IP Library Granted Patent US 10,197,547
Granted Patent B2
US 10,197,547 · App. 15/677,231 · Granted Feb 5, 2019

Methods of analyzing crude oil

Inventors: Robert Graham Cooks (West Lafayette, IN); Fred Paul Mark Jjunju (West Lafayette, IN); Anyin Li (West Lafayette, IN); Iman S. Roqan (Thuwal, SA)
Assignee: Purdue Research Foundation
G01N33/2823G01N30/724G01N30/7266H01J49/0031H01J49/04H01J49/10H01J49/164
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Quick Facts
Patent No.
US 10,197,547
App. No.
15/677,231
Granted
Feb 5, 2019
Kind
B2
Abstract

The invention generally relates to methods of analyzing crude oil. In certain embodiments, methods of the invention involve obtaining a crude oil sample, and subjecting the crude oil sample to mass spectrometry analysis. In certain embodiments, the method is performed without any sample pre-purification steps.

Claims (11)

1. A method for quantifying a corrosion inhibitor in crude oil, the method comprising:

obtaining a crude oil sample comprising a corrosion inhibitor;

subjecting the crude oil sample to mass spectrometry analysis comprising introducing the crude oil sample to a paper substrate and applying solvent and voltage to the crude oil sample on the substrate to generate ions of the corrosion inhibitor directly and only from the crude oil sample, wherein the applying step is conducted without an external heat source; and

quantifying the corrosion inhibitor in the crude oil sample based on results of the mass spectrometry analysis, wherein the method is performed without any sample pre-purification steps.

2. The method according to claim 1 , wherein the mass spectrometer is selected from the group consisting of a bench-top mass spectrometer and a miniature mass spectrometer.

3. The method according to claim 1 , wherein the paper is filter paper.

4. The method according to claim 1 , wherein the corrosion inhibitor comprises at least one alkyl ammonium salt.

5. The method according to claim 4 , wherein the alkyl ammonium salt is selected from the group consisting of tetradodecylammonium bromide, benzylhexadecyldimethylammonium chloride, and a combination thereof.

6. The method according to claim 1 , wherein the mass spectrometer is coupled with a discontinuous atmospheric pressure interface.

7. The method according to claim 1 , wherein the solvent comprises a mixture of methanol and acetonitrile.

8. The method according to claim 1 , wherein the mass spectrometry analysis is performed in an ambient environment.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 24, 2019
From: COOKS, ROBERT GRAHAM; LI, ANYIN
To: PURDUE RESEARCH FOUNDATION
Reel/Frame 050470/0440 →
CONFIRMATORY LICENSE Recorded Apr 10, 2018
From: PURDUE UNIVERSITY
To: UNITED STATES DEPARTMENT OF ENERGY
Reel/Frame 045889/0038 →
Continuity (3)
Continuation 14426879
Provisional Application 61759097 · Jan 31, 2013
Related Publication 20170343526A1 · Nov 30, 2017