

B74

B74

Compound 251

Se

A1

A1

B75

B75

Compound 252

Se

A1

A1

B76

B76

Compound 253

Se

A1

A1

B77

B77

Compound 254

Se

A1

A1

B78

B78

Compound 255

Se

A1

A1

B79

B79

Compound 256

Se

A1

A1

B80

B80

Compound 257

Se

A1

A1

B81

B81

Compound 258

Se

A1

A1

B82

B82

Compound 259

Se

A1

A1

B83

B83

Compound 260

Se

A1

A1

B84

B84

Compound 261

Se

A1

A1

B85

B85

Compound 262

Se

A1

A1

B86

B86

Compound 263

Se

A1

A1

B87

B87

Compound 264

Se

A1

A1

B88

B88

Compound 265

O

A2

A2

B1

B1

Compound 266

O

A2

A2

B6

B6

Compound 267

O

A2

A2

B10

B10

Compound 268

O

A2

A2

B16

B16

Compound 269

O

A2

A2

B25

B25

Compound 270

O

A2

A2

B28

B28

Compound 271

O

A2

A2

B29

B29

Compound 272

O

A2

A2

B30

B30

Compound 273

O

A2

A2

B38

B38

Compound 274

O

A2

A2

B39

B39

Compound 275

O

A2

A2

B40

B40

Compound 276

O

A2

A2

B41

B41

Compound 277

O

A2

A2

B43

B43

Compound 278

O

A2

A2

B52

B52

Compound 279

O

A2

A2

B56

B56

Compound 280

O

A2

A2

B67

B67

Compound 281

O

A2

A2

B68

B68

Compound 282

O

A2

A2

B69

B69

Compound 283

O

A2

A2

B70

B70

Compound 284

O

A2

A2

B71

B71

Compound 285

O

A2

A2

B72

B72

Compound 286

O

A2

A2

B74

B74

Compound 287

O

A2

A2

B79

B79

Compound 288

O

A2

A2

B80

B80

Compound 289

O

A2

A2

B82

B82

Compound 290

O

A2

A2

B83

B83

Compound 291

O

A2

A2

B86

B86

Compound 292

O

A2

A2

B88

B88

Compound 293

S

A2

A2

B1

B1

Compound 294

S

A2

A2

B6

B6

Compound 295

S

A2

A2

B10

B10

Compound 296

S

A2

A2

B16

B16

Compound 297

S

A2

A2

B25

B25

Compound 298

S

A2

A2

B28

B28

Compound 299

S

A2

A2

B29

B29

Compound 300

S

A2

A2

B30

B30

Compound 301

S

A2

A2

B38

B38

Compound 302

S

A2

A2

B39

B39

Compound 303

S

A2

A2

B40

B40

Compound 304

S

A2

A2

B41

B41

Compound 305

S

A2

A2

B43

B43

Compound 306

S

A2

A2

B52

B52

Compound 307

S

A2

A2

B56

B56

Compound 308

S

A2

A2

B67

B67

Compound 309

S

A2

A2

B68

B68

Compound 310

S

A2

A2

B69

B69

Compound 311

S

A2

A2

B70

B70

Compound 312

S

A2

A2

B71

B71

Compound 313

S

A2

A2

B72

B72

Compound 314

S

A2

A2

B74

B74

Compound 315

S

A2

A2

B79

B79

Compound 316

S

A2

A2

B80

B80

Compound 317

S

A2

A2

B82

B82

Compound 318

S

A2

A2

B83

B83

Compound 319

S

A2

A2

B86

B86

Compound 320

S

A2

A2

B88

B88

Compound 321

Se

A2

A2

B1

B1

Compound 322

Se

A2

A2

B6

B6

Compound 323

Se

A2

A2

B10

B10

Compound 324

Se

A2

A2

B16

B16

Compound 325

Se

A2

A2

B25

B25

Compound 326

Se

A2

A2

B28

B28

Compound 327

Se

A2

A2

B29

B29

Compound 328

Se

A2

A2

B30

B30

Compound 329

Se

A2

A2

B38

B38

Compound 330

Se

A2

A2

B39

B39

Compound 331

Se

A2

A2

B40

B40

Compound 332

Se

A2

A2

B41

B41

Compound 333

Se

A2

A2

B43

B43

Compound 334

Se

A2

A2

B52

B52

Compound 335

Se

A2

A2

B56

B56

Compound 336

Se

A2

A2

B67

B67

Compound 337

Se

A2

A2

B68

B68

Compound 338

Se

A2

A2

B69

B69

Compound 339

Se

A2

A2

B70

B70

Compound 340

Se

A2

A2

B71

B71

Compound 341

Se

A2

A2

B72

B72

Compound 342

Se

A2

A2

B74

B74

Compound 343

Se

A2

A2

B79

B79

Compound 344

Se

A2

A2

B80

B80

Compound 345

Se

A2

A2

B82

B82

Compound 346

Se

A2

A2

B83

B83

Compound 347

Se

A2

A2

B86

B86

Compound 348

Se

A2

A2

B88

B88

Compound 349

O

A3

A3

B1

B1

Compound 350

O

A3

A3

B6

B6

Compound 351

O

A3

A3

B10

B10

Compound 352

O

A3

A3

B16

B16

Compound 353

O

A3

A3

B25

B25

Compound 354

O

A3

A3

B28

B28

Compound 355

O

A3

A3

B29

B29

Compound 356

O

A3

A3

B30

B30

Compound 357

O

A3

A3

B38

B38

Compound 358

O

A3

A3

B39

B39

Compound 359

O

A3

A3

B40

B40

Compound 360

O

A3

A3

B41

B41

Compound 361

O

A3

A3

B43

B43

Compound 362

O

A3

A3

B52

B52

Compound 363

O

A3

A3

B56

B56

Compound 364

O

A3

A3

B67

B67

Compound 365

O

A3

A3

B68

B68

Compound 366

O

A3

A3

B69

B69

Compound 367

O

A3

A3

B70

B70

Compound 368

O

A3

A3

B71

B71

Compound 369

O

A3

A3

B72

B72

Compound 370

O

A3

A3

B74

B74

Compound 371

O

A3

A3

B79

B79

Compound 372

O

A3

A3

B80

B80

Compound 373

O

A3

A3

B82

B82

Compound 374

O

A3

A3

B83

B83

Compound 375

O

A3

A3

B86

B86

Compound 376

O

A3

A3

B88

B88

Compound 377

S

A3

A3

B1

B1

Compound 378

S

A3

A3

B6

B6

Compound 379

S

A3

A3

B10

B10

Compound 380

S

A3

A3

B16

B16

Compound 381

S

A3

A3

B25

B25

Compound 382

S

A3

A3

B28

B28

Compound 383

S

A3

A3

B29

B29

Compound 384

S

A3

A3

B30

B30

Compound 385

S

A3

A3

B38

B38

Compound 386

S

A3

A3

B39

B39

Compound 387

S

A3

A3

B40

B40

Compound 388

S

A3

A3

B41

B41

Compound 389

S

A3

A3

B43

B43

Compound 390

S

A3

A3

B52

B52

Compound 391

S

A3

A3

B56

B56

Compound 392

S

A3

A3

B67

B67

Compound 393

S

A3

A3

B68

B68

Compound 394

S

A3

A3

B69

B69

Compound 395

S

A3

A3

B70

B70

Compound 396

S

A3

A3

B71

B71

Compound 397

S

A3

A3

B72

B72

Compound 398

S

A3

A3

B74

B74

Compound 399

S

A3

A3

B79

B79

Compound 400

S

A3

A3

B80

B80

Compound 401

S

A3

A3

B82

B82

Compound 402

S

A3

A3

B83

B83

Compound 403

S

A3

A3

B86

B86

Compound 404

S

A3

A3

B88

B88

Compound 405

Se

A3

A3

B1

B1

Compound 406

Se

A3

A3

B6

B6

Compound 407

Se

A3

A3

B10

B10

Compound 408

Se

A3

A3

B16

B16

Compound 409

Se

A3

A3

B25

B25

Compound 410

Se

A3

A3

B28

B28

Compound 411

Se

A3

A3

B29

B29

Compound 412

Se

A3

A3

B30

B30

Compound 413

Se

A3

A3

B38

B38

Compound 414

Se

A3

A3

B39

B39

Compound 415

Se

A3

A3

B40

B40

Compound 416

Se

A3

A3

B41

B41

Compound 417

Se

A3

A3

B43

B43

Compound 418

Se

A3

A3

B52

B52

Compound 419

Se

A3

A3

B56

B56

Compound 420

Se

A3

A3

B67

B67

Compound 421

Se

A3

A3

B68

B68

Compound 422

Se

A3

A3

B69

B69

Compound 423

Se

A3

A3

B70

B70

Compound 424

Se

A3

A3

B71

B71

Compound 425

Se

A3

A3

B72

B72

Compound 426

Se

A3

A3

B74

B74

Compound 427

Se

A3

A3

B79

B79

Compound 428

Se

A3

A3

B80

B80

Compound 429

Se

A3

A3

B82

B82

Compound 430

Se

A3

A3

B83

B83

Compound 431

Se

A3

A3

B86

B86

Compound 432

Se

A3

A3

B88

B88

Compound 433

O

A4

A4

B1

B1

Compound 434

O

A4

A4

B6

B6

Compound 435

O

A4

A4

B10

B10

Compound 436

O

A4

A4

B16

B16

Compound 437

O

A4

A4

B25

B25

Compound 438

O

A4

A4

B28

B28

Compound 439

O

A4

A4

B29

B29

Compound 440

O

A4

A4

B30

B30

Compound 441

O

A4

A4

B38

B38

Compound 442

O

A4

A4

B39

B39

Compound 443

O

A4

A4

B40

B40

Compound 444

O

A4

A4

B41

B41

Compound 445

O

A4

A4

B43

B43

Compound 446

O

A4

A4

B52

B52

Compound 447

O

A4

A4

B56

B56

Compound 448

O

A4

A4

B67

B67

Compound 449

O

A4

A4

B68

B68

Compound 450

O

A4

A4

B69

B69

Compound 451

O

A4

A4

B70

B70

Compound 452

O

A4

A4

B71

B71

Compound 453

O

A4

A4

B72

B72

Compound 454

O

A4

A4

B74

B74

Compound 455

O

A4

A4

B79

B79

Compound 456

O

A4

A4

B80

B80

Compound 457

O

A4

A4

B82

B82

Compound 458

O

A4

A4

B83

B83

Compound 459

O

A4

A4

B86

B86

Compound 460

O

A4

A4

B88

B88

Compound 461

S

A4

A4

B1

B1

Compound 462

S

A4

A4

B6

B6

Compound 463

S

A4

A4

B10

B10

Compound 464

S

A4

A4

B16

B16

Compound 465

S

A4

A4

B25

B25

Compound 466

S

A4

A4

B28

B28

Compound 467

S

A4

A4

B29

B29

Compound 468

S

A4

A4

B30

B30

Compound 469

S

A4

A4

B38

B38

Compound 470

S

A4

A4

B39

B39

Compound 471

S

A4

A4

B40

B40

Compound 472

S

A4

A4

B41

B41

Compound 473

S

A4

A4

B43

B43

Compound 474

S

A4

A4

B52

B52

Compound 475

S

A4

A4

B56

B56

Compound 476

S

A4

A4

B67

B67

Compound 477

S

A4

A4

B68

B68

Compound 478

S

A4

A4

B69

B69

Compound 479

S

A4

A4

B70

B70

Compound 480

S

A4

A4

B71

B71

Compound 481

S

A4

A4

B72

B72

Compound 482

S

A4

A4

B74

B74

Compound 483

S

A4

A4

B79

B79

Compound 484

S

A4

A4

B80

B80

Compound 485

S

A4

A4

B82

B82

Compound 486

S

A4

A4

B83

B83

Compound 487

S

A4

A4

B86

B86

Compound 488

S

A4

A4

B88

B88

Compound 489

Se

A4

A4

B1

B1

Compound 490

Se

A4

A4

B6

B6

Compound 491

Se

A4

A4

B10

B10

Compound 492

Se

A4

A4

B16

B16

Compound 493

Se

A4

A4

B25

B25

Compound 494

Se

A4

A4

B28

B28

Compound 495

Se

A4

A4

B29

B29

Compound 496

Se

A4

A4

B30

B30

Compound 497

Se

A4

A4

B38

B38

Compound 498

Se

A4

A4

B39

B39

Compound 499

Se

A4

A4

B40

B40

Compound 500

Se

A4

A4

B41

B41

Compound 501

Se

A4

A4

B43

B43

Compound 502

Se

A4

A4

B52

B52

Compound 503

Se

A4

A4

B56

B56

Compound 504

Se

A4

A4

B67

B67

Compound 505

Se

A4

A4

B68

B68

Compound 506

Se

A4

A4

B69

B69

Compound 507

Se

A4

A4

B70

B70

Compound 508

Se

A4

A4

B71

B71

Compound 509

Se

A4

A4

B72

B72

Compound 510

Se

A4

A4

B74

B74

Compound 511

Se

A4

A4

B79

B79

Compound 512

Se

A4

A4

B80

B80

Compound 513

Se

A4

A4

B82

B82

Compound 514

Se

A4

A4

B83

B83

Compound 515

Se

A4

A4

B86

B86

Compound 516

Se

A4

A4

B88

B88

Compound 517

O

A5

A5

B1

B1

Compound 518

O

A5

A5

B6

B6

Compound 519

O

A5

A5

B10

B10

Compound 520

O

A5

A5

B16

B16

Compound 521

O

A5

A5

B25

B25

Compound 522

O

A5

A5

B28

B28

Compound 523

O

A5

A5

B29

B29

Compound 524

O

A5

A5

B30

B30

Compound 525

O

A5

A5

B38

B38

Compound 526

O

A5

A5

B39

B39

Compound 527

O

A5

A5

B40

B40

Compound 528

O

A5

A5

B41

B41

Compound 529

O

A5

A5

B43

B43

Compound 530

O

A5

A5

B52

B52

Compound 531

O

A5

A5

B56

B56

Compound 532

O

A5

A5

B67

B67

Compound 533

O

A5

A5

B68

B68

Compound 534

O

A5

A5

B69

B69

Compound 535

O

A5

A5

B70

B70

Compound 536

O

A5

A5

B71

B71

Compound 537

O

A5

A5

B72

B72

Compound 538

O

A5

A5

B74

B74

Compound 539

O

A5

A5

B79

B79

Compound 540

O

A5

A5

B80

B80

Compound 541

O

A5

A5

B82

B82

Compound 542

O

A5

A5

B83

B83

Compound 543

O

A5

A5

B86

B86

Compound 544

O

A5

A5

B88

B88

Compound 545

S

A5

A5

B1

B1

Compound 546

S

A5

A5

B6

B6

Compound 547

S

A5

A5

B10

B10

Compound 548

S

A5

A5

B16

B16

Compound 549

S

A5

A5

B25

B25

Compound 550

S

A5

A5

B28

B28

Compound 551

S

A5

A5

B29

B29

Compound 552

S

A5

A5

B30

B30

Compound 553

S

A5

A5

B38

B38

Compound 554

S

A5

A5

B39

B39

Compound 555

S

A5

A5

B40

B40

Compound 556

S

A5

A5

B41

B41

Compound 557

S

A5

A5

B43

B43

Compound 558

S

A5

A5

B52

B52

Compound 559

S

A5

A5

B56

B56

Compound 560

S

A5

A5

B67

B67

Compound 561

S

A5

A5

B68

B68

Compound 562

S

A5

A5

B69

B69

Compound 563

S

A5

A5

B70

B70

Compound 564

S

A5

A5

B71

B71

Compound 565

S

A5

A5

B72

B72

Compound 566

S

A5

A5

B74

B74

Compound 567

S

A5

A5

B79

B79

Compound 568

S

A5

A5

B80

B80

Compound 569

S

A5

A5

B82

B82

Compound 570

S

A5

A5

B83

B83

Compound 571

S

A5

A5

B86

B86

Compound 572

S

A5

A5

B88

B88

Compound 573

Se

A5

A5

B1

B1

Compound 574

Se

A5

A5

B6

B6

Compound 575

Se

A5

A5

B10

B10

Compound 576

Se

A5

A5

B16

B16

Compound 577

Se

A5

A5

B25

B25

Compound 578

Se

A5

A5

B28

B28

Compound 579

Se

A5

A5

B29

B29

Compound 580

Se

A5

A5

B30

B30

Compound 581

Se

A5

A5

B38

B38

Compound 582

Se

A5

A5

B39

B39

Compound 583

Se

A5

A5

B40

B40

Compound 584

Se

A5

A5

B41

B41

Compound 585

Se

A5

A5

B43

B43

Compound 586

Se

A5

A5

B52

B52

Compound 587

Se

A5

A5

B56

B56

Compound 588

Se

A5

A5

B67

B67

Compound 589

Se

A5

A5

B68

B68

Compound 590

Se

A5

A5

B69

B69

Compound 591

Se

A5

A5

B70

B70

Compound 592

Se

A5

A5

B71

B71

Compound 593

Se

A5

A5

B72

B72

Compound 594

Se

A5

A5

B74

B74

Compound 595

Se

A5

A5

B79

B79

Compound 596

Se

A5

A5

B80

B80

Compound 597

Se

A5

A5

B82

B82

Compound 598

Se

A5

A5

B83

B83

Compound 599

Se

A5

A5

B86

B86

Compound 600

Se

A5

A5

B88

B88

Compound 601

O

A6

A6

B1

B1

Compound 602

O

A6

A6

B6

B6

Compound 603

O

A6

A6

B10

B10

Compound 604

O

A6

A6

B16

B16

Compound 605

O

A6

A6

B25

B25

Compound 606

O

A6

A6

B28

B28

Compound 607

O

A6

A6

B29

B29

Compound 608

O

A6

A6

B30

B30

Compound 609

O

A6

A6

B38

B38

Compound 610

O

A6

A6

B39

B39

Compound 611

O

A6

A6

B40

B40

Compound 612

O

A6

A6

B41

B41

Compound 613

O

A6

A6

B43

B43

Compound 614

O

A6

A6

B52

B52

Compound 615

O

A6

A6

B56

B56

Compound 616

O

A6

A6

B67

B67

Compound 617

O

A6

A6

B68

B68

Compound 618

O

A6

A6

B69

B69

Compound 619

O

A6

A6

B70

B70

Compound 620

O

A6

A6

B71

B71

Compound 621

O

A6

A6

B72

B72

Compound 622

O

A6

A6

B74

B74

Compound 623

O

A6

A6

B79

B79

Compound 624

O

A6

A6

B80

B80

Compound 625

O

A6

A6

B82

B82

Compound 626

O

A6

A6

B83

B83

Compound 627

O

A6

A6

B86

B86

Compound 628

O

A6

A6

B88

B88

Compound 629

S

A6

A6

B1

B1

Compound 630

S

A6

A6

B6

B6

Compound 631

S

A6

A6

B10

B10

Compound 632

S

A6

A6

B16

B16

Compound 633

S

A6

A6

B25

B25

Compound 634

S

A6

A6

B28

B28

Compound 635

S

A6

A6

B29

B29

Compound 636

S

A6

A6

B30

B30

Compound 637

S

A6

A6

B38

B38

Compound 638

S

A6

A6

B39

B39

Compound 639

S

A6

A6

B40

B40

Compound 640

S

A6

A6

B41

B41

Compound 641

S

A6

A6

B43

B43

Compound 642

S

A6

A6

B52

B52

Compound 643

S

A6

A6

B56

B56

Compound 644

S

A6

A6

B67

B67

Compound 645

S

A6

A6

B68

B68

Compound 646

S

A6

A6

B69

B69

Compound 647

S

A6

A6

B70

B70

Compound 648

S

A6

A6

B71

B71

Compound 649

S

A6

A6

B72

B72

Compound 650

S

A6

A6

B74

B74

Compound 651

S

A6

A6

B79

B79

Compound 652

S

A6

A6

B80

B80

Compound 653

S

A6

A6

B82

B82

Compound 654

S

A6

A6

B83

B83

Compound 655

S

A6

A6

B86

B86

Compound 656

S

A6

A6

B88

B88

Compound 657

Se

A6

A6

B1

B1

Compound 658

Se

A6

A6

B6

B6

Compound 659

Se

A6

A6

B10

B10

Compound 660

Se

A6

A6

B16

B16

Compound 661

Se

A6

A6

B25

B25

Compound 662

Se

A6

A6

B28

B28

Compound 663

Se

A6

A6

B29

B29

Compound 664

Se

A6

A6

B30

B30

Compound 665

Se

A6

A6

B38

B38

Compound 666

Se

A6

A6

B39

B39

Compound 667

Se

A6

A6

B40

B40

Compound 668

Se

A6

A6

B41

B41

Compound 669

Se

A6

A6

B43

B43

Compound 670

Se

A6

A6

B52

B52

Compound 671

Se

A6

A6

B56

B56

Compound 672

Se

A6

A6

B67

B67

Compound 673

Se

A6

A6

B68

B68

Compound 674

Se

A6

A6

B69

B69

Compound 675

Se

A6

A6

B70

B70

Compound 676

Se

A6

A6

B71

B71

Compound 677

Se

A6

A6

B72

B72

Compound 678

Se

A6

A6

B74

B74

Compound 679

Se

A6

A6

B79

B79

Compound 680

Se

A6

A6

B80

B80

Compound 681

Se

A6

A6

B82

B82

Compound 682

Se

A6

A6

B83

B83

Compound 683

Se

A6

A6

B86

B86

Compound 684

Se

A6

A6

B88

B88

Compound 685

O

A7

A7

B1

B1

Compound 686

O

A7

A7

B6

B6

Compound 687

O

A7

A7

B10

B10

Compound 688

O

A7

A7

B16

B16

Compound 689

O

A7

A7

B25

B25

Compound 690

O

A7

A7

B28

B28

Compound 691

O

A7

A7

B29

B29

Compound 692

O

A7

A7

B30

B30

Compound 693

O

A7

A7

B38

B38

Compound 694

O

A7

A7

B39

B39

Compound 695

O

A7

A7

B40

B40

Compound 696

O

A7

A7

B41

B41

Compound 697

O

A7

A7

B43

B43

Compound 698

O

A7

A7

B52

B52

Compound 699

O

A7

A7

B56

B56

Compound 700

O

A7

A7

B67

B67

Compound 701

O

A7

A7

B68

B68

Compound 702

O

A7

A7

B69

B69

Compound 703

O

A7

A7

B70

B70

Compound 704

O

A7

A7

B71

B71

Compound 705

O

A7

A7

B72

B72

Compound 706

O

A7

A7

B74

B74

Compound 707

O

A7

A7

B79

B79

Compound 708

O

A7

A7

B80

B80

Compound 709

O

A7

A7

B82

B82

Compound 710

O

A7

A7

B83

B83

Compound 711

O

A7

A7

B86

B86

Compound 712

O

A7

A7

B88

B88

Compound 713

S

A7

A7

B1

B1

Compound 714

S

A7

A7

B6

B6

Compound 715

S

A7

A7

B10

B10

Compound 716

S

A7

A7

B16

B16

Compound 717

S

A7

A7

B25

B25

Compound 718

S

A7

A7

B28

B28

Compound 719

S

A7

A7

B29

B29

Compound 720

S

A7

A7

B30

B30

Compound 721

S

A7

A7

B38

B38

Compound 722

S

A7

A7

B39

B39

Compound 723

S

A7

A7

B40

B40

Compound 724

S

A7

A7

B41

B41

Compound 725

S

A7

A7

B43

B43

Compound 726

S

A7

A7

B52

B52

Compound 727

S

A7

A7

B56

B56

Compound 728

S

A7

A7

B67

B67

Compound 729

S

A7

A7

B68

B68

Compound 730

S

A7

A7

B69

B69

Compound 731

S

A7

A7

B70

B70

Compound 732

S

A7

A7

B71

B71

Compound 733

S

A7

A7

B72

B72

Compound 734

S

A7

A7

B74

B74

Compound 735

S

A7

A7

B79

B79

Compound 736

S

A7

A7

B80

B80

Compound 737

S

A7

A7

B82

B82

Compound 738

S

A7

A7

B83

B83

Compound 739

S

A7

A7

B86

B86

Compound 740

S

A7

A7

B88

B88

Compound 741

Se

A7

A7

B1

B1

Compound 742

Se

A7

A7

B6

B6

Compound 743

Se

A7

A7

B10

B10

Compound 744

Se

A7

A7

B16

B16

Compound 745

Se

A7

A7

B25

B25

Compound 746

Se

A7

A7

B28

B28

Compound 747

Se

A7

A7

B29

B29

Compound 748

Se

A7

A7

B30

B30

Compound 749

Se

A7

A7

B38

B38

Compound 750

Se

A7

A7

B39

B39

Compound 751

Se

A7

A7

B40

B40

Compound 752

Se

A7

A7

B41

B41

Compound 753

Se

A7

A7

B43

B43

Compound 754

Se

A7

A7

B52

B52

Compound 755

Se

A7

A7

B56

B56

Compound 756

Se

A7

A7

B67

B67

Compound 757

Se

A7

A7

B68

B68

Compound 758

Se

A7

A7

B69

B69

Compound 759

Se

A7

A7

B70

B70

Compound 760

Se

A7

A7

B71

B71

Compound 761

Se

A7

A7

B72

B72

Compound 762

Se

A7

A7

B74

B74

Compound 763

Se

A7

A7

B79

B79

Compound 764

Se

A7

A7

B80

B80

Compound 765

Se

A7

A7

B82

B82

Compound 766

Se

A7

A7

B83

B83

Compound 767

Se

A7

A7

B86

B86

Compound 768

Se

A7

A7

B88

B88

Compound 769

O

O

O

B1

B1

Compound 770

O

O

O

B6

B6

Compound 771

O

O

O

B10

B10

Compound 772

O

O

O

B22

B22

Compound 773

O

O

O

B25

B25

Compound 774

O

O

O

B28

B28

Compound 775

O

O

O

B29

B29

Compound 776

O

O

O

B30

B30

Compound 777

O

O

O

B38

B38

Compound 778

O

O

O

B39

B39

Compound 779

O

O

O

B40

B40

Compound 780

O

O

O

B41

B41

Compound 781

O

O

O

B43

B43

Compound 782

O

O

O

B52

B52

Compound 783

O

O

O

B56

B56

Compound 784

O

O

O

B67

B67

Compound 785

O

O

O

B68

B68

Compound 786

O

O

O

B69

B69

Compound 787

O

O

O

B70

B70

Compound 788

O

O

O

B71

B71

Compound 789

O

O

O

B72

B72

Compound 790

O

O

O

B74

B74

Compound 791

O

O

O

B79

B79

Compound 792

O

O

O

B80

B80

Compound 793

O

O

O

B82

B82

Compound 794

O

O

O

B83

B83

Compound 795

O

O

O

B86

B86

Compound 796

O

O

O

B88

B88

Compound 797

S

O

O

B1

B1

Compound 798

S

O

O

B6

B6

Compound 799

S

O

O

B10

B10

Compound 800

S

O

O

B22

B22

Compound 801

S

O

O

B25

B25

Compound 802

S

O

O

B28

B28

Compound 803

S

O

O

B29

B29

Compound 804

S

O

O

B30

B30

Compound 805

S

O

O

B38

B38

Compound 806

S

O

O

B39

B39

Compound 807

S

O

O

B40

B40

Compound 808

S

O

O

B41

B41

Compound 809

S

O

O

B43

B43

Compound 810

S

O

O

B52

B52

Compound 811

S

O

O

B56

B56

Compound 812

S

O

O

B67

B67

Compound 813

S

O

O

B68

B68

Compound 814

S

O

O

B69

B69

Compound 815

S

O

O

B70

B70

Compound 816

S

O

O

B71

B71

Compound 817

S

O

O

B72

B72

Compound 818

S

O

O

B74

B74

Compound 819

S

O

O

B79

B79

Compound 820

S

O

O

B80

B80

Compound 821

S

O

O

B82

B82

Compound 822

S

O

O

B83

B83

Compound 823

S

O

O

B86

B86

Compound 824

S

O

O

B88

B88

Compound 825

Se

O

O

B1

B1

Compound 826

Se

O

O

B6

B6

Compound 827

Se

O

O

B10

B10

Compound 828

Se

O

O

B22

B22

Compound 829

Se

O

O

B25

B25

Compound 830

Se

O

O

B28

B28

Compound 831

Se

O

O

B29

B29

Compound 832

Se

O

O

B30

B30

Compound 833

Se

O

O

B38

B38

Compound 834

Se

O

O

B39

B39

Compound 835

Se

O

O

B40

B40

Compound 836

Se

O

O

B41

B41

Compound 837

Se

O

O

B43

B43

Compound 838

Se

O

O

B52

B52

Compound 839

Se

O

O

B56

B56

Compound 840

Se

O

O

B67

B67

Compound 841

Se

O

O

B68

B68

Compound 842

Se

O

O

B69

B69

Compound 843

Se

O

O

B70

B70

Compound 844

Se

O

O

B71

B71

Compound 845

Se

O

O

B72

B72

Compound 846

Se

O

O

B74

B74

Compound 847

Se

O

O

B79

B79

Compound 848

Se

O

O

B80

B80

Compound 849

Se

O

O

B82

B82

Compound 850

Se

O

O

B83

B83

Compound 851

Se

O

O

B86

B86

Compound 852

Se

O

O

B88

B88

Compound 853

O

S

S

B1

B1

Compound 854

O

O

O

B6

B6

Compound 855

O

S

S

B10

B10

Compound 856

O

S

S

B22

B22

Compound 857

O

S

S

B25

B25

Compound 858

O

S

S

B28

B28

Compound 859

O

S

S

B29

B29

Compound 860

O

S

S

B30

B30

Compound 861

O

S

S

B38

B38

Compound 862

O

S

S

B39

B39

Compound 863

O

S

S

B40

B40

Compound 864

O

S

S

B41

B41

Compound 865

O

S

S

B43

B43

Compound 866

O

S

S

B52

B52

Compound 867

O

S

S

B56

B56

Compound 868

O

S

S

B67

B67

Compound 869

O

S

S

B68

B68

Compound 870

O

S

S

B69

B69

Compound 871

O

S

S

B70

B70

Compound 872

O

S

S

B71

B71

Compound 873

O

S

S

B72

B72

Compound 874

O

S

S

B74

B74

Compound 875

O

S

S

B79

B79

Compound 876

O

S

S

B80

B80

Compound 877

O

S

S

B82

B82

Compound 878

O

S

S

B83

B83

Compound 879

O

S

S

B86

B86

Compound 880

O

S

S

B88

B88

Compound 881

S

S

S

B1

B1

Compound 882

S

S

S

B6

B6

Compound 883

S

S

S

B10

B10

Compound 884

S

S

S

B22

B22

Compound 885

S

S

S

B25

B25

Compound 886

S

S

S

B28

B28

Compound 887

S

S

S

B29

B29

Compound 888

S

S

S

B30

B30

Compound 889

S

S

S

B38

B38

Compound 890

S

S

S

B39

B39

Compound 891

S

S

S

B40

B40

Compound 892

S

S

S

B41

B41

Compound 893

S

S

S

B43

B43

Compound 894

S

S

S

B52

B52

Compound 895

S

S

S

B56

B56

Compound 896

S

S

S

B67

B67

Compound 897

S

S

S

B68

B68

Compound 898

S

S

S

B69

B69

Compound 899

S

S

S

B70

B70

Compound 900

S

S

S

B71

B71

Compound 901

S

S

S

B72

B72

Compound 902

S

S

S

B74

B74

Compound 903

S

S

S

B79

B79

Compound 904

S

S

S

B80

B80

Compound 905

S

S

S

B82

B82

Compound 906

S

S

S

B83

B83

Compound 907

S

S

S

B86

B86

Compound 908

S

S

S

B88

B88

Compound 909

Se

S

S

B1

B1

Compound 910

Se

S

S

B6

B6

Compound 911

Se

S

S

B10

B10

Compound 912

Se

S

S

B22

B22

Compound 913

Se

S

S

B25

B25

Compound 914

Se

S

S

B28

B28

Compound 915

Se

S

S

B29

B29

Compound 916

Se

S

S

B30

B30

Compound 917

Se

S

S

B38

B38

Compound 918

Se

S

S

B39

B39

Compound 919

Se

S

S

B40

B40

Compound 920

Se

S

S

B41

B41

Compound 921

Se

S

S

B43

B43

Compound 922

Se

S

S

B52

B52

Compound 923

Se

S

S

B56

B56

Compound 924

Se

S

S

B67

B67

Compound 925

Se

S

S

B68

B68

Compound 926

Se

S

S

B69

B69

Compound 927

Se

S

S

B70

B70

Compound 928

Se

S

S

B71

B71

Compound 929

Se

S

S

B72

B72

Compound 930

Se

S

S

B74

B74

Compound 931

Se

S

S

B79

B79

Compound 932

Se

S

S

B80

B80

Compound 933

Se

S

S

B82

B82

Compound 934

Se

S

S

B83

B83

Compound 935

Se

S

S

B86

B86

Compound 936

Se

S

S

B88

B88

Compound 937

O

Se

Se

B1

B1

Compound 938

O

Se

Se

B6

B6

Compound 939

O

Se

Se

B10

B10

Compound 940

O

Se

Se

B22

B22

Compound 941

O

Se

Se

B25

B25

Compound 942

O

Se

Se

B28

B28

Compound 943

O

Se

Se

B29

B29

Compound 944

O

Se

Se

B30

B30

Compound 945

O

Se

Se

B38

B38

Compound 946

O

Se

Se

B39

B39

Compound 947

O

Se

Se

B40

B40

Compound 948

O

Se

Se

B41

B41

Compound 949

O

Se

Se

B43

B43

Compound 950

O

Se

Se

B52

B52

Compound 951

O

Se

Se

B56

B56

Compound 952

O

Se

Se

B67

B67

Compound 953

O

Se

Se

B68

B68

Compound 954

O

Se

Se

B69

B69

Compound 955

O

Se

Se

B70

B70

Compound 956

O

Se

Se

B71

B71

Compound 957

O

Se

Se

B72

B72

Compound 958

O

Se

Se

B74

B74

Compound 959

O

Se

Se

B79

B79

Compound 960

O

Se

Se

B80

B80

Compound 961

O

Se

Se

B82

B82

Compound 962

O

Se

Se

B83

B83

Compound 963

O

Se

Se

B86

B86

Compound 964

O

Se

Se

B88

B88

Compound 965

S

Se

Se

B1

B1

Compound 966

S

Se

Se

B6

B6

Compound 967

S

Se

Se

B10

B10

Compound 968

S

Se

Se

B22

B22

Compound 969

S

Se

Se

B25

B25

Compound 970

S

Se

Se

B28

B28

Compound 971

S

Se

Se

B29

B29

Compound 972

S

Se

Se

B30

B30

Compound 973

S

Se

Se

B38

B38

Compound 974

S

Se

Se

B39

B39

Compound 975

S

Se

Se

B40

B40

Compound 976

S

Se

Se

B41

B41

Compound 977

S

Se

Se

B43

B43

Compound 978

S

Se

Se

B52

B52

Compound 979

S

Se

Se

B56

B56

Compound 980

S

Se

Se

B67

B67

Compound 981

S

Se

Se

B68

B68

Compound 982

S

Se

Se

B69

B69

Compound 983

S

Se

Se

B70

B70

Compound 984

S

Se

Se

B71

B71

Compound 985

S

Se

Se

B72

B72

Compound 986

S

Se

Se

B74

B74

Compound 987

S

Se

Se

B79

B79

Compound 988

S

Se

Se

B80

B80

Compound 989

S

Se

Se

B82

B82

Compound 990

S

Se

Se

B83

B83

Compound 991

S

Se

Se

B86

B86

Compound 992

S

Se

Se

B88

B88

Compound 993

Se

Se

Se

B1

B1

Compound 994

Se

Se

Se

B6

B6

Compound 995

Se

Se

Se

B10

B10

Compound 996

Se

Se

Se

B22

B22

Compound 997

Se

Se

Se

B25

B25

Compound 998

Se

Se

Se

B28

B28

Compound 999

Se

Se

Se

B29

B29

Compound 1000

Se

Se

Se

B30

B30

Compound 1001

Se

Se

Se

B38

B38

Compound 1002

Se

Se

Se

B39

B39

Compound 1003

Se

Se

Se

B40

B40

Compound 1004

Se

Se

Se

B41

B41

Compound 1005

Se

Se

Se

B43

B43

Compound 1006

Se

Se

Se

B52

B52

Compound 1007

Se

Se

Se

B56

B56

Compound 1008

Se

Se

Se

B67

B67

Compound 1009

Se

Se

Se

B68

B68

Compound 1010

Se

Se

Se

B69

B69

Compound 1011

Se

Se

Se

B70

B70

Compound 1012

Se

Se

Se

B71

B71

Compound 1013

Se

Se

Se

B72

B72

Compound 1014

Se

Se

Se

B74

B74

Compound 1015

Se

Se

Se

B79

B79

Compound 1016

Se

Se

Se

B80

B80

Compound 1017

Se

Se

Se

B82

B82

Compound 1018

Se

Se

Se

B83

B83

Compound 1019

Se

Se

Se

B86

B86

Compound 1020

Se

Se

Se

B88

B88

Compound 1021

O

A1

A1

B1

B6

Compound 1022

O

A1

A1

B2

B6

Compound 1023

O

A1

A1

B25

B26

Compound 1024

O

A1

A1

B27

B28

Compound 1025

O

A1

A1

B29

B30

Compound 1026

O

A1

A1

B39

B40

Compound 1027

O

A1

A1

B54

B41

Compound 1028

O

A1

A1

B54

B52

Compound 1029

O

A1

A1

B52

B56

Compound 1030

O

A1

A1

B55

B56

Compound 1031

O

A1

A1

B64

B56

Compound 1032

O

A1

A1

B68

B69

Compound 1033

O

A1

A1

B69

B70

Compound 1034

O

A1

A1

B71

B72

Compound 1035

O

A1

A1

B68

B80

Compound 1036

O

A1

A1

B68

B83

Compound 1037

S

A1

A1

B1

B6

Compound 1038

S

A1

A1

B2

B6

Compound 1039

S

A1

A1

B25

B26

Compound 1040

S

A1

A1

B27

B28

Compound 1041

S

A1

A1

B29

B30

Compound 1042

S

A1

A1

B39

B40

Compound 1043

S

A1

A1

B54

B41

Compound 1044

S

A1

A1

B54

B52

Compound 1045

S

A1

A1

B52

B56

Compound 1046

S

A1

A1

B55

B56

Compound 1047

S

A1

A1

B64

B56

Compound 1048

S

A1

A1

B68

B69

Compound 1049

S

A1

A1

B69

B70

Compound 1050

S

A1

A1

B71

B72

Compound 1051

S

A1

A1

B68

B80

Compound 1052

S

A1

A1

B68

B83

Compound 1053

Se

A1

A1

B1

B6

Compound 1054

Se

A1

A1

B2

B6

Compound 1055

Se

A1

A1

B25

B26

Compound 1056

Se

A1

A1

B27

B28

Compound 1057

Se

A1

A1

B29

B30

Compound 1058

Se

A1

A1

B39

B40

Compound 1059

Se

A1

A1

B54

B41

Compound 1060

Se

A1

A1

B54

B52

Compound 1061

Se

A1

A1

B52

B56

Compound 1062

Se

A1

A1

B55

B56

Compound 1063

Se

A1

A1

B64

B56

Compound 1064

Se

A1

A1

B68

B69

Compound 1065

Se

A1

A1

B69

B70

Compound 1066

Se

A1

A1

B71

B72

Compound 1067

Se

A1

A1

B68

B80

Compound 1068

Se

A1

A1

B68

B83

Compound 1069

O

A2

A2

B1

B6

Compound 1070

O

A2

A2

B2

B6

Compound 1071

O

A2

A2

B25

B26

Compound 1072

O

A2

A2

B27

B28

Compound 1073

O

A2

A2

B29

B30

Compound 1074

O

A2

A2

B39

B40

Compound 1075

O

A2

A2

B54

B41

Compound 1076

O

A2

A2

B54

B52

Compound 1077

O

A2

A2

B52

B56

Compound 1078

O

A2

A2

B55

B56

Compound 1079

O

A2

A2

B64

B56

Compound 1080

O

A2

A2

B68

B69

Compound 1081

O

A2

A2

B69

B70

Compound 1082

O

A2

A2

B71

B72

Compound 1083

O

A2

A2

B68

B80

Compound 1084

O

A2

A2

B68

B83

Compound 1085

S

A2

A2

B1

B6

Compound 1086

S

A2

A2

B2

B6

Compound 1087

S

A2

A2

B25

B26

Compound 1088

S

A2

A2

B27

B28

Compound 1089

S

A2

A2

B29

B30

Compound 1090

S

A2

A2

B39

B40

Compound 1091

S

A2

A2

B54

B41

Compound 1092

S

A2

A2

B54

B52

Compound 1093

S

A2

A2

B52

B56

Compound 1094

S

A2

A2

B55

B56

Compound 1095

S

A2

A2

B64

B56

Compound 1096

S

A2

A2

B68

B69

Compound 1097

S

A2

A2

B69

B70

Compound 1098

S

A2

A2

B71

B72

Compound 1099

S

A2

A2

B68

B80

Compound 1100

S

A2

A2

B68

B83

Compound 1101

Se

A2

A2

B1

B6

Compound 1102

Se

A2

A2

B2

B6

Compound 1103

Se

A2

A2

B25

B26

Compound 1104

Se

A2

A2

B27

B28

Compound 1105

Se

A2

A2

B29

B30

Compound 1106

Se

A2

A2

B39

B40

Compound 1107

Se

A2

A2

B54

B41

Compound 1108

Se

A2

A2

B54

B52

Compound 1109

Se

A2

A2

B52

B56

Compound 1110

Se

A2

A2

B55

B56

Compound 1111

Se

A2

A2

B64

B56

Compound 1112

Se

A2

A2

B68

B69

Compound 1113

Se

A2

A2

B69

B70

Compound 1114

Se

A2

A2

B71

B72

Compound 1115

Se

A2

A2

B68

B80

Compound 1116

Se

A2

A2

B68

B83

Compound 1117

O

A3

A3

B1

B1

Compound 1118

O

A3

A3

B6

B6

Compound 1119

O

A3

A3

B25

B25

Compound 1120

O

A3

A3

B28

B28

Compound 1121

O

A3

A3

B29

B29

Compound 1122

O

A3

A3

B30

B30

Compound 1123

O

A3

A3

B56

B56

Compound 1124

O

A3

A3

B67

B67

Compound 1125

O

A3

A3

B68

B68

Compound 1126

O

A3

A3

B69

B69

Compound 1127

O

A3

A3

B70

B70

Compound 1128

O

A3

A3

B71

B71

Compound 1129

O

A3

A3

B72

B72

Compound 1130

O

A3

A3

B74

B74

Compound 1131

O

A3

A3

B80

B80

Compound 1132

O

A3

A3

B83

B83

Compound 1133

S

A3

A3

B1

B1

Compound 1134

S

A3

A3

B6

B6

Compound 1135

S

A3

A3

B25

B25

Compound 1136

S

A3

A3

B28

B28

Compound 1137

S

A3

A3

B29

B29

Compound 1138

S

A3

A3

B30

B30

Compound 1139

S

A3

A3

B56

B56

Compound 1140

S

A3

A3

B67

B67

Compound 1141

S

A3

A3

B68

B68

Compound 1142

S

A3

A3

B69

B69

Compound 1143

S

A3

A3

B70

B70

Compound 1144

S

A3

A3

B71

B71

Compound 1145

S

A3

A3

B72

B72

Compound 1146

S

A3

A3

B74

B74

Compound 1147

S

A3

A3

B80

B80

Compound 1148

S

A3

A3

B83

B83

Compound 1149

Se

A3

A3

B1

B1

Compound 1150

Se

A3

A3

B6

B6

Compound 1151

Se

A3

A3

B25

B25

Compound 1152

Se

A3

A3

B28

B28

Compound 1153

Se

A3

A3

B29

B29

Compound 1154

Se

A3

A3

B30

B30

Compound 1155

Se

A3

A3

B56

B56

Compound 1156

Se

A3

A3

B67

B67

Compound 1157

Se

A3

A3

B68

B68

Compound 1158

Se

A3

A3

B69

B69

Compound 1159

Se

A3

A3

B70

B70

Compound 1160

Se

A3

A3

B71

B71

Compound 1161

Se

A3

A3

B72

B72

Compound 1162

Se

A3

A3

B74

B74

Compound 1163

Se

A3

A3

B80

B80

Compound 1164

Se

A3

A3

B83

B83

Compound 1165

O

O

A1

B1

B1

Compound 1166

O

O

A1

B6

B6

Compound 1167

O

O

A1

B25

B25

Compound 1168

O

O

A1

B28

B28

Compound 1169

O

O

A1

B29

B29

Compound 1170

O

O

A1

B30

B30

Compound 1171

O

O

A1

B56

B56

Compound 1172

O

O

A1

B67

B67

Compound 1173

O

O

A1

B68

B68

Compound 1174

O

O

A1

B69

B69

Compound 1175

O

O

A1

B70

B70

Compound 1176

O

O

A1

B71

B71

Compound 1177

O

O

A1

B72

B72

Compound 1178

O

O

A1

B74

B74

Compound 1179

O

O

A1

B80

B80

Compound 1180

O

O

A1

B83

B83

Compound 1181

S

O

A1

B1

B1

Compound 1182

S

O

A1

B6

B6

Compound 1183

S

O

A1

B25

B25

Compound 1184

S

O

A1

B28

B28

Compound 1185

S

O

A1

B29

B29

Compound 1186

S

O

A1

B30

B30

Compound 1187

S

O

A1

B56

B56

Compound 1188

S

O

A1

B67

B67

Compound 1189

S

O

A1

B68

B68

Compound 1190

S

O

A1

B69

B69

Compound 1191

S

O

A1

B70

B70

Compound 1192

S

O

A1

B71

B71

Compound 1193

S

O

A1

B72

B72

Compound 1194

S

O

A1

B74

B74

Compound 1195

S

O

A1

B80

B80

Compound 1196

S

O

A1

B83

B83

Compound 1197

Se

O

A1

B1

B1

Compound 1198

Se

O

A1

B6

B6

Compound 1199

Se

O

A1

B25

B25

Compound 1200

Se

O

A1

B28

B28

Compound 1201

Se

O

A1

B29

B29

Compound 1202

Se

O

A1

B30

B30

Compound 1203

Se

O

A1

B56

B56

Compound 1204

Se

O

A1

B67

B67

Compound 1205

Se

O

A1

B68

B68

Compound 1206

Se

O

A1

B69

B69

Compound 1207

Se

O

A1

B70

B70

Compound 1208

Se

O

A1

B71

B71

Compound 1209

Se

O

A1

B72

B72

Compound 1210

Se

O

A1

B74

B74

Compound 1211

Se

O

A1

B80

B80

Compound 1212

Se

O

A1

B83

B83

Compound 1213

O

A1

A2

B1

B1

Compound 1214

O

A1

A2

B6

B6

Compound 1215

O

A1

A2

B25

B25

Compound 1216

O

A1

A2

B28

B28

Compound 1217

O

A1

A2

B29

B29

Compound 1218

O

A1

A2

B30

B30

Compound 1219

O

A1

A2

B56

B56

Compound 1220

O

A1

A2

B67

B67

Compound 1221

O

A1

A2

B68

B68

Compound 1222

O

A1

A2

B69

B69

Compound 1223

O

A1

A2

B70

B70

Compound 1224

O

A1

A2

B71

B71

Compound 1225

O

A1

A2

B72

B72

Compound 1226

O

A1

A2

B74

B74

Compound 1227

O

A1

A2

B80

B80

Compound 1228

O

A1

A2

B83

B83

Compound 1229

S

A1

A2

B1

B1

Compound 1230

S

A1

A2

B6

B6

Compound 1231

S

A1

A2

B25

B25

Compound 1232

S

A1

A2

B28

B28

Compound 1233

S

A1

A2

B29

B29

Compound 1234

S

A1

A2

B30

B30

Compound 1235

S

A1

A2

B56

B56

Compound 1236

S

A1

A2

B67

B67

Compound 1237

S

A1

A2

B68

B68

Compound 1238

S

A1

A2

B69

B69

Compound 1239

S

A1

A2

B70

B70

Compound 1240

S

A1

A2

B71

B71

Compound 1241

S

A1

A2

B72

B72

Compound 1242

S

A1

A2

B74

B74

Compound 1243

S

A1

A2

B80

B80

Compound 1244

S

A1

A2

B83

B83

Compound 1245

Se

A1

A2

B1

B1

Compound 1246

Se

A1

A2

B6

B6

Compound 1247

Se

A1

A2

B25

B25

Compound 1248

Se

A1

A2

B28

B28

Compound 1249

Se

A1

A2

B29

B29

Compound 1250

Se

A1

A2

B30

B30

Compound 1251

Se

A1

A2

B56

B56

Compound 1252

Se

A1

A2

B67

B67

Compound 1253

Se

A1

A2

B68

B68

Compound 1254

Se

A1

A2

B69

B69

Compound 1255

Se

A1

A2

B70

B70

Compound 1256

Se

A1

A2

B71

B71

Compound 1257

Se

A1

A2

B72

B72

Compound 1258

Se

A1

A2

B74

B74

Compound 1259

Se

A1

A2

B80

B80

Compound 1260

Se

A1

A2

B83

B83

Compound 1261

O

A1

A3

B1

B1

Compound 1262

O

A1

A3

B6

B6

Compound 1263

O

A1

A3

B25

B25

Compound 1264

O

A1

A3

B28

B28

Compound 1265

O

A1

A3

B29

B29

Compound 1266

O

A1

A3

B30

B30

Compound 1267

O

A1

A3

B56

B56

Compound 1268

O

A1

A3

B67

B67

Compound 1269

O

A1

A3

B68

B68

Compound 1270

O

A1

A3

B69

B69

Compound 1271

O

A1

A3

B70

B70

Compound 1272

O

A1

A3

B71

B71

Compound 1273

O

A1

A3

B72

B72

Compound 1274

O

A1

A3

B74

B74

Compound 1275

O

A1

A3

B80

B80

Compound 1276

O

A1

A3

B83

B83

Compound 1277

S

A1

A3

B1

B1

Compound 1278

S

A1

A3

B6

B6

Compound 1279

S

A1

A3

B25

B25

Compound 1280

S

A1

A3

B28

B28

Compound 1281

S

A1

A3

B29

B29

Compound 1282

S

A1

A3

B30

B30

Compound 1283

S

A1

A3

B56

B56

Compound 1284

S

A1

A3

B67

B67

Compound 1285

S

A1

A3

B68

B68

Compound 1286

S

A1

A3

B69

B69

Compound 1287

S

A1

A3

B70

B70

Compound 1288

S

A1

A3

B71

B71

Compound 1289

S

A1

A3

B72

B72

Compound 1290

S

A1

A3

B74

B74

Compound 1291

S

A1

A3

B80

B80

Compound 1292

S

A1

A3

B83

B83

Compound 1293

Se

A1

A3

B1

B1

Compound 1294

Se

A1

A3

B6

B6

Compound 1295

Se

A1

A3

B25

B25

Compound 1296

Se

A1

A3

B28

B28

Compound 1297

Se

A1

A3

B29

B29

Compound 1298

Se

A1

A3

B30

B30

Compound 1299

Se

A1

A3

B56

B56

Compound 1300

Se

A1

A3

B67

B67

Compound 1301

Se

A1

A3

B68

B68

Compound 1302

Se

A1

A3

B69

B69

Compound 1303

Se

A1

A3

B70

B70

Compound 1304

Se

A1

A3

B71

B71

Compound 1305

Se

A1

A3

B72

B72

Compound 1306

Se

A1

A3

B74

B74

Compound 1307

Se

A1

A3

B80

B80

Compound 1308

Se

A1

A3

B83

B83

Compound 1309

O

A2

A6

B1

B1

Compound 1310

O

A2

A6

B6

B6

Compound 1311

O

A2

A6

B25

B25

Compound 1312

O

A2

A6

B28

B28

Compound 1313

O

A2

A6

B29

B29

Compound 1314

O

A2

A6

B30

B30

Compound 1315

O

A2

A6

B56

B56

Compound 1316

O

A2

A6

B67

B67

Compound 1317

O

A2

A6

B68

B68

Compound 1318

O

A2

A6

B69

B69

Compound 1319

O

A2

A6

B70

B70

Compound 1320

O

A2

A6

B71

B71

Compound 1321

O

A2

A6

B72

B72

Compound 1322

O

A2

A6

B74

B74

Compound 1323

O

A2

A6

B80

B80

Compound 1324

O

A2

A6

B83

B83

Compound 1325

S

A2

A6

B1

B1

Compound 1326

S

A2

A6

B6

B6

Compound 1327

S

A2

A6

B25

B25

Compound 1328

S

A2

A6

B28

B28

Compound 1329

S

A2

A6

B29

B29

Compound 1330

S

A2

A6

B30

B30

Compound 1331

S

A2

A6

B56

B56

Compound 1332

S

A2

A6

B67

B67

Compound 1333

S

A2

A6

B68

B68

Compound 1334

S

A2

A6

B69

B69

Compound 1335

S

A2

A6

B70

B70

Compound 1336

S

A2

A6

B71

B71

Compound 1337

S

A2

A6

B72

B72

Compound 1338

S

A2

A6

B74

B74

Compound 1339

S

A2

A6

B80

B80

Compound 1340

S

A2

A6

B83

B83

Compound 1341

Se

A2

A6

B1

B1

Compound 1342

Se

A2

A6

B6

B6

Compound 1343

Se

A2

A6

B25

B25

Compound 1344

Se

A2

A6

B28

B28

Compound 1345

Se

A2

A6

B29

B29

Compound 1346

Se

A2

A6

B30

B30

Compound 1347

Se

A2

A6

B56

B56

Compound 1348

Se

A2

A6

B67

B67

Compound 1349

Se

A2

A6

B68

B68

Compound 1350

Se

A2

A6

B69

B69

Compound 1351

Se

A2

A6

B70

B70

Compound 1352

Se

A2

A6

B71

B71

Compound 1353

Se

A2

A6

B72

B72

Compound 1354

Se

A2

A6

B74

B74

Compound 1355

Se

A2

A6

B80

B80

Compound 1356

Se

A2

A6

B83

B83.

12. The organic electroluminescence device according to claim 1 , wherein L is selected from a substituted or unsubstituted phenylene group, a substituted or unsubstituted biphenylene group, a substituted or unsubstituted terphenylene group, a substituted or unsubstituted naphthylene group, a substituted or unsubstituted fluorenylidene group, a substituted or unsubstituted silafluorenylidene group, a substituted or unsubstituted carbazolylene group, a substituted or unsubstituted dibenzofurylidene group, a substituted or unsubstituted dibenzothienylene group, a substituted or unsubstituted dibenzoselenophenylene group, a substituted or unsubstituted phenanthrylene group, a substituted or unsubstituted triphenylenylene group, a substituted or unsubstituted pyridylene group, a substituted or unsubstituted spirobifluorenylidene group, a substituted or unsubstituted anthrylene group, a substituted or unsubstituted pyrenylene group, or combinations thereof; optionally, L is selected from a substituted or unsubstituted phenylene group or a substituted or unsubstituted biphenylene group; and optionally, L is a phenylene group or a biphenylene group.

13. The organic electroluminescence device according to claim 1 , wherein R 1 is selected from hydrogen, deuterium, halogen, a substituted or unsubstituted alkyl group having 1 to 20 carbon atoms, a substituted or unsubstituted cycloalkyl group having 3 to 20 ring carbon atoms, a substituted or unsubstituted aryl group having 6 to 30 carbon atoms, or a substituted or unsubstituted heteroaryl group having 3 to 30 carbon atoms; optionally, R 1 is selected from hydrogen, deuterium, a substituted or unsubstituted aryl group having 6 to 30 carbon atoms, or a substituted or unsubstituted heteroaryl group having 3 to 30 carbon atoms.

14. The organic electroluminescence device according to claim 1 , wherein Ar 1 and Ar 2 are selected from a substituted or unsubstituted aryl group having 6 to 20 carbon atoms or a substituted or unsubstituted heteroaryl group having 3 to 20 carbon atoms; optionally, Ar 1 and Ar 2 are selected from a phenyl group, a biphenylyl group, a terphenyl group, a naphthyl group, a fluorenyl group, a dibenzothienyl group, a spirobifluorenyl group, a pyridyl group, or a pyrimidinyl group.

15. The organic electroluminescence device according to claim 1 , wherein the compound having the structure of Formula 2 is selected from a group consisting of the following compounds:

16. The organic electroluminescence device according to claim 1 , further comprising a second organic layer disposed between the anode and the light-emitting layer, wherein the second organic layer comprises the compound of Formula 2.

17. The organic electroluminescence device according to claim 16 , wherein the first organic layer is in contact with the anode.

18. The organic electroluminescence device according to claim 1 , wherein the compound of Formula 1 comprised in the first organic layer accounts for not higher than 5%, or not higher than 3%, or not higher than 2%, or not higher than 1% by weight of the entire first organic layer.

19. The organic electroluminescence device according to claim 16 , wherein the second organic layer is in contact with the light-emitting layer.

20. The organic electroluminescence device according to claim 1 , further comprising a third organic layer disposed between the anode and the light-emitting layer, wherein the third organic layer comprises a compound different from the compound comprised in the second organic layer.

21. A display assembly, comprising the organic electroluminescence device according to claim 1 .

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 1, 2020
From: PANG, HUIQING; JIA, RU; CUI, ZHIHAO; CHEN, XIAO; XIA, CHUANJUN; KWONG, CHI YUEN RAYMOND; WANG, JING
To: BEIJING SUMMER SPROUT TECHNOLOGY CO., LTD.
Reel/Frame 054506/0176 →
Priority Claims (1)
CN 201911209540.X · Dec 3, 2019 · national
Continuity (1)
Related Publication 20210167298A1 · Jun 3, 2021