IP Library Granted Patent US 10,266,822
Granted Patent B2
US 10,266,822 · App. 15/269,259 · Granted Apr 23, 2019

Spinal muscular atrophy (SMA) treatment via targeting of SMN2 splice site inhibitory sequences

Inventors: Ravindra N. Singh (Shrewsbury, MA); Natalia N. Singh (Shrewsbury, MA); Nirmal K. Singh (Temple, TX); Elliot J. Androphy (Natick, MA)
Assignee: UNIVERSITY OF MASSACHUSETTS
C12N15/113G01N33/6896C12N2310/11C12N2310/315C12N2310/322C12N2320/33G01N2500/04G01N2800/28
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Quick Facts
Patent No.
US 10,266,822
App. No.
15/269,259
Granted
Apr 23, 2019
Kind
B2
Abstract

The present invention is directed to methods and compositions capable of blocking the inhibitory effect of a newly-identified intronic inhibitory sequence element, named ISS-N1 (for “intronic splicing silencer”), located in the SMN2 gene. The compositions and methods of the instant invention include oligonucleotide reagents (e.g., oligoribonucleotides) that effectively target the SMN2 ISS-N1 site in the SMN2 pre-mRNA, thereby modulating the splicing of SMN2 pre-mRNA to include exon 7 in the processed transcript. The ISS-N1 blocking agents of the invention cause elevated expression of SMN protein, thus compensating for the loss of SMN protein expression commonly observed in subjects with spinal muscular atrophy (SMA).

Claims (19)

1. A method of increasing the level of exon 7-containing SMN2 mRNA in a cell or cell extract comprising contacting the cell or cell extract with an oligonucleotide, which oligonucleotide comprises a sequence sufficiently complementary to intron 7 of the SMN2 gene over the entire length of the oligonucleotide and sufficiently complementary to the sequence CCAGCAUUAUGAAAG (SEQ ID NO:3), such that the level of exon 7-containing SMN2 mRNA in the cell is increased.

2. The method of claim 1 , wherein the oligonucleotide is between about 5 and about 50 nucleotides in length.

3. The method of claim 1 , wherein the oligonucleotide is modified by substitution of at least one nucleotide with a modified nucleotide such that in vivo stability is enhanced as compared to an unmodified oligonucleotide.

4. The method of claim 3 , wherein the modified nucleotide is selected from the group consisting of: a sugar-modified nucleotide; a nucleobase-modified nucleotide; a 2′-deoxy ribonucleotide; a 2′-O-methyl ribonucleotide; a 2′-fluoro modified ribonucleotide; a 2′-amino modified ribonucleotide; a 2′-thio modified ribonucleotide; a 5-bromo-uridine; a 5-iodo-uridine; a 5-methyl-cytidine; a ribo-thymidine; a 2-aminopurine; a 5-fluoro-cytidine; a 5-fluoro-uridine; a 2,6-diaminopurine; a 4-thio-uridine; a 5-amino-allyl-uridine; a backbone-modified nucleotide; and a locked nucleic acid (LNA).

5. The method of claim 4 , wherein the 2′-deoxy ribonucleotide is 2′-deoxy adenosine or 2′-deoxy guanosine.

6. The method of claim 4 , wherein the 2′-fluoro modified nucleotide is 2′-fluoro-cytidine, 2′-fluoro-uridine, 2′-fluoro-adenosine, or 2′-fluoro-guanosine, or wherein the 2′-amino modified ribonucleotide is 2′-amino-cytidine, 2′-amino-uridine, 2′-amino-adenosine, 2′-amino-guanosine or 2′-amino-butyryl-pyrene-uridine.

7. The method of claim 4 , wherein the backbone-modified nucleotide contains a phosphorothioate group.

8. The method of claim 1 , wherein the cell or cell extract is a spinal muscular atrophy (SMA) patient-derived neuronal cell, muscle cell or fibroblast, or extract thereof.

9. The method of claim 1 , wherein the cell or cell extract is selected from the group consisting of an embryonic stem cell, an embryonic stem cell extract, a neuronal stem cell and a neuronal stem cell extract.

10. A method of increasing the level of exon 7-containing SMN2 mRNA in an organism, comprising administering to the organism an oligonucleotide, which oligonucleotide comprises a sequence sufficiently complementary to intron 7 of the SMN2gene over the entire length of the oligonucleotide and sufficiently complementary to the sequence CCAGCAUUAUGAAAG (SEQ ID NO:3), such that the level of exon 7-containing SMN2 mRNA in the organism is increased.

11. The method of claim 10 , wherein the organism is a mammal.

12. The method of claim 10 , wherein the organism is a human.

13. The method of claim 10 , wherein the human has spinal muscular atrophy (SMA).

14. A method of treating spinal muscular atrophy (SMA) in a patient, comprising administering to the patient an oligonucleotide, which oligonucleotide comprises a sequence sufficiently complementary to intron 7 of the SMN2 gene over the entire length of the oligonucleotide and sufficiently complementary to the sequence CCAGCAUUAUGAAAG (SEQ ID NO:3), in a dose effective to increase the level of exon 7-containing SMN2 mRNA in cells of the patient, such that SMA in the patient is treated.

15. A method of treating a subject that would benefit from increased levels of exon 7-containing SMN2mRNA in neuronal cells, comprising administering to the patient an oligonucleotide, which oligonucleotide comprises a sequence sufficiently complementary to intron 7 of the SMN2 gene over the entire length of the oligonucleotide and sufficiently complementary to the sequence CCAGCAUUAUGAAAG (SEQ ID NO:3), in a dose effective to increase the level of exon 7-containing SMN2 mRNA in cells of the subject.

16. The method of claim 15 , wherein the subject is suffering from amyotrophic lateral sclerosis (ALS).

17. A method of increasing the level of exon 7-containing SMN2 mRNA in a cell comprising contacting the cell with an oligonucleotide, which oligonucleotide comprises a sequence that is sufficiently complementary to a sequence selected from SEQ ID NO: 3, and SEQ ID NO: 40-66; such that the level of exon 7-containing SMN2mRNA in the cell is increased.

18. A method of increasing the level of exon 7-containing SMN2 mRNA in a cell comprising contacting the cell with an oligonucleotide, which oligonucleotide comprises a sequence sufficiently complementary to intron 7 of the SMN2 gene over the entire length of the oligonucleotide and complementary to nucleotide 1 and 6 of the sequence CCAGCAUUAUGAAAG (SEQ ID NO:3), such that the level of exon 7-containing SMN2 mRNA in the cell is increased.

19. The method of claim 1 , wherein the oligonucleotide is between about 8 and about 19 nucleotides in length or between about 8 and about 14 nucleotides in length.

Assignments (2)
CONFIRMATORY LICENSE Recorded Feb 13, 2017
From: UNIVERSITY OF MASSACHUSETTS MEDICAL SCH
To: NATIONAL INSTITUTES OF HEALTH (NIH), U.S. DEPT. OF HEALTH AND HUMAN SERVICES (DHHS), U.S. GOVERNMENT
Reel/Frame 041690/0082 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 16, 2016
From: SINGH, RAVINDRA N.; SINGH, NATALIA N.; SINGH, NIRMAL K.; ANDROPHY, ELLIOT J.
To: UNIVERSITY OF MASSACHUSETTS
Reel/Frame 040631/0097 →
Continuity (6)
Continuation 14054055 · Oct 15, 2013
Continuation 13329926 · Dec 19, 2011
Continuation 12545536 · Aug 21, 2009
Division 11295725 · Dec 5, 2005
Provisional Application 60633325 · Dec 3, 2004
Related Publication 20170096664A1 · Apr 6, 2017
Cited By (1)
US 12,241,065