IP Library › Granted Patent US 11,420,879
Granted Patent B2
US 11,420,879 · App. 16/825,638 · Granted Aug 23, 2022

Conductive, anticorrosive magnesium titanium oxide material

Inventors: Soo Kim (Cambridge, MA); Jonathan Mailoa (Cambridge, MA); Lei Cheng (San Jose, CA); Charles Tuffile (Swansea, MA)
Assignee: Robert Bosch GmbH
C01G23/006H01M4/8663H01M4/8803C01P2002/90C01P2006/40C01P2006/90
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Quick Facts
Patent No.
US 11,420,879
App. No.
16/825,638
Granted
Aug 23, 2022
Kind
B2
Abstract

An anticorrosive, conductive material includes a first oxide having oxygen vacancies and a formula (I): MgTi 2 O 5-δ (I), where δ is any number between 0 and 3 optionally including a fractional part denoting the oxygen vacancies; and a second oxide having a formula (II): Ti a O b (II), where 1<=a<=20 and 1<=b<=30, optionally including a fractional part, the first and second oxides of formulas (I) and (II) forming a polycrystalline matrix.

Claims (41)

1. An anticorrosive, conductive material comprising:

a first oxide having oxygen vacancies and a formula (I):

MgTi 2 O 5-δ   (I),

where δ is any number between 0 and 3 including a fractional part denoting the oxygen vacancies; and

a second oxide having a formula (II):

Ti a O b   (II),

where 1<=a<=20 and 1<=b<=30, optionally including a fractional part,

the first and second oxides of formulas (I) and (II) forming a polycrystalline matrix.

2. The material of claim 1 , wherein the second oxide is metallic.

3. The material of claim 1 , wherein Ti a O b is Ti 2 O 3 .

4. The material of claim 3 , wherein Ti 2 O 3 forms a segregated polycrystalline phase.

5. The material of claim 3 , wherein Ti 2 O 3 is located within about 1 nm to about 100 μm from grain boundaries of the matrix.

6. The material of claim 1 , wherein the matrix comprises at least about 0.5 wt. % Ti a O b , based on the total weight of the material.

7. The material of claim 1 , wherein at least one of the first and second oxides of formulas (I) and (II) comprises a dopant including Ge, Nb, Mo, Sn, Ta, W, or a combination thereof.

8. The material of claim 1 , wherein at least one of the first and second oxides of formulas (I) and (II) comprises a conducting agent.

9. A fuel cell system comprising:

an anticorrosive, conductive polycrystalline matrix having:

a first metal oxide having oxygen vacancies and a formula (I):

MgTi 2 O 5-δ   (I),

where δ is any number between 0 and 3 including a fractional part denoting the oxygen vacancies; and

a second metal oxide having a formula (II):

Ti a O b   (II),

where 1<=a<=20 and 1<=b<=30, optionally including a fractional part.

10. The system of claim 9 , wherein Ti a O b is Ti 2 O 3 .

11. The system of claim 10 , wherein Ti 2 O 3 forms a segregated polycrystalline phase within the matrix.

12. The system of claim 10 , wherein Ti 2 O 3 is located about 1 nm to about 100 μm from grain boundaries of the matrix.

13. The system of claim 9 , wherein the matrix comprises about at least about 0.5 wt. % Ti a O b , based on the total weight of the matrix.

14. The system of claim 9 , wherein at least one of the first and second oxides comprises a dopant including Ge, Nb, Mo, Sn, Ta, W, or a combination thereof.

15. The system of claim 9 further comprising a bipolar plate including the anticorrosive, conductive polycrystalline matrix.

16. A fuel cell catalyst support material comprising:

a first metal oxide having oxygen vacancies and a formula (I):

MgTi 2 O 5-δ   (I),

where δ is any number between 0 and 3 including a fractional part denoting the oxygen vacancies; and

a second metal oxide having a formula (II):

Ti a O b   (II),

where 1<=a<=20 and 1<=b<=30, optionally including a fractional part,

the first and second oxides forming a polycrystalline matrix.

17. The material of claim 16 , wherein Ti a O b is Ti 2 O 3 .

18. The material of claim 17 , wherein Ti 2 O 3 forms a segregated polycrystalline phase.

19. The material of claim 17 , wherein Ti 2 O 3 is located about 1 nm to about 100 μm from grain boundaries of the matrix.

20. The material of claim 16 , wherein the matrix comprises at least about 0.5 wt. % Ti a O b , based on the total weight of the material.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 20, 2020
From: KIM, SOO; MAILOA, JONATHAN; CHENG, LEI; TUFFILE, CHARLES
To: ROBERT BOSCH GMBH
Reel/Frame 052180/0793 →
Continuity (2)
Continuation In Part 16675538 · Nov 6, 2019
Related Publication 20210130186A1 · May 6, 2021
Cited By (1)
US 12,503,782