IP Library Granted Patent US 7,365,045
Granted Patent B2
US 7,365,045 · App. 11/094,113 · Granted Apr 29, 2008

Aqueous cleaner with low metal etch rate comprising alkanolamine and tetraalkylammonium hydroxide

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Quick Facts
Patent No.
US 7,365,045
App. No.
11/094,113
Granted
Apr 29, 2008
Kind
B2
Abstract

A cleaning solution is provided for cleaning metal-containing microelectronic substrates, particularly for post etch, via formation and post CMP cleaning. The cleaning solution consists of a quaternary ammonium hydroxide, an organic amine, and water. A preferred cleaning solution consists of tetramethylammonium hydroxide, monoethanolamine, and water. The pH of cleaning solution is greater than 10.

Claims (21)

1. A cleaning composition for cleaning microelectronic substrates, consisting of:

0.30 to 22.0% by weight alkanolamine;

0.02 to 13.5% by weight tetramethylammonium hydroxide;

balance water,

wherein the alkanolamine is selected from the group consisting of 1-amino-2 propanol, 2-(methylamino)ethanol and mixtures thereof, and wherein the cleaning composition is useful for removing residue from a microelectronic substrate having same thereon.

2. The composition according to claim 1 wherein the pH of the composition is greater than 10.

3. The composition according to claim 1 wherein the residue comprises post-chemical mechanical polishing (CMP) residue.

4. A cleaning composition for cleaning microelectronic substrates consisting of:

0.09 to 22.0% by weight alkanolamine;

0.02 to 13.5% by weight tetrabutylammonium hydroxide; balance water,

wherein the alkanolamine is selected from the group consisting of monoethanolamine, 1-amino-2 propanol, 2-(methylamino)ethanol, triethanolamine and mixtures thereof.

5. The composition according to claim 4 wherein the pH of the composition is greater than 10.

6. A composition according to claim 1 wherein said alkanolamine is present in an amount between 0.30 and 0.70% by weight, said tetramethylammonium hydroxide is present in an amount between 0.02 to 0.70% by weight, balance water.

7. A method of fabricating a microelectronic substrate comprising: (a) CMP processing a metal-containing substrate to form a chemical mechanical polishing (CMP) processing substrate; and (b) cleaning said CMP processed substrate with the cleaning composition of claim 1 .

8. A method of fabricating a microelectronic substrate comprising: (a) CMP processing a metal-containing substrate to form a CMP processing substrate; and (b) cleaning said CMP processed substrate with the cleaning composition of claim 4 .

9. The method of claim 7 , wherein the microelectronic substrate comprises at least one of Cu, Al, W, TiN, Ta, TiW and Silica.

10. The method of claim 7 , wherein the metal comprises copper.

11. The method of claim 7 , wherein the cleaning of said processed substrate is carried out at temperature in a range from ambient temperature to about 70° C.

12. The method of claim 8 , wherein the microelectronic substrate comprises at least one of Cu, Al, W, TiN, Ta, TiW and Silica.

13. The method of claim 8 , wherein the metal comprises copper.

14. The method of claim 8 , wherein the cleaning of said processed substrate is carried out at temperature in a range from ambient temperature to about 70° C.

Assignments (6)
SECURITY INTEREST Recorded Jul 8, 2022
From: ENTEGRIS, INC.; ENTEGRIS GP, INC.; POCO GRAPHITE, INC.; CMC MATERIALS, INC.; INTERNATIONAL TEST SOLUTIONS, LLC; QED TECHNOLOGIES INTERNATIONAL, INC.
To: TRUIST BANK, AS NOTES COLLATERAL AGENT
Reel/Frame 060613/0072 →
ASSIGNMENT OF PATENT SECURITY INTEREST RECORDED AT REEL/FRAME 048811/0679 Recorded Nov 5, 2019
From: GOLDMAN SACHS BANK USA
To: MORGAN STANLEY SENIOR FUNDING, INC.
Reel/Frame 050965/0035 →
SECURITY INTEREST Recorded Nov 13, 2018
From: ENTEGRIS, INC.; SAES PURE GAS, INC.
To: GOLDMAN SACHS BANK USA
Reel/Frame 048811/0679 →
RELEASE OF SECURITY INTEREST Recorded Nov 8, 2018
From: GOLDMAN SACHS BANK USA, AS COLLATERAL AGENT
To: ENTEGRIS, INC.; POCO GRAPHITE, INC.; ATMI, INC.; ATMI PACKAGING, INC.; ADVANCED TECHNOLOGY MATERIALS, INC.
Reel/Frame 047477/0032 →
RELEASE OF SECURITY INTEREST Recorded Nov 8, 2018
From: GOLDMAN SACHS BANK USA, AS COLLATERAL AGENT
To: ENTEGRIS, INC.; POCO GRAPHITE, INC.; ATMI, INC.; ATMI PACKAGING, INC.; ADVANCED TECHNOLOGY MATERIALS, INC.
Reel/Frame 047477/0151 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 19, 2016
From: ADVANCED TECHNOLOGY MATERIALS, INC.
To: ENTEGRIS, INC.
Reel/Frame 041029/0903 →