IP Library Granted Patent US 12,391,892
Granted Patent B2
US 12,391,892 · App. 18/452,388 · Granted Aug 19, 2025

Integration of polymeric waste co-processing in cokers to produce circular chemical products from coker gas oil

Inventors: Bryan A. Patel (Jersey City, TX); Brenda A. Raich (Annandale, NJ); Steven M. Slack (Humble, TX); Derrick B. Callander (Humble, TX); Eric M. Yucha (Spring, TX); Fritz A. Bernatz (Spring, TX); Rainer Kolb (Kingwood, TX); Alex S. Kolb (Houston, TX)
Assignee: ExxonMobil Chemical Patents Inc.
C10G65/10C10B49/22C10G2300/1007C10G2400/20
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Quick Facts
Patent No.
US 12,391,892
App. No.
18/452,388
Granted
Aug 19, 2025
Kind
B2
Abstract

Systems and methods are provided for integration of polymeric waste co-processing in cokers to produce circular chemical products from coker gas oil, including a method of producing circular chemical products comprising: providing a coker gas oil that is at least partially derived from polymeric waste, wherein the coker gas oil has a paraffin content of about 5 wt % to about 50 wt %, a sulfur content of about 0.1 wt % to about 7 wt %, and a halide content of about 0.1 wppm to about 5 wppm; and converting the coker gas oil into at least a polymer.

Claims (29)

1. A method of producing circular chemical products comprising:

providing a coker gas oil that is at least partially derived from polymeric waste, wherein the coker gas oil has a paraffin content of about 5 wt % to about 50 wt %, a sulfur content of about 0.1 wt % to about 7 wt %, and a halide content of about 0.1 wppm to about 5 wppm; and

converting the coker gas oil into at least a polymer.

2. The method of claim 1 , wherein the coker gas oil is derived from co-processing of polymeric waste and a heavy oil with a T10 distillation point of about 343° C. to about 575° C.

3. The method of claim 1 , wherein providing the coker gas oil comprises: coking a feedstock comprising the polymeric waste and a heavy oil with a T10 distillation point of about 343° C. to about 575° C. to form at least a coker effluent and coke; and separating the coker gas oil from the coker effluent.

4. The method of claim 3 , wherein the polymeric waste comprises plastic waste.

5. The method of claim 3 , wherein the heavy oil comprises petroleum vacuum resid.

6. The method of claim 3 , wherein the feedstock comprises the polymeric waste in an amount of about 0.1 wt % to about 25 wt %.

7. The method of claim 3 , wherein the coking comprises exposing the feedstock to delayed coking conditions.

8. The method of claim 1 , wherein providing the coker gas oil comprises pyrolyzing the polymeric waste to produce at least a pyrolysis oil and then coking at least the pyrolysis oil and a heavy oil with a T10 distillation point of about 343° C. to about 575° C.

9. The method of claim 1 , wherein the polymeric waste comprises plastic waste.

10. The method of claim 1 , wherein at least a portion of the polymer is attributable to polymers in the polymeric waste.

11. The method of claim 1 , wherein the polymer comprises a circular polymer.

12. The method of claim 1 , wherein the polymer comprises a polymer that is certified circular in accordance with International Sustainability and Carbon Certification.

13. The method of claim 1 , further comprising treating the coker gas oil to reduce a concentration of one or more contaminants prior to the step of converting the coker gas oil.

14. The method of claim 13 , wherein the treating comprises hydroprocessing the coker gas oil.

15. The method of claim 1 , wherein the converting the coker gas oil into at least the polymer comprises recovering olefins from the coker gas oil; and polymerizing at least a portion of the olefins.

16. The method of claim 1 , wherein the converting the coker gas oil into at least the polymer comprises hydroprocessing at least a portion of the coker gas oil to form at least a hydroprocessing effluent, steam cracking at least a portion of the hydroprocessing effluent to form at least a steam cracking effluent; recovering olefins from the steam cracking effluent; and polymerizing at least a portion of the olefins.

17. The method of claim 16 , wherein the hydroprocessing comprises hydrotreating at least a portion of the coker gas oil to form at least a hydrotreating effluent; and hydrocracking at least a portion of the hydrotreating effluent to form at least the hydroprocessing effluent.

18. The method of claim 1 , wherein the converting the coker gas oil into at least the polymer comprises fluid catalytic cracking at least a portion of the coker gas oil to form at least a fluid catalytic cracking effluent; recovering olefins from at least a portion of the fluid catalytic cracking effluent; and polymerizing at least a portion of the olefins.

19. The method of claim 1 , wherein the converting the coker gas oil into at least the polymer comprises partially oxidizing at least a portion of the coker gas oil by at least combustion of the coker gas oil and an oxygen-containing gas to form at least an oxidation effluent comprising carbon monoxide and hydrogen; and reacting at least a portion of the oxidation effluent in the presence of olefins and a hydroformylation catalyst to form at least oxo alcohols.

20. A method of producing circular chemical products comprising:

providing a coker gas oil that is at least partially derived from polymeric waste, wherein the coker gas oil has a paraffin content of about 5 wt % to about 50 wt %, a sulfur content of about 0.1 wt % to about 7 wt %, and a halide content of about 0.1 wppm to about 5 wppm;

hydroprocessing at least a portion of the coker gas oil to form at least a hydroprocessing effluent;

steam cracking at least a portion of the hydroprocessing effluent to form at least a steam cracking effluent;

recovering olefins from the steam cracking effluent; and

polymerizing at least a portion of the olefins to form at least polyolefins.

21. The method of claim 20 , wherein the hydroprocessing comprises hydrotreating at least a portion of the coker gas oil to form at least a hydrotreating effluent; and hydrocracking at least a portion of the hydrotreating effluent to form at least the hydroprocessing effluent.

22. The method of claim 20 , further comprising coking a feedstock comprising the polymeric waste and a heavy oil with a T10 distillation point of about 343° C. to about 575° C. to form at least a coker effluent and coke; and separating the coker gas oil from the coker effluent.

Continuity (2)
Provisional Application 63374946 · Sep 8, 2022
Related Publication 20240093102A1 · Mar 21, 2024
References Cited (42)
US 4118281A · Yan · 1978 [cited by examiner]
US 4851601A · Fukuda et al. · 1989 [cited by applicant]
US 5705724A · Collins et al. · 1998 [cited by applicant]
US 6407301B1 · Foley et al. · 2002 [cited by applicant]
US 6652737B2 · Touvelle et al. · 2003 [cited by applicant]
US 6803494B1 · Ladwig · 2004 [cited by examiner]
US 10294432B2 · Srivastava et al. · 2019 [cited by applicant]
US 10472574B2 · Al-Ghamdi et al. · 2019 [cited by applicant]
US 11174436B2 · Timken · 2021 [cited by applicant]
US 11174437B2 · Timken · 2021 [cited by applicant]
US 11306253B2 · Timken et al. · 2022 [cited by applicant]
US 11421159B2 · Pradeep · 2022 [cited by examiner]
US 20050101814A1 · Foley et al. · 2005 [cited by applicant]
US 20080194900A1 · Bhirud · 2008 [cited by applicant]
US 20110005911A1 · Bernatz et al. · 2011 [cited by applicant]
US 20110005912A1 · Sabottke et al. · 2011 [cited by applicant]
US 20210189248A1 · Timken · 2021 [cited by applicant]
US 20210189249A1 · Timken · 2021 [cited by applicant]
US 20210189250A1 · Timken · 2021 [cited by applicant]
US 20210189251A1 · Timken · 2021 [cited by applicant]
US 20210189252A1 · Timken · 2021 [cited by applicant]
US 20210189253A1 · Timken · 2021 [cited by applicant]
US 20210189254A1 · Timken · 2021 [cited by applicant]
US 20210301209A1 · Timken et al. · 2021 [cited by applicant]
US 20210301210A1 · Timken et al. · 2021 [cited by applicant]
US 20210332299A1 · Timken · 2021 [cited by applicant]
US 20210332300A1 · Timken · 2021 [cited by applicant]
US 20220098490A1 · Abbott et al. · 2022 [cited by applicant]
US 20220098491A1 · Abbott et al. · 2022 [cited by applicant]
US 20220325189A1 · Shen et al. · 2022 [cited by applicant]
US 20220333026A1 · Brown et al. · 2022 [cited by applicant]
US 20220372375A1 · Patel et al. · 2022 [cited by applicant]
US 20230047205A1 · Siddiqui · 2023 [cited by examiner]
CN 1837331 · 2009 [cited by applicant]
CN 101230284 · 2013 [cited by applicant]
EP 3795656 · 2021 [cited by applicant]
PL 216590 · 2014 [cited by applicant]
WO WO1995014069 · 1995 [cited by applicant]
WO WO2021091724 · 2021 [cited by applicant]
WO WO2021138593 · 2021 [cited by applicant]
WO WO2021201932 · 2021 [cited by applicant]
Nchare, M. et al. (2012) “Co-Processing Vacuum Residue with Waste Plastics in a Delayed Coking Process: Kinetics and Modeling,” [cited by applicant]