IP Library Granted Patent US 12,474,262
Granted Patent B2
US 12,474,262 · App. 18/569,343 · Granted Nov 18, 2025

Single-shot multi-frame ultrafast terahertz imaging method and system

Inventors: Junliang Dong (Longueuil, CA); Pei You (Urbana, IL); Alessandro Tomasino (Lausanne, CH); Aycan Yurtsever (Longueuil, CA); Yoann Jestin (Montreal, CA); Roberto Morandotti (Montreal, CA)
Assignee: INSTITUT NATIONAL DE LA RECHERCHE SCIENTIFIQUE
G01N21/3586G01N21/17G01N2021/1765G01N2021/1791G01N21/21G01N2201/061G03B39/00
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Quick Facts
Patent No.
US 12,474,262
App. No.
18/569,343
Granted
Nov 18, 2025
Kind
B2
Abstract

A method and a system for single-shot multi-frame ultrafast terahertz imaging of a scene, the method comprising generating a pump beam and a probe beam: generating a THz beam from the pump beam and passing the THz beam through the scene: multiplexing the probe beam in the time domain and in the spatial-frequency domain, yielding a multiplexed probe beam; detecting a THz beam passing through the scene; guiding the multiplexed probe beam to a THz detection crystal and converting the multiplexed probe beam into mutually orthogonal linear polarized beams; guiding the mutually orthogonal linear polarized beams to a camera; and recovering frames of the scene from multiplexed images acquired by the camera.

Claims (35)

1 . A system for single-shot multi-frame ultrafast terahertz imaging of a scene, the system comprising:

a laser producing a pump beam and a probe beam;

a THz generator generating a THz beam from said pump beam, the THz beam being passed through the scene;

a multiplexer selected for multiplexing the probe beam in the time domain and in the spatial-frequency domain, yielding a multiplexed probe beam;

a THz detector detecting a THz beam passing through the scene;

a first optical lens guiding the multiplexed probe beam to the THz detector;

a polariser selected for conversion of the multiplexed probe beam into mutually orthogonal linear polarized beams;

a camera; and

a second optical lens selected for directing the mutually orthogonal linear polarized beams to the camera.

2 . The system of claim 1 , wherein the pump beam and the probe beam have a pulse duration in a range between 50 fs and 200 fs.

3 . The system of claim 1 , wherein the multiplexer comprises delay lines selected for multiplexing the probe beam in the time domain and gratings selected for multiplexing the probe beam in the spatial-frequency domain.

4 . The system of claim 1 , wherein the THz generator is a first Pockels crystal.

5 . The system of claim 1 , wherein the THz generator is one of: a ZnTe crystal, a LiNbO 3 crystal, and a GaSe crystal.

6 . The system of claim 1 , wherein the THz detector is a Pockels crystal.

7 . The system of claim 1 , wherein the THz detector is one of: a ZnTe crystal, a LiNbO 3 crystal, and a GaSe crystal.

8 . The system of claim 1 , wherein the multiplexer comprises optical delay lines selected for multiplexing the probe beam in the time domain and gratings selected for multiplexing the probe beam in the spatial-frequency domain, first beam-splitters splitting the probe beam into equally intense sub-pulses, and each sub-pulse being directed into one of the optical delay lines to control respective arrival times separately, the gratings receiving the delayed sub-pulses, each grating being selected with a unique orientation for spatial-frequency multiplexing, the system comprising a lens collecting ±1 diffraction orders of the beam and forming sinusoidal fringe patterns in a volume of the probe beam, a final beam-splitter recombining the sub-pulses to form the multiplexed probe beam.

9 . The system of claim 1 , wherein the multiplexer comprises optical delay lines selected for multiplexing the probe beam in the time domain and gratings selected for multiplexing the probe beam in the spatial-frequency domain, first beam-splitters splitting the probe beam into equally intense sub-pulses, and each sub-pulse being directed into one of the optical delay lines to control respective arrival times separately, the gratings receiving the delayed sub-pulses, each grating being selected with a unique orientation for spatial-frequency multiplexing, the system comprising an imaging lens collecting ±1 diffraction orders of the beam and forming sinusoidal fringe patterns in a volume of the probe beam, a final beam-splitter recombining the sub-pulses to form the multiplexed probe beam, a distance between the third lens and the gratings being selected equal to a focal length of the imaging lens for each sub-pulse.

10 . The system of claim 1 , wherein the multiplexed probe beam first illuminates the THz detector in a counter-propagation direction of the THz beam, and the multiplexed probe beam co-propagates with the THz beam, polarization of each sub-pulses of the multiplexed probe beam being modulated by THz electric fields, and thus, carrying a 2D information of the scene at four different times.

11 . The system of claim 1 , wherein the first optical lens is selected with a focal length in a range between 100 mm and 500 mm.

12 . The system of claim 1 , wherein the second optical lens is selected with a focal length in a range between 100 mm and 500 mm.

13 . The system of claim 1 , wherein the camera is a charged-coupled device camera.

14 . The system of claim 1 , wherein the multiplexer comprises beam splitters and gratings, the beam-splitters splitting the probe beam into equally intense sub-pulses, and each sub-pulse being directed into an optical delay line to control respective arrival times separately, the gratings receiving the delayed sub-pulses, each grating being selected with a unique orientation for spatial-frequency multiplexing, the system comprising an imaging lens collecting ±1 diffraction orders of the beam and forming sinusoidal fringe patterns in a volume of the probe beam, a final beam-splitter recombining the sub-pulses to form the multiplexed probe beam, a distance between the imaging lens and the gratings being selected equal to a focal length of the imaging lens for each sub-pulse, wherein the gratings are Ronchi gratings selected with frequencies in a range between 10 lp/mm and 50 lp/mm.

15 . The system of claim 1 , wherein the polarization beam splitter converts the multiplexed probe beam into mutually orthogonal linear polarized beams and the camera captures two polarization intensities of the multiplexed probe beam to produce an image.

16 . The system of claim 1 , wherein the polarization beam splitter converts the multiplexed probe beam into mutually orthogonal linear polarized beams and the camera captures two polarization intensities of the multiplexed probe beam to produce an image an overlapped/multiplexed image of different frames related to sub-pulses comprising the probe beam, each frame, corresponding to 2D information of the scene at different times.

17 . The system of claim 1 , wherein the polarization beam splitter is a Wollaston prism.

18 . A method for single-shot multi-frame ultrafast terahertz imaging of a scene, comprising:

generating a pump beam and a probe beam;

generating a THz beam from the pump beam and passing the THz beam through the scene;

multiplexing the probe beam in the time domain and in the spatial-frequency domain, yielding a multiplexed probe beam;

detecting a THz beam passing through the scene

guiding the multiplexed probe beam to a THz detection crystal and converting the multiplexed probe beam into mutually orthogonal linear polarized beams;

guiding the mutually orthogonal linear polarized beams to a camera; and

recovering frames of the scene from multiplexed images acquired by the camera.

19 . The method of claim 18 , comprising using crystals for said generating the THz beam and for said detecting the THz beam using electro-optic sampling.

20 . The method of claim 18 , wherein the pump beam and the probe beam have a pulse duration in a range between 50 fs and 200 fs.

Assignments (6)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 13, 2023
From: DONG, JUNLIANG
To: INSTITUT NATIONAL DE LA RECHERCHE SCIENTIFIQUE
Reel/Frame 065858/0745 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 13, 2023
From: JESTIN, YOANN
To: INSTITUT NATIONAL DE LA RECHERCHE SCIENTIFIQUE
Reel/Frame 065858/0761 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 13, 2023
From: MORANDOTTI, ROBERTO
To: INSTITUT NATIONAL DE LA RECHERCHE SCIENTIFIQUE
Reel/Frame 065858/0792 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 13, 2023
From: TOMASINO, ALESSANDRO
To: INSTITUT NATIONAL DE LA RECHERCHE SCIENTIFIQUE
Reel/Frame 065858/0811 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 13, 2023
From: YOU, PEI
To: INSTITUT NATIONAL DE LA RECHERCHE SCIENTIFIQUE
Reel/Frame 065858/0831 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 13, 2023
From: YURTSEVER, AYCAN
To: INSTITUT NATIONAL DE LA RECHERCHE SCIENTIFIQUE
Reel/Frame 065858/0835 →
Continuity (2)
Provisional Application 63202886 · Jun 29, 2021
Related Publication 20240385110A1 · Nov 21, 2024
References Cited (46)
US 9335213B2 · Sharma · 2016 [cited by examiner]
US 10175111B2 · Ozaki · 2019 [cited by examiner]
US 11604139B2 · Piccoli · 2023 [cited by examiner]
US 20170336262A1 · Ozaki · 2017 [cited by examiner]
US 20210096066A1 · Piccoli · 2021 [cited by examiner]
US 20220021473A1 · Dong · 2022 [cited by examiner]
International Search Report and Written Opinion issued in PCT application No. CA2022/050942. [cited by applicant]
Moon et al., Single-shot imaging of microscopic dynamic scenes at 5 THz frame rates by time and spatial frequency multiplexing, Optic Express 4469, vol. 28 No. 4/17/Feb. 2020. [cited by applicant]
Bidare, P., Bitharas, I., Ward, R. M., Attallah, M. M. & Moore, A. J. Fluid and particle dynamics in laser powder bed fusion. Acta Mater. 142, 107-120 (2018). [cited by applicant]
Blanchard, F. et al. Real-time terahertz near-field microscope. Opt. Express 19, 8277 (2011). [cited by applicant]
Dong, J. et al. Nondestructive evaluation of forced delamination in glass fiber-reinforced composites by terahertz and ultrasonic waves. Compos. Part B Eng. 79, 667-675 (2015). [cited by applicant]
Dong, J., Wu, X., Locquet, A. & Citrin, D. S. Terahertz Superresolution Stratigraphic Characterization of Multilayered Structures Using Sparse Deconvolution. IEEE Trans. Terahertz Sci. Technol. 7, 260-267 (2017). [cited by applicant]
Dong, R. et al. High-mobility band-like charge transport in a semiconducting two-dimensional metal-organic framework. Nat. Mater. 17, 1027-1032 (2018). [cited by applicant]
Ehn, A. et al. FRAME: femtosecond videography for atomic and molecular dynamics. Light Sci. Appl. 6, e17045-e17045 (2017). [cited by applicant]
Fülöp, J. A., Páfalvi, L., Almási, G. & Hebling, J. Design of high-energy terahertz sources based on optical rectification. Opt. Express 18, 12311 (2010). [cited by applicant]
Gao, L., Liang, J., Li, C. & Wang, L. V. Single-shot compressed ultrafast photography at one hundred billion frames per second. Nature 516, 74-77 (2014). [cited by applicant]
Gragston, M., Smith, C., Kartashov, D., Shneider, M. N. & Zhang, Z. Single-shot nanosecond-resolution multiframe passive imaging by multiplexed structured image capture. Opt. Express 26, 28441 (2018). [cited by applicant]
Guerboukha, H., Nallappan, K. & Skorobogatiy, M. Toward real-time terahertz imaging. Adv. Opt. Photonics 10, 843 (2018). [cited by applicant]
Jepsen, P. U., Cooke, D. G. & Koch, M. Terahertz spectroscopy and imaging—Modern techniques and applications. Laser Photon. Rev. 5, 124-166 (2011). [cited by applicant]
Lai, Y. et al. Single-Shot Ultraviolet Compressed Ultrafast Photography. Laser Photon. Rev. 14, 2000122 (2020). [cited by applicant]
Lane, P. A., Cunningham, P. D., Melinger, J. S., Esenturk, O. & Heilweil, E. J. Hot photocarrier dynamics in organic solar cells. Nat. Commun. 6, 7558 (2015). [cited by applicant]
Li, Z., Zgadzaj, R., Wang, X., Chang, Y.-Y. & Downer, M. C. Single-shot tomographic movies of evolving light-velocity objects. Nat. Commun. 5, 3085 (2014). [cited by applicant]
Liang, J. & Wang, L. V. Single-shot ultrafast optical imaging. Optica 5, 1113 (2018). [cited by applicant]
Luo, L. et al. Ultrafast manipulation of topologically enhanced surface transport driven by mid-infrared and terahertz pulses in Bi2Se3. Nat. Commun. 10, 607 (2019). [cited by applicant]
Mikami, H., Gao, L. & Goda, K. Ultrafast optical imaging technology: principles and applications of emerging methods. Nanophotonics 5, 441-453 (2016). [cited by applicant]
Mittleman, D. M. Twenty years of terahertz imaging [Invited]. Opt. Express 26, 9417 (2018). [cited by applicant]
Nakagawa, K. et al. Sequentially timed all-optical mapping photography (STAMP). Nat. Photonics 8, 695-700 (2014). [cited by applicant]
Olivieri, L. et al. Hyperspectral terahertz microscopy via nonlinear ghost imaging. Optica 7, 186 (2020). [cited by applicant]
Poulin, P. R. Irreversible organic crystalline chemistry monitored in real time. Science. 313, 1756-1760 (2006). [cited by applicant]
Qingli Zhou, Q. Z. & Xicheng Zhang, X. Z. Applications of time-resolved terahertz spectroscopy in ultrafast carrier dynamics (Invited Paper). Chinese Opt. Lett. 9, 110006-110009 (2011). [cited by applicant]
Richter, C. & Schmuttenmaer, C. A. Exciton-like trap states limit electron mobility in TiO2 nanotubes. Nat. Nanotechnol. 5, 769-772 (2010). [cited by applicant]
Shan, J. et al. Single-shot measurement of terahertz electromagnetic pulses by use of electro-optic sampling. Opt. Lett. 25, 426 (2000). [cited by applicant]
Šiaulys, N., Gallais, L. & Melninkaitis, A. Direct holographic imaging of ultrafast laser damage process in thin films. Opt. Lett. 39, 2164 (2014). [cited by applicant]
Stantchev, R. I. et al. Noninvasive, near-field terahertz imaging of hidden objects using a single-pixel detector. Sci. Adv. 2, (2016). [cited by applicant]
Stantchev, R. I., Yu, X., Blu, T. & Pickwell-MacPherson, E. Real-time terahertz imaging with a single-pixel detector. Nat. Commun. 11, 2535 (2020). [cited by applicant]
Sun, Q. et al. Recent advances in terahertz technology for biomedical applications. Quant. Imaging Med. Surg. 7, 345-355 (2017). [cited by applicant]
Suzuki, T. et al. Sequentially timed all-optical mapping photography (STAMP) utilizing spectral filtering. Opt. Express 23, 30512 (2015). [cited by applicant]
Takasawa, K. et al. Single-Shot 2-D Burst Ultrafast THz Imaging Utilizing SF-STAMP. in 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) Part F140—, 1-1 (IE… [cited by applicant]
Teo, S. M., Ofori-Okai, B. K., Werley, C. A. & Nelson, K. A. Invited Article: Single-shot THz detection techniques optimized for multidimensional THz spectroscopy. Rev. Sci. Instrum. 86, 051301 (2015). [cited by applicant]
Tomasino, A. et al. Wideband THz Time Domain Spectroscopy based on Optical Rectification and Electro-Optic Sampling. Sci. Rep. 3, 3116 (2013). [cited by applicant]
Tonouchi, M. Cutting-edge terahertz technology. Nat. Photonics 1, 97-105 (2007). [cited by applicant]
Ulbricht, R., Hendry, E., Shan, J., Heinz, T. F. & Bonn, M. Carrier dynamics in semiconductors studied with time-resolved terahertz spectroscopy. Rev. Mod. Phys. 83, 543-586 (2011). [cited by applicant]
Wang, X., Cui, Y., Sun, W., Ye, J. & Zhang, Y. Terahertz polarization real-time imaging based on balanced electro-optic detection. J. Opt. Soc. Am. A 27, 2387 (2010). [cited by applicant]
Yue, Q.-Y., Cheng, Z.-J., Han, L., Yang, Y. & Guo, C.-S. One-shot time-resolved holographic polarization microscopy for imaging laser-induced ultrafast phenomena. Opt. Express 25, 14182 (2017). [cited by applicant]
Zhai, Z. H. et al. Time-resolved single-shot terahertz time-domain spectroscopy for ultrafast irreversible processes. Rev. Sci. Instrum. 87, (2016). [cited by applicant]
Zhao, J., E, Y., Williams, K., Zhang, X. & Boyd, R. Spatial Sampling of Terahertz Fields with Sub-wavelength Accuracyvia Probe Beam Encoding. Light Sci. Appl. (2019). doi:10.1038/s41377-019-0166-6. [cited by applicant]