IP Library Granted Patent US 11,927,708
Granted Patent B2
US 11,927,708 · App. 17/992,004 · Granted Mar 12, 2024

Dense high-speed scintillator material of low afterglow

Inventors: Bernard Ferrand (Voreppe, FR); Bruno Viana (Montgeron, FR); Ludivine Pidol (Cachan, FR); Pieter Dorenbos (GM Rijswijk, NL)
Assignee: LUXIUM SOLUTIONS, LLC
G01T1/2023C09K11/745C09K11/77742C09K11/77744G21K4/00A61B6/4258
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Quick Facts
Patent No.
US 11,927,708
App. No.
17/992,004
Granted
Mar 12, 2024
Kind
B2
Abstract

The invention relates to an inorganic scintillator material of formula Lu (2−y) Y (y−z−x) Ce x M z Si (1−v) M′ v O 5 , in which: M represents a divalent alkaline earth metal and M′ represents a trivalent metal, (z+v) being greater than or equal to 0.0001 and less than or equal to 0.2; z being greater than or equal to 0 and less than or equal to 0.2; v being greater than or equal to 0 and less than or equal to 0.2; x being greater than or equal to 0.0001 and less than 0.1; and y ranging from (x+z) to 1. In particular, this material may equip scintillation detectors for applications in industry, for the medical field (scanners) and/or for detection in oil drilling. The presence of Ca in the crystal reduces the afterglow, while stopping power for high-energy radiation remains high.

Claims (35)

1. An inorganic LYSO-type scintillator material comprising Lu, Y, Si, O, Ce, and Ca wherein:

the relative amounts of Lu, Y, Si, O, Ce, and Ca satisfy formula (2):

Lu (2-y) Y (y-z-x) Ce x Ca z SiO 5   (2),

z is greater than or equal to 0.0001 and less than 0.05;

x is greater than or equal to 0.0001 and less than 0.1; and

y is from (x+z) to 1.

2. The inorganic scintillator material according to claim 1 , wherein z is less than to 0.01.

3. The inorganic scintillator material according to claim 1 , wherein z is between 0.0002 and 0.001.

4. The inorganic scintillator material according to claim 1 , wherein x is greater than 0.0001 and less than 0.001.

5. An inorganic LYSO-type scintillator material comprising Lu, Y, Si, O, Ce, and Ca wherein:

the relative amounts of Lu, Y, Si, 0, Ce, and Ca satisfy formula (2):

Lu (2-y) Y (y-z-x) Ce x Ca z SiO 5   (2),

z is greater than or equal to 0.0001 and less than 0.05;

x is greater than or equal to 0.0001 and less than 0.1;

y is from (x+z) to 1; and

the inorganic scintillator material is a single crystal.

6. The inorganic scintillator material according to claim 5 , wherein z is less than to 0.01.

7. The inorganic scintillator material according to claim 5 , wherein z is between 0.0002 and 0.001.

8. The inorganic scintillator material according to claim 5 , wherein x is greater than 0.0001 and less than 0.001.

9. A radiation detector comprising an inorganic LYSO-type scintillator material comprising Lu, Y, Si, O, Ce, and Ca wherein:

the relative amounts of Lu, Y, Si, O, Ce, and Ca satisfy formula (2):

Lu (2-y) Y (y-z-x) Ce x Ca z SiO 5   (2),

z is greater than or equal to 0.0001 and less than 0.05;

x is greater than or equal to 0.0001 and less than 0.1; and

y is from (x+z) to 1.

10. The radiation detector according to claim 9 , wherein an inorganic scintillator material is a single crystal.

11. The radiation detector according to claim 9 , wherein the radiation detector is a positron emission tomography detector.

12. The radiation detector according to claim 11 , wherein z is less than to 0.01.

13. The radiation detector according to claim 11 , wherein z is between 0.0002 and 0.001.

14. The radiation detector according to claim 11 , wherein x is greater than 0.0001 and less than 0.001.

15. The radiation detector according to claim 9 , wherein the radiation detector is a time-of-flight positron emission tomography detector.

16. The radiation detector according to claim 9 , wherein the inorganic scintillator material is coupled to a light detector which produces an electrical signal proportional to a number of light pulses received by the light detector and the intensity of the light pulses received by the light detector.

17. The radiation detector according to claim 9 , wherein z is less than to 0.01.

18. The radiation detector according to claim 9 , wherein z is between 0.0002 and 0.001.

19. The radiation detector according to claim 9 , wherein x is greater than 0.0001 and less than 0.001.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 22, 2023
From: SAINT-GOBAIN CRISTAUX ET DETECTEURS
To: LUXIUM SOLUTIONS, LLC
Reel/Frame 063066/0758 →
Priority Claims (1)
FR 0451815 · Aug 9, 2004 · national
Continuity (8)
Continuation 17114841 · Dec 8, 2020
Continuation 16400195 · May 1, 2019
Continuation 15358341 · Nov 22, 2016
Continuation 14039888 · Sep 27, 2013
Continuation 13214648 · Aug 22, 2011
Division 12622881 · Nov 20, 2009
Division 11573323
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