IP Library › Granted Patent US 12,240,036
Granted Patent B2
US 12,240,036 · App. 18/164,038 · Granted Mar 4, 2025

MnAl alloy, particles thereof, and method for production

Inventors: Hailiang Fang (Uppsala, SE); Martin Häggblad Sahlberg (Uppsala, SE); Björn Skårman (Höganäs, SE)
Assignee: Höganäs AB (Publ)
B22F1/05B22F1/142B22F9/08C22C1/045C22C22/00B22F2301/20B22F2304/10
View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 12,240,036
App. No.
18/164,038
Granted
Mar 4, 2025
Kind
B2
Abstract

An alloy represented by the formula (Mn x Al y )C z , the alloy being aluminum (Al), manganese (Mn), and carbon (C), and optionally unavoidable impurities; wherein x=56.0 to 59.0 y=41.0 to 44.0 x+y=100, and z=1.5 to 2.4. The alloy is highly suitable for forming the ε and τ phase in high purity and high microstructural homogeneity. A method for processing an alloy of formula (Mn x′ Al y′ )C z′ , wherein x′=52.0 to 59.0, y′=41.0 to 48.0, x′+y′=100, and z′=0.1 to 3.0, the process including providing the raw materials of the alloy, melting the raw materials, and forming particles of the alloy by gas atomization of the molten alloy.

Claims (37)

1. A method for producing or treating an alloy having a composition of formula (II)

(Mn x′ Al y′ )C z′   (II)

wherein

x′=52.0 to 59.0

y′=41.0 to 48.0

x′+y′=100, and

z′=0.1 to 3.0

wherein the ratio of x′ to z′ (x′/z′) is in the range of 26 to 30,

the alloy consisting of Mn, Al, C, and optionally unavoidable impurities, the process comprising:

a. optionally, providing the raw materials of the alloy, melting the raw materials, and forming particles of the alloy by gas atomization of the molten alloy;

b. optionally, performing a heat treatment on the alloy at 900-1200° C.;

c. milling the alloy represented by formula (II) at a temperature of −20° C. or below-; and

d. performing a heat treatment on particles of the alloy represented by formula (II) at a temperature of 900 to 1000° C. for a time of 0.5 to 20 minutes,

wherein the milling c. is performed prior to the heat treatment d.

2. The method according to claim 1 , wherein

x′=56.0 to 59.0

y′=41.0 to 448.0

x′+y′=100, and

z′=1.5 to 2.4.

3. The method according to claim 1 , wherein z′=1.7 to 2.2.

4. The method according to claim 1 , wherein x′=56.5 to 58.5 and y′=41.5 to 43.5.

5. The method according to claim 1 , wherein x′=57.0 to 58.0 and y′=42.0 to 43.0.

6. The method according to claim 1 , wherein the ratio of x′ to z′ (x′/z′) is in the range of 27.5 to 30.

7. The method according to claim 1 , wherein the alloy has a & phase content of 90% by mass or more.

8. The method according to claim 1 , wherein all of steps a. to d. are performed.

9. The method according to claim 1 , wherein step a. is performed.

10. The method according to claim 1 , wherein step c. is performed at a temperature of −100° C. or lower.

11. The method according to claim 1 , wherein step c. is performed at a temperature of −150° C. or lower.

12. The method according to claim 1 , wherein step d. is performed for 5 to 15 minutes.

13. An alloy obtainable by the method according to claim 1 .

14. The alloy according to claim 13 , which has a content of the t phase of 80% or more.

15. The alloy according to claim 13 , which has a saturation magnetization M S of 100 emu/g or more.

16. The alloy according to claim 13 , which is in the form of particles having a median particle diameter D50, as determined by a light scattering method, of 5000 μm or less.

17. The alloy according to claim 13 , which is in the form of particles having a median particle diameter D50, as determined by a light scattering method, of 200 μm or less.

18. The alloy according to claim 13 , which is in the form of particles having a median particle diameter D50, as determined by a light scattering method, of 100 μm or less.

19. The alloy according to claim 13 , wherein the alloy is in the form of particles.

20. The alloy according to claim 13 , wherein the alloy has a saturation magnetization M S of 100 emu/g or more.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 3, 2023
From: FANG, HAILIANG; SAHLBERG, MARTIN HÄGGBLAD; SKÅRMAN, BJÖRN
To: HÖGANÄS AB (PUBL)
Reel/Frame 062583/0503 →
Priority Claims (1)
EP 17189240 · Sep 4, 2017 · regional
Continuity (2)
Division 16644397
Related Publication 20230249248A1 · Aug 10, 2023
References Cited (24)
US 3944445A · Ohtani et al. · 1976 [cited by applicant]
US 11738389B2 · Fang · 2023 [cited by examiner]
US 20070220772A1 · Kato et al. · 2007 [cited by applicant]
US 20100218858A1 · Baker et al. · 2010 [cited by applicant]
US 20120003114A1 · Baker et al. · 2012 [cited by applicant]
US 20160307677A1 · Baker · 2016 [cited by examiner]
US 20210062305A1 · Fang et al. · 2021 [cited by applicant]
US 20220165463A1 · Vidarsson et al. · 2022 [cited by applicant]
CN 105734374A · 2016 [cited by applicant]
JP S3912223B · 1965 [cited by applicant]
JP S5067213A · 1975 [cited by applicant]
JP S56147412A · 1981 [cited by applicant]
JP 2002356703A · 2002 [cited by applicant]
WO WO2008048277A2 · 2008 [cited by examiner]
WO 2008048277A3 · 2008 [cited by applicant]
H. Fang et al., Structural, Microstructural, and Magnetic Evolution in Cryo Milled Carbon Doped MnAl, Jun. 2, 2018, Scientific Reports, 8, 2525(2018) (Year: 2018). [cited by examiner]
International Search Report (PCT/ISA/210) issued on Oct. 8, 2018, by the European Patent Office as the International Searching Authority for International Application No. PCT/EP2018/073595. [cited by applicant]
Office Action (Notice of Reasons for Refusal) issued on Oct. 14, 2022, by the Japanese Patent Office in corresponding Japanese Patent Application No. 2020-512792, and an English Translation of the Office Action. (20 pag… [cited by applicant]
Ogheneyunume et al., “Effect of Ambient Aging on Heat-Treated Mechanically Alloyed Mn—Al—C Powders”, IEEE Transactions on Magnetics, vol. 49, No. 7, pp. 3372-3374, Jul. 1, 2013. XP011519975. [cited by applicant]
V. T. et al., “Neutron Diffraction Study of the [tau]-Phase of Carbon-Doped Mn—Al Alloy”, Physica Status Sou Di (A). Applied Research, vol. 159, No. 2, Feb. 1, 1997, pp. 323-326. XP055460019. [cited by applicant]
Written Opinion (PCT/ISA/237) issued on Oct. 8, 2018, by the European Patent Office as the International Searching Authority for International Application No. PCT/EP2018/073595. [cited by applicant]
Zeng, et al., “Structural and magnetic properties of nanostructured Mn—Al—C magnetic materials”, Journal of Magnetism and Magnetic Mater, Elsevier, vol. 308, No. 2, pp. 214-226, Jan. 1, 2007. XP005708070. [cited by applicant]
Wyslocki , et al. , “Magnetic Domain Structure of Isotropic MnAlC Permanent Magnet Alloys”, Journal of Materials Science, vol. 19 , 1983 , pp. 1261-1266. [cited by applicant]
Office Action (Request for the Submission of an Opinion) issued on Mar. 16, 2023, by the Intellectual Property Office in corresponding Korean Patent Application No. 10-2020-7009489, and an English Translation of the Off… [cited by applicant]